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Related papers: On Factorization of Molecular Wavefunctions

200 papers

The exact factorization (EF) approach to coupled electron-ion dynamics recasts the time-dependent molecular Schr\"odinger equation as two coupled equations, one for the nuclear wavefunction and one for the conditional electronic…

Chemical Physics · Physics 2019-05-22 Graeme H. Gossel , Lionel Lacombe , Neepa T. Maitra

Density functional theory is generalized to incorporate electron-phonon coupling. A Kohn-Sham equation yielding the electronic density $n_U(\mathbf{r})$, a conditional probability density depending parametrically on the phonon normal mode…

Materials Science · Physics 2019-04-25 Ryan Requist , C. R. Proetto , E. K. U. Gross

We generalize Schroedinger's factorization method for Hydrogen from the conventional separation into angular and radial coordinates to a Cartesian-based factorization. Unique to this approach, is the fact that the Hamiltonian is represented…

Quantum Physics · Physics 2022-01-28 Xinliang Lyu , Christina Daniel , James K. Freericks

We introduce a pseudo-mass parameterized Schr\"odinger-like alchemical equation which contains nuclear charges as variables, treating nuclear charges, nuclear coordinates and electronic coordinates on the equal footing. The eigenfunctions…

Chemical Physics · Physics 2020-12-03 Qing-Long Liu

The position operator (defined within Schroedinger representation as usual) becomes meaningless when the usual Born-von Karman periodic boundary conditions are adopted: this fact is at the root of the polarization problem. I show how to…

Materials Science · Physics 2009-10-31 R. Resta

Shor's factoring algorithm illustrates the potential power of quantum computation. Here we present and numerically investigate a proposal for a compiled version of such an algorithm based on a quantum-wire network exploiting the…

Quantum Physics · Physics 2011-01-14 Fabrizio Buscemi

Schr{\"o}dinger noticed in 1952 that a scalar complex wave function can be made real by a gauge transformation. The author showed recently that one real function is also enough to describe matter in the Dirac equation in an arbitrary…

General Physics · Physics 2022-04-22 Andrey Akhmeteli

The theoretical and computational description of materials properties is a task of utmost scientific and technological importance. A first-principles description of electron-electron interactions poses an immense challenge that is usually…

Chemical Physics · Physics 2022-04-06 Jakub Kocák , Eli Kraisler , Axel Schild

We have implemented a three-dimensional finite element approach, based on tricubic polynomials in spherical coordinates, which solves the Schrodinger equation for scattering of a low energy electron from a molecule, approximating the…

Chemical Physics · Physics 2009-11-10 Stefano Tonzani , Chris H. Greene

This paper gives a new perspective on how to solve the second-order linear differential equation written in normal form. Extending the argument of the potential to a complex number leads to solving exactly the Schr\"odinger equation when…

Quantum Physics · Physics 2023-01-12 Jamal Benbourenane

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

This is a brief review of the Schrodinger's factorization method and its relations to supersymmetric quantum mechanics and its nonlinear (parastatistical, etc) modifications, self-similar infinite soliton potentials, quantum algebras,…

High Energy Physics - Theory · Physics 2007-05-23 V. P. Spiridonov

In a recent paper Cari\~nena et al analyzed a non-polynomial one-dimensional quantum potential representing an oscillator which they argued was intermediate between the harmonic and isotonic oscillators. In particular they proved that it is…

Quantum Physics · Physics 2009-02-19 Jonathan M Fellows , Robert A Smith

There are different ways to obtain an exact one-electron theory for a many-electron system, and the exact electron factorization (EEF) is one of them. In the EEF, the Schr\"odinger equation for one electron in the environment of other…

Chemical Physics · Physics 2022-04-06 Jakub Kocák , Eli Kraisler , Axel Schild

Conventional theoretical and computational approaches to fully coupled quantum molecular dynamics, i.e. when both the electrons and nuclei are treated as quantum-mechanical particles, are impractical for all but the smallest chemical…

Chemical Physics · Physics 2025-10-10 Julian Stetzler , Sophya Garashchuk , Vitaly A. Rassolov

It was recently shown [Phys. Rev. Lett. 105, 123002 (2010)] that the complete wavefunction for a system of electrons and nuclei evolving in a time-dependent external potential can be exactly factorized into an electronic wavefunction and a…

Chemical Physics · Physics 2015-06-11 Ali Abedi , Neepa T. Maitra , E. K. U. Gross

This paper systematically develops the Schr\"odinger formalism that is valid also for gyrotropic media where the material weights $W = \left ( \begin{smallmatrix} \varepsilon & \chi \chi^* & \mu \end{smallmatrix} \right ) \neq \overline{W}$…

Optics · Physics 2018-09-26 Giuseppe De Nittis , Max Lein

A recent article by Lohmiller \& Slotine (Proc.\ R.\ Soc.\ A \textbf{482}: 20250413) claims that the Schr\"odinger equation can be solved exactly using only classical least action and classical fluid density, asserting that this formulation…

Quantum Physics · Physics 2026-05-05 Gabor Vattay

The Schr\"odinger theory of electrons in an external electromagnetic field can be described from the perspective of the individual electron via the `Quantal Newtonian' laws (or differential virial theorems). These laws are in terms of…

Quantum Physics · Physics 2016-11-23 Viraht Sahni , Xiao-Yin Pan

A set of factorization energies is introduced, giving rise to a generalization of the Schr\"{o}dinger (or Infeld and Hull) factorization for the radial hydrogen-like Hamiltonian. An algebraic intertwining technique involving such…

Quantum Physics · Physics 2008-11-26 J. Oscar Rosas-Ortiz