Related papers: Rydberg blockade with multivalent atoms: engineeri…
We show that the dipole-dipole interaction between two Rydberg atoms can give rise to long range molecules. The binding potential arises from two states that converge to different separated atom asymptotes. These states interact weakly at…
We demonstrate Rydberg blockade due to the charge-dipole interaction between a single Rb atom and a single RbCs molecule confined in optical tweezers. The molecule is formed by magnetoassociation of a Rb+Cs atom pair and subsequently…
We report on the experimental characterization of various types of spin-exchange interactions between two individual atoms, where pseudo-spin degrees of freedom are encoded in different Rydberg states. For the case of the direct…
Using the reactance matrix approach, we systematically develop new multichannel quantum defect theory models for the singlet and triplet S, P, D and F states of strontium based on improved energy level measurements. The new models reveal…
We demonstrate experimentally that a single Rb atom excited to the $79d_{5/2}$ level blocks the subsequent excitation of a second atom located more than $10 \mu\rm m$ away. The observed probability of double excitation of $\sim 30%$ is…
We report the creation of ultralong-range Sr$_2$ molecules comprising one ground-state $5s^2$ $^1S_0$ atom and one atom in a $5sns$ $^3S_1$ Rydberg state for $n$ ranging from 29 to 36. Molecules are created in a trapped ultracold atomic gas…
Interaction between Rydberg atoms can significantly modify Rydberg excitation dynamics. Under a resonant driving field the Rydberg-Rydberg interaction in high-lying states can induce shifts in the atomic resonance such that a secondary…
We report on the observation of ultralong range interactions in a gas of cold Rubidium Rydberg atoms. The van-der-Waals interaction between a pair of Rydberg atoms separated as far as 100,000 Bohr radii features two important effects:…
We discuss the computational complexity of finding the ground state of the two-dimensional array of quantum bits that interact via strong van der Waals interactions. Specifically, we focus on systems where the interaction strength between…
High resolution laser Stark excitation of np (60 < n < 85) Rydberg states of ultra-cold cesium atoms shows an efficient blockade of the excitation attributed to long-range dipole-dipole interaction. The dipole blockade effect is observed as…
Rydberg states of atoms are of great current interest for quantum manipulation of mesoscopic samples of atoms. Long-range Rydberg-Rydberg interactions can inhibit multiple excitations of atoms under the appropriate conditions. These…
We report on the direct measurement of the van der Waals interaction between two isolated, single Rydberg atoms separated by a controlled distance of a few micrometers. By working in a regime where the single-atom Rabi frequency of the…
The structure and photoexcitation dynamics of high lying doubly excited states of the strontium atom with high angular momenta are studied in the vicinity of the Sr$^+(N=5)$ threshold. The spectra recorded using resonant multiphoton…
Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their…
Blockade effects on the single quantum level are at the heart of quantum devices like single-electron transistors. The blockade mechanisms are based on strong interactions like the Coulomb interaction in case of single electrons. Neutral…
Assemblies of Rydberg atoms subject to resonant dipole-dipole interactions form Frenkel excitons. We show that van-der-Waals shifts can significantly modify the exciton wave function, whenever atoms approach each other closely. As a result,…
The dipole-dipole interaction among ultra-cold Rydberg atoms is simulated. We examine a general interaction scheme in which two atoms excited to the x and x' states are converted to y and y' states via a Forster resonance. The atoms are…
High resolution laser excitation of np Rydberg states of cesium atoms shows a dipole blockade at F\"{o}rster resonances corresponding to the resonant dipole-dipole energy transfer of the np + np → ns + (n + 1)s reaction. The…
$^{87}{\rm Rb}$ atoms are known to have long-lived Rydberg excited states with controllable excitation amplitude (detuning) and strong repulsive van der Waals interaction $V_{{\bf r} {\bf r'}}$ between excited atoms at sites ${\bf r}$ and…
Motivated by experimental advances [e.g. A. Ga{\"e}tan {\it et.al.} Nat. Phys. 5 115 (2009)] that the collective excitation of two Rydberg atoms was observed, we provide an elaborate theoretical study for the dynamical behavior of two-atom…