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We study the prototype 5d pyrochlore iridate Y2Ir2O7 from first principles using the local density approximation and dynamical mean-field theory (LDA+DMFT). We map out the phase diagram in the space of temperature, onsite Coulomb repulsion…

Strongly Correlated Electrons · Physics 2015-10-14 Hiroshi Shinaoka , Shintaro Hoshino , Matthias Troyer , Philipp Werner

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

Strongly Correlated Electrons · Physics 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a prototypical example of the pyrochlore iridates. The density of states, the Fermi surface, and the near Fermi level band dispersion in the plane…

Strongly Correlated Electrons · Physics 2013-11-14 Q. Wang , Y. Cao , X. G. Wan , J. D. Denlinger , T. F. Qi , O. B. Korneta , G. Cao , D. S. Dessau

The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

Strongly Correlated Electrons · Physics 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher

We study the band structure topology and engineering from the interplay between local moments and itinerant electrons in the context of pyrochlore iridates. For the metallic iridate Pr$_2$Ir$_2$O$_7$, the Ir $5d$ conduction electrons…

Strongly Correlated Electrons · Physics 2018-12-12 Xu Ping Yao , Gang Chen

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central…

Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

We perform combined density functional and dynamical mean-field calculations to study the pyrochlore iridates Lu$_2$Ir$_2$O$_7$, Y$_2$Ir$_2$O$_7$ and Eu$_2$Ir$_2$O$_7$. Both single-site and cluster dynamical mean-field calculations are…

Strongly Correlated Electrons · Physics 2017-01-27 Runzhi Wang , Ara Go , Andrew J. Millis

In 5d transition metal oxides such as the iridates, novel properties arise from the interplay of electron correlations and spin-orbit interactions. We investigate the electronic structure of the pyrochlore iridates, (such as…

Strongly Correlated Electrons · Physics 2015-05-19 Xiangang Wan , Ari Turner , Ashvin Vishwanath , Sergey Y. Savrasov

Polycrystalline Nd2Ru2O7 samples have been prepared and examined using a combination of structural, magnetic, and electrical and thermal transport studies. Analysis of synchrotron X-ray and neutron diffraction patterns suggests some site…

Our single crystal study of the magneto-thermal and transport properties of the pyrochlore iridate Eu2Ir2O7 reveals a continuous phase transition from a paramagnetic metal to an antiferromagnetic insulator for a sample with stoichiometry…

Strongly Correlated Electrons · Physics 2015-06-04 Jun J. Ishikawa , Eoin C. T. O'Farrell , Satoru Nakatsuji

First-principles calculations are performed to investigate f magnetism in A$_2$Ti$_2$O$_7$ (A=Eu, Gd, Tb, Dy, Ho, Er, Yb) magnetic pyrochlore oxides. The Hubbard U parameter and the relativistic spin orbit correction is applied for more…

Strongly Correlated Electrons · Physics 2015-12-09 Najmeh Deilynazar , Elham Khorasani , Mojtaba Alaei , S. Javad Hashemifar

Strong electronic interactions and spin orbit coupling can be conducive for realizing novel broken symmetry phases supporting quasiparticles with nontrivial band topology. 227 pyrochlore iridates provide a suitable material platform for…

Strongly Correlated Electrons · Physics 2017-02-22 Pallab Goswami , Bitan Roy , Sankar Das Sarma

In the pyrochlore iridates, \textit{R}$_{2}$Ir$_{2}$O$_{7}$ (\textit{R} = Lanthanide, Y), determination of the magnetic structure of the iridium moments remains an outstanding problem despite the role this is expected to play in the…

Strongly Correlated Electrons · Physics 2014-06-23 Steven M. Disseler

A comprehensive study of the structural properties of the heavily investigated rare-earth A2Ir2O7 series under extreme conditions is presented. The series is covered by studying iridates with A = Pr, Sm, Dy-Lu. Temperature- and…

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

Strongly Correlated Electrons · Physics 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

We present an ab initio pseudopotential local density functional calculation for stoichiometric high-Tc cuprate YBa_2Cu_3O_7 using the plane-wave basis set. We have overcome well-known difficulties in applying pseudopotential methods to…

Condensed Matter · Physics 2009-10-22 Hanchul Kim , Jisoon Ihm

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

First principles density functional calculations within the local spin density approximation (LSDA) and the generalized gradient approximation (GGA) are reported for pyrochlore Cd$_2$Os$_2$O$_7$ and Cd$_{2}$Re$_{2}$O$_7$. The transition…

Condensed Matter · Physics 2009-11-07 D. J. Singh , P. Blaha , K. Schwarz , J. O. Sofo
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