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In this work, we report a pronounced light upconversion in few-layer transition metal dichalcogenides. Our joint theory-experiment study attributes the upconversion photoluminescence to a resonant exciton-exciton annihilation involving a…

We examine the photoluminescence of highly-excited exciton-polariton condensates in semiconductor microcavities. Under strong pumping, exciton-polariton condensates have been observed to undergo a lasing transition where strong coupling…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Natsuko Ishida , Tim Byrnes , Tomoyuki Horikiri , Franco Nori , Yoshihisa Yamamoto

Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that…

Mesoscale and Nanoscale Physics · Physics 2022-03-02 Valentin Walther , Lida Zhang , Susanne F. Yelin , Thomas Pohl

Semiconductor nanoparticles and nanostructures in the strong coupling regime exhibit an intriguing energy scale in the optical frequencies, which is specified by the Rabi splitting between the upper and lower exciton-polariton states.…

Optics · Physics 2019-11-19 Burak Gerislioglu , Arash Ahmadivand

Reversible exchange of photons between a material and an optical cavity can lead to the formation of hybrid light--matter states where material properties such as the work function\cite{Hutchison_AM2013a}, chemical…

There is an increasing scientific and technological interest on the design and implementation of nanoscale sources of quantum light. Here, we investigate the quantum statistics of the light scattered from a plasmonic nanocavity coupled to a…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 R. Sáez-Blázquez , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

Semiconductors in all dimensionalities ranging from 0D quantum dots and molecules to 3D bulk crystals support bound electron-hole pair quasiparticles termed as excitons. Over the past two decades, the emergence of a variety of…

Materials Science · Physics 2021-08-03 Surendra B. Anantharaman , Kiyoung Jo , Deep Jariwala

We propose a system of highly efficient photoemitters comprising metal-dielectric (plasmonic-excitonic) multilayered structures. In the proposed structure, the absorption in the excitonic layer is greatly enhanced through quantum…

Mesoscale and Nanoscale Physics · Physics 2017-08-17 Takuya Matsuda , Hajime Ishihara

Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…

Optics · Physics 2024-10-22 Adam D. Alfieri , Tobia Ruth , Cheryl Lim , Jason Lynch , Deep Jariwala

Semiconductor microcavities are widely used to study collective interactions of cavity exciton-polaritons leading to their condensation phenomenon. Exciton-light interaction is highly enhanced in such structures due to the resonance…

Mesoscale and Nanoscale Physics · Physics 2014-07-17 Mikhail Lebedev , Andrey Parakhonsky , Andrey Demenev

We theoretically investigate up-conversion process of entangled two photons on a dimer molecule, which is coupled by a cavity or nanoscale metallic structure. Within one-dimensional input-output theory, the propagators of the photons are…

Mesoscale and Nanoscale Physics · Physics 2015-10-01 Yoshiki Osaka , Nobuhiko Yokoshi , Masatoshi Nakatani , Hajime Ishihara

Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…

Optics · Physics 2025-02-18 Tom Hoekstra , Jorik van de Groep

Plexciton is the formation of new hybridized energy states originated from the coupling between plasmon and exciton. To reveal the optical properties of both exciton and plexciton, we develop a classic oscillator model to describe the…

Optics · Physics 2022-07-12 Yuqing Cheng , Mengtao Sun

Photoluminescence is commonly used to identify the electronic structure of individual nanotubes. But, nanotubes naturally occur in bundles. Thus, we investigate photoluminescence of nanotube bundles. We show that their complex spectra are…

Materials Science · Physics 2015-05-13 P. H. Tan , A. G. Rozhin , T. Hasan , P. Hu , V. Scardaci , W. I. Milne , A. C. Ferrari

In this work, we theoretically investigate the optical orientation and alignment of excitons in quantum dots with weak electron-hole exchange interaction and long exciton radiative lifetimes. This particular regime is realized in…

Mesoscale and Nanoscale Physics · Physics 2023-08-30 D. S. Smirnov , E. L. Ivchenko

Interlayer excitons in two dimensional semiconductor heterostructures show suppressed electron-hole overlap resulting in longer radiative lifetimes as compared to intralyer excitons. Such tightly bound interlayer excitons are relevant for…

Controlled non-local energy and coherence transfer enables light harvesting in photosynthesis and non-local logical operations in quantum computing. The most relevant mechanism of coherent coupling of distant qubits is coupling via the…

Photoinduced Kerr rotation by more than $\pi /2$ radians is demonstrated in planar quantum well microcavity in the strong coupling regime. This result is close to the predicted theoretical maximum of $\pi $. It is achieved by engineering…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 R. V. Cherbunin , M. Vladimirova , K. V. Kavokin , A. V. Mikhailov , N. E. Kopteva , P. G. Lagoudakis , A. V. Kavokin

Exciton-polaritons in semiconductors are quasi-particles which have recently shown the capability to undergo phase transition into a coherent hybrid state of light and matter. The observation of such quasi-particles in organic microcavities…

Thin film interference is integral to modern photonics and optoelectronics, e.g. allowing for precise design of high performance optical filters, efficiency enhancements in photovoltaics and light-emitting devices, as well as the…

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