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We report inelastic neutron scattering study of a quasi-two-dimensional S=1/2 dimer system Piperazinium Hexachlorodicuprate under hydrostatic pressure. The spin gap {\Delta} becomes softened with the increase of the hydrostatic pressure up…

Strongly Correlated Electrons · Physics 2010-12-01 Tao Hong , C. Stock , I. Cabrera , C. Broholm , Y. Qiu , J. B. Leao , S. J. Poulton , J. R. D. Copley

Piperazinium Hexachlorodicuprate (PHCC) is shown to be a frustrated quasi-two-dimensional quantum Heisenberg antiferromagnet with a gapped spectrum. Zero-field inelastic neutron scattering and susceptibility and specific heat measurements…

Strongly Correlated Electrons · Physics 2009-11-07 M. B. Stone , I. Zaliznyak , Daniel H. Reich , C. Broholm

An inelastic neutron scattering study was performed on a Zn-substituted spin-1/2 Heisenberg 2-leg ladder compound Sr(Cu1-xZnx)2O3 (x < 0.04) to investigate nonmagnetic impurity effects on the quantum spin system with a large spin gap of…

Condensed Matter · Physics 2009-10-30 M. Azuma , M. Takano , R. S. Eccleston

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

Investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet which has a quantum…

We report an inelastic neutron scattering study of magnetic excitations in a quantum paramagnet driven into a magnetically ordered state by chemical substitution, namely Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$ with $x=0.21(2)$. The…

Strongly Correlated Electrons · Physics 2018-12-13 A. Mannig , K. Yu. Povarov , J. Ollivier , A. Zheludev

Neutron elastic scattering measurements have been performed under the hydrostatic pressure in order to investigate the spin structure of the pressure-induced magnetic ordering in the spin gap system TlCuCl$_3$. Below the ordering…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , M. Fujisawa , T. Osakabe , K. Kakurai , H. Tanaka

Inelastic neutron scattering and bulk magnetic susceptibility studies of the quantum S=1/2 spin ladder system IPA-CuCl3 are performed under hydrostatic pressure. The pressure dependence of the spin gap $\Delta$ is determined. At $P=1.5$ GPa…

Strongly Correlated Electrons · Physics 2008-12-10 Tao Hong , V. O. Garlea , A. Zheludev , J. Fernandez-Baca , H. Manaka , S. Chang , J. B. Leao , S. J. Poulton

The quasi-two-dimensional Heisenberg spin $S=1/2$ dimer system bis(2-amino-5-fluoro-pyridinium) tetrachlorocuprate(II) is studied by means of inelastic neutron scattering, calorimetry and nuclear magnetic resonance (NMR) experiments. In the…

Strongly Correlated Electrons · Physics 2019-08-02 Dominic Blosser , Mladen Horvatić , Robert Bewley , Severian Gvasaliya , Andrey Zheludev

Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer…

NH4CuCl3 has two magnetization plateaus at one-quarter and three-quarters of the saturation magnetization, irrespective of the external field direction. Magnetic excitations in NH4CuCl3 have been investigated by means of neutron inelastic…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Ono , K. Kakurai , H. Tanaka

We present results of inelastic neutron scattering study on two bond disordered quasi twodimensional quantum magnets (C$_4$H$_12$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ with x=0.035 and 0.075. We observe the increase of spin gap, reduction of…

Strongly Correlated Electrons · Physics 2013-07-02 D. Huvonen , S. Zhao , G. Ehlers , M. Månsson , S. N. Gvasaliya , A. Zheludev

Inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 have been performed under magnetic fields below and above a critical field Hc at which the energy gap closes.…

Strongly Correlated Electrons · Physics 2007-05-23 M. Hagiwara , L. P. Regnault , A. Zheludev , A. Stunault , N. Metoki , T. Suzuki , S. Suga , K. Kakurai , Y. Koike , P. Vorderwisch , J. H. Chung

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

A study is presented of a two-dimensional frustrated and dimerized quantum spin-system which models the effect of inter-chain coupling in a spin-Peierls compound. Employing a bond-boson method to account for quantum disorder in the ground…

Strongly Correlated Electrons · Physics 2009-10-30 Wolfram Brenig

Inelastic neutron scattering experiments performed on a single crystal of the antiferromagnetic compound Ce$_{0.87}$La$_{0.13}$Ru$_{2}$Si$_{2}$ under applied pressures of up to 5 kbar are reported. A quantum critical point is reached at…

Strongly Correlated Electrons · Physics 2009-11-07 S. Raymond , L. P. Regnault , J. Flouquet , A. Wildes , P. Lejay

Detailed neutron scattering measurements on the bond frustrated magnet ZnCr2S4 reveal a rich H-T phase diagram. The field dependence of the two subsequent antiferromagnetic transitions follows closely that of recently reported structural…

Strongly Correlated Electrons · Physics 2014-06-03 D. Hsieh , Y. W. Li , S. Watauchi , Chang Liu , Q. Huang , R. J. Cava , J. W. Lynn , M. Z. Hasan

Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…

Strongly Correlated Electrons · Physics 2007-11-14 V. O. Garlea , A. Zheludev , L. -P. Regnault , J. -H. Chung , Y. Qiu , M. Boehm , K. Habicht , M. Meissner

Magnetization maesurements under hydrostatic pressure were performed on an S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic field H parallel to the [2,0,1] direction. With increasing applied pressure P, the gap…

Statistical Mechanics · Physics 2009-11-10 Kenji Goto , Masashi Fujisawa , Toshio Ono , Hidekazu Tanaka , Yoshiya Uwatoko

Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic…

Strongly Correlated Electrons · Physics 2025-04-15 Jieming Sheng , Le Wang , Wenrui Jiang , Han Ge , Nan Zhao , Tiantian Li , Maiko Kofu , Dehong Yu , Wei Zhu , Jia-Wei Mei , Zhentao Wang , Liusuo Wu
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