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Point defects exist widely in engineering materials and are known to scatter vibrational modes to reduce thermal conductivity. The Klemens description of point defect scattering is the most prolific analytical model for this effect. This…

Materials Science · Physics 2020-03-11 Ramya Gurunathan , Riley Hanus , Maxwell Dylla , Ankita Katre , G. Jeffrey Snyder

We demonstrate how supercell implementations of conventional lattice dynamical calculations can be used to determine the extent and nature of disorder-induced broadening in the phonon dispersion spectrum of disordered crystalline materials.…

Disordered Systems and Neural Networks · Physics 2017-04-26 Alistair R. Overy , Arkadiy Simonov , Philip A. Chater , Matthew G. Tucker , Andrew L. Goodwin

The coherence properties of mechanical resonators are often limited by multiple unavoidable forms of loss -- including phonon-phonon and phonon-defect scattering -- which result in the scattering of sound into other resonant modes and into…

Quantum Physics · Physics 2016-12-30 Xunnong Xu , Seunghwi Kim , Gaurav Bahl , Jacob M. Taylor

We present a theory and a simulation of thermal diffuse scattering due to the excitation of magnons in scanning transmission electron microscopy. The calculations indicate that magnons can present atomic contrast when detected by electron…

The size-effect of Kondo-scattering in nanometer-sized metallic point contacts is measured with the simplified, mechanically-controlled break-junction technique for CuMn alloy of different Mn concentrations: 0.017; 0.035; and 0.18…

Mesoscale and Nanoscale Physics · Physics 2017-02-14 I. K. Yanson , V. V. Fisun , N. L. Bobrov , J. A. Mydosh , J. M. van Ruitenbeek

We present techniques to model and design membrane phononic crystals with low-mass defects, optimized for force sensing. Further, we identify the importance of the phononic crystal mass contrast as it pertains to the size of acoustic…

Understanding phonon scattering by topological defects in graphene is of particular interest for thermal management in graphene-based devices. We present a study that quantifies the roles of the different mechanisms governing defect phonon…

Materials Science · Physics 2016-11-04 Ziming Zhu , Xiaolong Yang , Mingyuan Huang , Qingfeng He , Guang Yang , Zhao Wang

The lattice dynamics in substitutional disordered alloys with constituents having large size differences is driven by strong disorder in masses, inter-atomic force constants and local environments. In this letter, a new first-principles…

Materials Science · Physics 2016-08-14 Oscar Grånäs , Biswanath Dutta , Subhradip Ghosh , Biplab Sanyal

Small-angle scattering (SAS) intensities observed experimentally are often characterized by the presence of successive power-law regimes with various scattering exponents whose values vary from -4 to -1. This usually indicates multiple…

Statistical Mechanics · Physics 2014-01-31 A. Yu. Cherny , E. M. Anitas , V. A. Osipov , A. I. Kuklin

Interest in high entropy alloy thermoelectric materials is predicated on achieving ultralow lattice thermal conductivity $\kappa\sub{L}$ through large compositional disorder. However, here we show that for a given mechanism, such as mass…

Inelastic and elastic neutron scattering have been used to study a single crystal of the Ni$_{54}$Mn$_{23}$Al$_{23}$ Heusler alloy over a broad temperature range. The paper reports the first experimental determination of the low-lying…

We present the results of a Molecular Dynamics computer simulations of a two component isotope mixture of Lennard-Jones particles, monodisperse in size but different in masses, at a fixed average density and temperature. We study changes in…

Condensed Matter · Physics 2007-05-23 N. Kiriushcheva , S. V. Kuzmin

Because electrons and ions form a coupled system, it is a priori clear that the dynamics of the lattice should reflect symmetry breaking within the electronic degrees of freedom. This has been recently clearly evidenced for the case of…

Strongly Correlated Electrons · Physics 2023-03-03 Léo Mangeolle , Leon Balents , Lucile Savary

Medium and high entropy ceramics, with their distinctive disordered structures, exhibit ultra-low thermal conductivity and high temperature stability. These properties make them strong contenders for next generation thermal barrier coating…

Materials Science · Physics 2024-05-27 Yuxuan Wang , Guoqiang Lan , Jun Song

The new model of phonon transmission across the interface between two crystals is proposed featured by taking into account the mismatch of crystal lattices. It has been found that the mismatch of lattices results in phonon scattering at the…

Other Condensed Matter · Physics 2016-02-22 Aleksandr Meilakhs

The impact of lattice type, period, porosity and thickness of two-dimensional silicon phononic crystals on the reduction of thermal conductance by coherent modification of phonon dispersion is investigated using the theory of elasticity and…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Roman Anufriev , Masahiro Nomura

Phonons diffraction and interference patterns are observed at the atomic scale, using molecular dynamics simulations in systems containing crystalline silicon and nanometric obstacles as voids or amorphous-inclusions. The diffraction…

We use the approximation-free Bold Diagrammatic Monte Carlo technique to study the effects of a finite dispersion of the optical phonon mode on the properties of the Holstein polaron, especially its effective mass. For weak electron-phonon…

Strongly Correlated Electrons · Physics 2013-09-02 Dominic J. J. Marchand , Mona Berciu

We study the effect of nanoscale precipitates on lattice thermal conduction in thermoelectric PbTe using a combination of ab-initio phonon calculations and molecular dynamics. We take into account the effects of mass difference and change…

Materials Science · Physics 2016-11-04 Xiaolong Yang , Jesús Carrete , Zhao Wang

The phonon scattering processes on the three solid phases of ethanol are investigated by means of thermal conductivity, light and neutron scattering measurements as well as molecular dynamics simulations on single-crystalline models for the…

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