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In this work, we examine how the structure of system-bath interactions can determine commonly encountered temporal decoherence patterns, such as Gaussian and exponential decay, in molecular and other qubits coupled to a thermal bosonic…

Chemical Physics · Physics 2025-02-12 Ignacio Gustin , Xinxian Chen , Ignacio Franco

We discuss a fundamental effect of the interaction-induced decoherence of the electron wave function in disordered metals. In the first part of the paper we consider a simple model of a quantum particle interacting with a bath of harmonic…

Condensed Matter · Physics 2009-10-31 D. S. Golubev , A. D. Zaikin

The processes of radiation damping and decoherence in Quantum Electrodynamics are studied from an open system's point of view. Employing functional techniques of field theory, the degrees of freedom of the radiation field are eliminated to…

Quantum Physics · Physics 2007-05-23 Heinz-Peter Breuer , Francesco Petruccione

We describe a new mechanism of decoherence in excited atoms as a result of thermal particles scattering by the atomic nucleus. It is based on the idea that a single scattering will produce a sudden displacement of the nucleus, which will be…

Quantum Physics · Physics 2017-06-13 Diego A. Quiñones , Benjamin Varcoe

Coulomb interactions that occur in electronic structure calculations are correlated by allowing basis function components of the interacting densities to polarize, thereby reducing the magnitude of the interaction. Exchange integrals of…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

We investigate the impact of electronic correlations and quantum delocalization onto the static structure factor and static density response function of the strongly coupled electron liquid. In contrast to a classical system, the density…

Chemical Physics · Physics 2024-05-21 Tobias Dornheim , Panagiotis Tolias , Jan Vorberger , Zhandos Moldabekov

The decoherence of quantum states defines the transition between the quantum world and classical physics. Decoherence or, analogously, quantum mechanical collapse events pose fundamental questions regarding the interpretation of quantum…

Mesoscale and Nanoscale Physics · Physics 2021-09-24 P. Bredol , H. Boschker , D. Braak , J. Mannhart

Decoherence of electron spins in nanoscale systems is important to quantum technologies such as quantum information processing and magnetometry. It is also an ideal model problem for studying the crossover between quantum and classical…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Wen Yang , Wen-Long Ma , Ren-Bao Liu

Coherence of spins of electrons confined in III-V quantum dots is strongly affected by their hyperfine interaction with the nuclei. In this paper an introduction to this subject will be given. Some theoretical approaches to the problem will…

Mesoscale and Nanoscale Physics · Physics 2016-04-18 Łukasz Cywiński

The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Oleksandr Tsyplyatyev , Daniel Loss

A theory of electronic friction is developed using the exact factorization of the electron-nuclear wavefunction. No assumption is made regarding the electronic bath, which can be made of independent or interacting electrons, and the nuclei…

Quantum Physics · Physics 2022-06-01 Rocco Martinazzo , Irene Burghardt

The question of classicality is addressed in relation with the shape of the nuclear skeleton of molecular systems. As the most natural environment, the electrons of the molecule are considered as continuously monitoring agents for the…

Quantum Physics · Physics 2021-01-05 Edit Matyus , Patrick Cassam-Chenai

Discontinuous changes in the electronic structure upon infinitesimal changes to the Hamiltonian are demonstrated. Remarkably, these are revealed in one and two electron molecular systems if the realm of the nuclear charge is extended to be…

Chemical Physics · Physics 2015-06-16 Aron J. Cohen , Paula Mori-Sánchez

The decoherence induced on a single qubit by its interaction with the environment is studied. The environment is modelled as a scalar two-level boson system that can go through either first order or continuous excited state quantum phase…

Quantum Physics · Physics 2015-05-14 P. Perez-Fernandez , A. Relano , J. M. Arias , J. Dukelsky , J. E. Garcia-Ramos

We characterize both entanglement and quantum coherence in a molecular system by connecting the linear entropy of electronic-nuclear entanglement with Wigner-Yanase skew information measuring vibronic coherence and local quantum uncertainty…

Quantum Physics · Physics 2018-11-21 Mihaela Vatasescu

The concept of correlation is central to all approaches that attempt the description of many-body effects in electronic systems. Multipartite correlation is a quantum information theoretical property that is attributed to quantum states…

I show that the decoherence in a system of $N$ degenerate two--level atoms interacting with a bosonic heat bath is for any number of atoms $N$ governed by a generalized Hamming distance (called ``decoherence metric'') between the superposed…

Quantum Physics · Physics 2009-11-11 Daniel Braun

Minimizing decoherence due to coupling of a quantum system to its fluctuating environment is at the forefront of quantum information science and photonics research. Nature sets the ultimate limit, however, given by the strength of the…

Mesoscale and Nanoscale Physics · Physics 2016-01-27 Galan Moody , Corey McDonald , Ari Feldman , Todd Harvey , Richard P. Mirin , Kevin L. Silverman

Purely quantum electron systems exhibit intriguing correlated electronic phases by virtue of quantum fluctuations in addition to electron-electron interactions. To realize such quantum electron systems, a key ingredient is dense electrons…

We present a quantum solution to the electron spin decoherence by a nuclear pair-correlation method for the electron-nuclear spin dynamics under a strong magnetic field and a temperature high for the nuclear spins but low for the electron.…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Wang Yao , Ren-Bao Liu , L. J. Sham