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Related papers: Generation of 1.5-octave intense infrared pulses b…

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Octave-spanning, 12.5 fs, (1.9 cycle) pulses with 115 {\mu}J energy in the short-wavelength mid-infrared spectral range (1-2.5 {\mu}m) have been generated via phase-mismatched cascaded nonlinear frequency conversion using organic DAST…

Optics · Physics 2015-06-17 A. Trisorio , M. Divall , C. P. Hauri

High energy terahertz pulses are produced by optical rectification (OR) in organic crystals DAST and DSTMS by a Ti:sapphire amplifier system centered at 0.8 microns. The simple scheme provides broadband spectra between 1 and 5 THz, when…

Optics · Physics 2015-06-17 B. Monoszlai , C. Vicario , M. Jazbinsek , C. P. Hauri

Generating energetic femtosecond mid-IR pulses is crucial for ultrafast spectroscopy, and currently relies on parametric processes that, while efficient, are also complex. Here we experimentally show a simple alternative that uses a single…

Optics · Physics 2015-04-10 B. B. Zhou , H. R. Guo , M. Bache

We report the generation of intense deep ultraviolet pulses at 200 nm with a duration of 48 fs and pulse energy of 130 uJ, achieved via cascaded sum frequency generation using 800 nm femtosecond pulses in barium borate crystals. Efficient…

Optics · Physics 2025-07-04 X. Xie , S. Soultanis , G. Knopp , A. L. Cavalieri , S. L. Johnson

We report on the development of tunable few-cycle pulses with central wavelengths from 1.6 um to 2 um. Theses pulses were used as a proof of principle for high harmonic generation in atomic and molecular targets. In order to generate such…

We report on the generation of nanosecond mid-infrared pulses having frequency tunability, a narrow linewidth, and a high pulse energy. These pulses are obtained by frequency mixing between injection-seeded near-infrared pulses in potassium…

The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses…

Optics · Physics 2023-03-08 Yuxuan Wei , Jiaming Le , Chuanshan Tian

We report on the generation of broadband, high-energy femtosecond pulses centered at 1.28 um by stimulated Raman scattering in pressurized hydrogen cell. Stimulated Raman scattering is performed by two chirped and delayed pulses originating…

We present a numerical parametric study of single-cycle electromagnetic pulse generation in a DAST/SiO2 multilayer structure via collinear optical rectification of 800 nm femtosecond laser pulses. It is shown that modifications of the…

We demonstrate a fibre-based approach that generates mid-infrared femtosecond pulses in the 3-4 {\mu}m spectral region with microjoule-level single pulse energy. This is realised in a piece of gas-filled antiresonant hollow-core fibre that…

We report a multi-microjoule, ultra-broadband mid-infrared optical parametric amplifier based on a GaSe nonlinear crystal pumped at ~2 {\mu}m. The generated idler pulse has a flat spectrum spanning from 4.5 to 13.3 {\mu}m at -3 dB and 4.2…

Optics · Physics 2019-07-30 Kun Liu , Houkun Liang , Lifeng Wang , Shizhen Qu , Tino Lang , Hao Li , Qi Jie Wang , Ying Zhang

The availability of intense, ultrashort coherent radiation sources in the infrared region of the spectrum is enabling the generation of attosecond X-ray pulses via high harmonic generation, pump-probe experiments in the "molecular…

We demonstrate an efficient procedure for terahertz-wave radiation generation by applying a nonlinear wavelength conversion approach using a mid-infrared pump source. We used a 3.3 {\mu}m dual-chirped optical parametric amplification source…

Cascaded nonlinearities have attracted much interest, but ultrafast applications have been seriously hampered by the simultaneous requirements of being near phase-matching and having ultrafast femtosecond response times. Here we show that…

Optics · Physics 2012-10-24 B. B. Zhou , A. Chong , F. W. Wise , M. Bache

We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagom\'e-style photonic crystal fiber. By pumping with ultrashort, few $\mu$J, pulses…

Periodically poled thin film lithium niobate waveguides provide simultaneous access to efficient second and third order nonlinear processes, enabling broadband generation of coherent laser light. Here, we demonstrate the generation of a…

Bright and broadband coherent mid-IR radiation is important for exciting and probing molecular vibrations. Using cascaded nonlinearities in conventional quadratic nonlinear crystal like lithium niobate, self-defocusing near-IR solitons have…

Optics · Physics 2016-07-01 Binbin Zhou , Morten Bache

BGGSe is a newly developed nonlinear material that is attractive for ultrabroad frequency mixing and ultrashort pulse generation due to its comparably low dispersion and high damage threshold.In a first experiment, we show that a long…

We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary…

We report on a high-power mid-infrared frequency comb source based on a femtosecond Er:fiber oscillator with a stabilized repetition rate at 250 MHz. The mid-infrared frequency comb is produced through difference frequency generation in a…

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