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Structural phase transition can occur due to complex mechanisms other than simple dynamical instability, especially when the parent and daughter structure is of low dimension. This article reports such an inversion symmetry-breaking…

The structure and vibrational density of states (VDOS) of polymer glasses are investigated using numerical simulations based on the classical Kremer-Grest bead-spring model. We focus on the roles of chain length and bending stiffness, the…

Soft Condensed Matter · Physics 2018-02-16 Rico Milkus , Christopher Ness , Vladimir V. Palyulin , Jana Weber , Alexei Lapkin , Alessio Zaccone

We report measurements of vibrational mode shapes of mechanical resonators made from ultrathin carbon nanomembranes (CNMs) with a thickness of approximately 1 nm. CNMs are prepared from electron irradiation induced cross-linking of aromatic…

Materials Science · Physics 2018-04-30 Xianghui Zhang , Reimar Waitz , Fan Yang , Carolin Lutz , Polina Angelova , Armin Gölzhäuser , Elke Scheer

Adsorbed atoms and molecules play an important role in controlling and tuning the functional properties of two-dimensional (2D) materials. Understanding and predicting this process from theory is challenging because of the need to capture…

Mesoscale and Nanoscale Physics · Physics 2017-07-12 Fabiano Corsetti , Arash A. Mostofi , Johannes Lischner

We study a phononic crystal interacting with an artificial atom { a superconducting quantum system { in the quantum regime. The phononic crystal is made of a long lattice of narrow metallic stripes on a quatz surface. The artificial atom in…

Inspired by recent visible pump - infrared probe spectra reported for molecular catalysts adsorbed to quantum dots, we introduce a theory of non-equilibrium vibronic Fano resonances arising from the interference of quantum dot excited-state…

Chemical Physics · Physics 2024-10-16 Luis Martinez-Gomez , Sara T. Gebre , Tianquan Lian , Raphael F. Ribeiro

Carbon nanotubes have attracted considerable interest for their unique electronic properties. They are fascinating candidates for fundamental studies of one dimensional materials as well as for future molecular electronics applications. The…

We study the vicinal surface of the restricted solid-on-solid model coupled with the Langmuir adsorbates which we regard as two-dimensional lattice gas without lateral interaction. The effect of the vapor pressure of the adsorbates in the…

Statistical Mechanics · Physics 2009-11-07 Noriko Akutsu , Yasuhiro Akutsu , Takao Yamamoto

The electronic spectra of carbon nanotubes and other nanoscale systems are quantized because of their small radii. Similar quantization in the phonon spectra has been difficult to observe because of the far smaller energy scale. We probed…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 J. Hone , B. Batlogg , Z. Benes , A. T. Johnson , J. E. Fischer

The dynamic structure factor and the eigenmodes of density fluctuations in the uniform liquid $^3$He are studied using a novel non-perturbative approach. This new version of the self-consistent method of moments invokes up to nine sum rules…

Computational Physics · Physics 2023-11-10 A. V. Filinov , J. Ara , I. M. Tkachenko

We investigate theoretically the spectrum of resonance fluorescence of a harmonically trapped atom, whose internal transitions are $\Lambda$--shaped and driven at two-photon resonance by a pair of lasers, which cool the center--of--mass…

Quantum Physics · Physics 2009-11-10 Marc Bienert , Wolfgang Merkel , Giovanna Morigi

Phonon spectra of CdSe nanoplatelets (2-6 ML) with the zinc-blende structure were calculated from first principles within the density-functional theory. It turned out that the Lamb modes in nanoplatelets are in fact optical rather than…

Materials Science · Physics 2017-11-29 Alexander I. Lebedev

In this manuscript, we provide a general theory for how surface phonons couple to molecular adsorbates. Our theory maps the extended dynamics of a surface's atomic vibrational motions to a generalized Langevin equation, and by doing so…

Chemical Physics · Physics 2024-05-03 Ardavan Farahvash , Adam P. Willard

We develop a formalism to describe the discrete-time dynamics of systems containing an arbitrary number of interacting species. The individual-based model, which forms our starting point, is described by a Markov chain, which in the limit…

Statistical Mechanics · Physics 2014-10-06 César Parra-Rojas , Joseph D. Challenger , Duccio Fanelli , Alan J. McKane

We present analytical model and molecular dynamics simulations of phonon heat transport in nanowires and nanoribbons with anharmonic lattices and dynamically rough surfaces and edges. In agreement with recent experiments on heat transport…

Statistical Mechanics · Physics 2011-12-30 Yuriy A. Kosevich , Alexander V. Savin

We develop a microscopic calculation scheme for the excitation spectrum of a single-electron atom localized near a dielectric nanostructure. The atom originally has an arbitrary degenerate structure of its Zeeman sublevels on its closed…

Quantum Physics · Physics 2024-02-02 N. A. Moroz , L. V. Gerasimov , A. D. Manukhova , D. V. Kupriyanov

We theoretically study the quantum dynamics of transverse vibrations of a one-dimensional chain of trapped ions in harmonic potentials interacting via a Reggeon-type cubic nonlinearity that is nonunitary but preserves PT symmetry. We…

Quantum Gases · Physics 2013-11-13 Philipp Strack , Vincenzo Vitelli

We consider a one-dimensional lattice model with the nearest-neighbor interaction $V_1$ and the next-nearest neighbor interaction $V_2$ with filling factor 1/2 at zero temperature. The particles are assumed to be spinless fermions or…

Condensed Matter · Physics 2009-10-30 E. V. Tsiper , A. L. Efros

Raman spectroscopy has been the most extensively employed method to study carbon nanotubes at high pressures. This review covers reversible pressure-induced changes of the lattice dynamics and structure of single- and multi-wall carbon…

Condensed Matter · Physics 2009-09-29 I. Loa

As the length-scales of materials decrease, heterogeneities associated with interfaces approach the importance of the surrounding materials. Emergent electronic and magnetic interface properties in superlattices have been studied…

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