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The isotope $^{229}$Th is unique in that it possesses an isomeric state of only a few eV above the ground state, suitable for nuclear laser excitation. An optical clock based on this transition is expected to be a very sensitive probe for…

The hyperfine structure of $^{229}$Th$^{3+}$ ions in the nuclear ground state is investigated via laser spectroscopy of trapped Th$^{3+}$ ions that are sympathetically cooled by laser-cooled $^{88}$Sr$^+$ ions in a linear Paul trap. The…

Atomic Physics · Physics 2025-04-02 G. Zitzer , J. Tiedau , Ch. E. Düllmann , M. V. Okhapkin , E. Peik

The hyperfine splitting of the ground and low-energy $3/2^+(7.8 \pm 0.5$ eV) levels in the $^{229}$Th nucleus in muonic atom ($\mu^-_{1S_{1/2}}{}^{229}$Th$)^*$ has been calculated considering the distribution of the nuclear magnetization in…

Nuclear Theory · Physics 2016-07-20 E. V. Tkalya

The isomeric first excited state of the isotope 229Th exhibits the lowest nuclear excitation energy in the whole landscape of known atomic nuclei. For a long time this energy was reported in the literature as 3.5(5) eV, however, a new…

Nuclear Experiment · Physics 2015-06-12 L. v. d. Wense , P. G. Thirolf , D. Kalb , M. Laatiaoui

The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…

A measurement of the hyperfine coefficients and isotope shifts for the Dy I 421.291 nm transition [$4f^{10}6s^2 (J=8)\to4f^{10}6s6p (J=9)$] using atomic beam laser-induced fluorescence spectroscopy is presented. A King Plot analysis is…

Atomic Physics · Physics 2015-05-13 N. Leefer , A Cingöz , D. Budker

The electromagnetic transition between the almost degenerate 5/2+ and 3/2+ states in Th229 is deemed to be very sensitive to potential changes in the fine structure constant alpha. State of the art Hartree-Fock and Hartree-Fock-Bogoliubov…

Nuclear Theory · Physics 2009-08-18 Elena Litvinova , Hans Feldmeier , Jacek Dobaczewski , Victor Flambaum

We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou

We calculate hyperfine structure of $^{229}$Th and its ions (Th~IV, Th~III, Th~II, Th~I) to reveal the dependence of the nuclear clock frequency on the hyperfine interaction (hfi). We calculate first and second-order hfi shifts and…

Atomic Physics · Physics 2023-12-18 V. A. Dzuba , V. V. Flambaum

We demonstrate a technique for frequency measurements of UV transitions with sub-MHz precision. The frequency is measured using a ring-cavity resonator whose length is calibrated against a reference laser locked to the $D_2$ line of…

Atomic Physics · Physics 2007-05-23 Ayan Banerjee , Umakant D. Rapol , Dipankar Das , Anusha Krishna , Vasant Natarajan

We have produced laser-cooled Wigner crystals of 229Th3+ in a linear Paul trap. The magnetic dipole (A) and electric quadrupole (B) hyperfine constants for four low-lying electronic levels and the relative isotope shifts with respect to…

Atomic Physics · Physics 2011-10-12 C. J. Campbell , A. G. Radnaev , A. Kuzmich

$^{229}$Th, a crucial candidate for nuclear clocks and many other applications, is a typical heavy nucleus with an extremely low-energy isomeric state $^{229m}$Th. A detailed study of the nuclear structure of $^{229}$Th is performed here by…

Nuclear Theory · Physics 2025-08-28 Zi-Rui Chen , Long-Jun Wang , Yuanbin Wu

We identify a potential means to extract the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy from precision microwave spectroscopy of the $5F_{5/2,7/2}$ hyperfine manifolds in the ion $^{229g}$Th$^{3+}$. The hyperfine…

Atomic Physics · Physics 2014-02-14 K. Beloy

The thorium nucleus with mass number $A=229$ has attracted much interest because its extremely low lying first excited isomeric state at about $8$eV opens the possibility for the development of a nuclear clock. However, neither the exact…

Isotope shifts and hyperfine structure of tungsten were studied in the near UV range. We have used laser induced fluorescence spectroscopy on a pulsed supersonic beam to probe the 5D0 -> 5F1 transition at 384.9 nm, 7S3 -> 7P4 transition at…

Atomic Physics · Physics 2015-06-12 Jeongwon Lee , Jinhai Chen , Aaron Leanhardt

$^{229}$Th with a low-lying nuclear isomeric state is an essential candidate for a nuclear clock as well as many other applications. Laser excitation of the isomeric state has been a long-standing goal. With relativistic $^{229}$Th ions in…

The lowest-known excited state in nuclei is the 7.6 eV isomer of 229Th. This energy is within the range of laser-based investigations that could allow accurate measurements of possible temporal variation of this energy splitting. This in…

Nuclear Theory · Physics 2008-11-26 A. C. Hayes , J. L Friar , P. Moller

We report measurements of the isotope shifts of the 3d6 4s2 a 5D3 - 3d6 4s4p z 5F4o FeI resonance line at 373.7 nm between all four stable isotopes 54Fe, 56Fe, 57Fe and 58Fe, as well as the complete hyperfine structure of that line for…

Atomic Physics · Physics 2012-05-15 S. Krins , N. Huet , T. Bastin

We measure isotope shifts for five Yb$^+$ isotopes with zero nuclear spin on two narrow optical quadrupole transitions ${}^2S_{1/2} \rightarrow {}^2D_{3/2}$, ${}^2S_{1/2} \rightarrow {}^2D_{5/2}$ with an accuracy of $\sim 300$ Hz. The…

Excitation of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+, 8.28 \pm 0.17$ eV) in the process of inelastic electron scattering is studied theoretically in the framework of the perturbation theory for the quantum…

Nuclear Theory · Physics 2020-07-01 E. V. Tkalya
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