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Related papers: First-principles interatomic potentials for ten el…

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We show that a deep-learning neural network potential (DP) based on density functional theory (DFT) calculations can well describe Cu-Zr materials, an example of a binary alloy system that can coexist in several ordered intermetallics and…

Materials Science · Physics 2020-04-29 Christopher M. Andolina , Philip Williamson , Wissam A. Saidi

We introduce the alchemical harmonic approximation (AHA) of the absolute electronic energy for charge-neutral iso-electronic diatomics at fixed interatomic distance $d_0$. To account for variations in distance, we combine AHA with this…

Chemical Physics · Physics 2024-12-10 Simon León Krug , Danish Khan , O. Anatole von Lilienfeld

We propose an efficient scheme, which combines density functional theory (DFT) with deep potentials (DP), to systematically study the convergence issues of the computed electronic thermal conductivity of warm dense Al (2.7 g/cm$^3$,…

Computational Physics · Physics 2024-06-19 Qianrui Liu , Junyi Li , Mohan Chen

To date, density functional theory (DFT) is one of the most accurate and yet practical theory to gain insight about materials properties. Although successful, the computational cost is the main hurdle even today. A way out is combining DFT…

Materials Science · Physics 2019-04-19 Shweta Mehta , Sheena Agarwal , Kavita Joshi

We present a physically motivated strategy for the construction of training sets for transferable machine learning interatomic potentials. It is based on a systematic exploration of all possible space groups in random crystal structures,…

Materials Science · Physics 2023-03-29 Marvin Poul , Liam Huber , Erik Bitzek , Jörg Neugebauer

In recent years there has been great progress in the use of machine learning algorithms to develop interatomic potential models. Machine-learned potential models are typically orders of magnitude faster than density functional theory but…

Materials Science · Physics 2023-03-28 Alberto Hernandez , Tim Mueller

Developing reliable interatomic potential models with quantified predictive accuracy is crucial for atomistic simulations. Commonly used potentials, such as those constructed through the embedded atom method (EAM), are derived from…

Materials Science · Physics 2022-08-05 Arun Hegde , Elan Weiss , Wolfgang Windl , Habib N. Najm , Cosmin Safta

Molecular dynamics simulations provide a versatile framework to study interfacial heat transport, but their accuracy remains limited by the accuracy of available interatomic potentials. In the past, researchers have adopted the use of…

Materials Science · Physics 2021-05-11 Spencer Wyant , Andrew Rohskopf , Asegun Henry

The unique properties exhibited in immiscible metals, such as excellent strength, hardness, and radiation-damage tolerance, have stimulated the interest of many researchers. As a typical immiscible metal system, the Cu-W nano-multilayers…

Materials Science · Physics 2024-07-02 Jiahao Pan , Huiqun Cheng , Gaosheng Yan , Lei Zhang , Wenshan Yu , Shengping Shen

A recently proposed class of machine-learning interatomic potentials --- Moment tensor potentials (MTPs) --- is investigated in this work. MTPs are able to actively select configurations and parametrize the potential on-the-fly. It is shown…

Computational Physics · Physics 2018-12-11 I. I. Novoselov , A. V. Yanilkin , A. V. Shapeev , E. V. Podryabinkin

First-principles based modeling on phonon dynamics and transport using density functional theory and Boltzmann transport equation has proven powerful in predicting thermal conductivity of crystalline materials, but it remains unfeasible for…

Materials Science · Physics 2019-07-23 Xin Qian , Shenyou Peng , Xiaobo Li , Yujie Wei , Ronggui Yang

We present a study on the transport and materials properties of aluminum spanning from ambient to warm dense matter conditions using a machine-learned interatomic potential (ML-IAP). Prior research has utilized ML-IAPs to simulate phenomena…

The advent of neural-network-based deep learning techniques has led to the emergence of increasingly sophisticated numerical interatomic potentials, including graph neural networks and large language-motivated foundation models.…

Chemical Physics · Physics 2026-03-09 Susan R. Atlas

We investigate shock-compressed copper in the warm dense matter regime by means of density functional theory molecular dynamics simulations. We use neural-network-driven interatomic potentials to increase the size of the simulation box and…

Other Condensed Matter · Physics 2022-12-07 Maximilian Schörner , Bastian B. L. Witte , Andrew D. Baczewski , Attila Cangi , Ronald Redmer

The central approximation made in classical molecular dynamics simulation of materials is the interatomic potential used to calculate the forces on the atoms. Great effort and ingenuity is required to construct viable functional forms and…

Computational Physics · Physics 2019-06-26 Mitchell A. Wood , Mary Alice Cusentino , Brian D. Wirth , Aidan P. Thompson

Plasmonic near-field transducers (NFTs) play a key role in administering nanoscale heating for a number of applications ranging from medical devices to next generation data processing technology. We present a novel multi-scale approach,…

Uranium mononitride (UN) is a promising accident-tolerant fuel because of its high fissile density and high thermal conductivity. In this study, we developed the first machine learning interatomic potentials for reliable atomic-scale…

The success of first principles electronic structure calculation for predictive modeling in chemistry, solid state physics, and materials science is constrained by the limitations on simulated length and time scales due to computational…

Materials Science · Physics 2018-12-19 Albert P. Bartok , James Kermode , Noam Bernstein , Gabor Csanyi

The influence of pressure on the structural and elastic properties of ScM (M = Rh, Cu, Ag, Hg) compounds has been performed by using ab initio approach pseudopotential plane- wave method based on the density functional theory within the…

Materials Science · Physics 2016-05-18 Md. Lokman Ali , Md. Zahidur Rahaman , Md. Atikur Rahman

We compare the predicted phase behaviour of lead (Pb) using three different interatomic potential models, including an embedded atom method (EAM), a modified embedded atom method (MEAM), and a neural network-based machine-learned model in…