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The 5d iridates have been the subject of much recent attention due to the predictions of a large array of novel electronic phases driven by twisting strong spin-orbit coupling and Hubbard correlation. As a prototype, the single layered…

Materials Science · Physics 2015-03-10 Chengliang Lu , Shuai Dong , Andy Quindeau , Daniele Preziosi , Ni Hu , Marin Alexe

The nature of the electronic groundstate of Ba2IrO4 has been addressed using soft X-ray absorption and inelastic scattering techniques in the vicinity of the oxygen K edge. From the polarization and angular dependence of XAS we deduce an…

Strongly Correlated Electrons · Physics 2014-03-06 M. Moretti Sala , M. Rossi , S. Boseggia , J. Akimitsu , N. B. Brookes , M. Isobe , M. Minola , H. Okabe , H. M. Ronnow , L. Simonelli , D. F. McMorrow , G. Monaco

Crystal structure of spinel compound CuIr$_{2}$S$_{4}$ was examined by powder X-ray diffraction for the insulating phase below the metal-insulator transition at $T_{MI}$ = 230 K. The superstructure spots are reproduced by considering the…

Strongly Correlated Electrons · Physics 2007-05-23 T. Furubayashi , T. Matsumoto , S. Nagata

Employing $\textit{ab-initio}$ density functional theory (DFT), we performed a systematic investigation of the electronic structures and the magnetic properties of atomic bilayers composed of a 4$d$ transition-metal layer (Rh, Pd and Ru)…

Materials Science · Physics 2023-12-08 Souvik Paul , Stefan Heinze

The checkerboard lattice, with alternating 'crossed' plaquettes, serves as the two dimensional analog of the pyrochlore lattice. The corner sharing plaquette structure leads to a hugely degenerate ground state, and no magnetic order, for…

Strongly Correlated Electrons · Physics 2017-01-24 Nyayabanta Swain , Pinaki Majumdar

We investigate the metal-insulator transition in the layered Ruddelsden Popper series of strontium iridates Srn+1IrnO3n+1. Tight-binding models of t2g orbitals for n = 1, 2, and infinity are constructed, and changes in band dispersion due…

Strongly Correlated Electrons · Physics 2015-06-05 Jean-Michel Carter , V. Vijay Shankar , Hae-Young Kee

We study the thermodynamic and high-magnetic-field properties of the magnetic insulator Ba$_5$CuIr$_3$O$_{12}$, which shows no magnetic order down to 2 K consistent with a spin liquid ground state. While the temperature dependence of the…

Strongly Correlated Electrons · Physics 2020-01-20 Pavel A. Volkov , Choong-Jae Won , D. I. Gorbunov , Jae-Wook Kim , Mai Ye , Heung-Sik Kim , J. H. Pixley , Sang-Wook Cheong , G. Blumberg

We study a bandwidth controlled Mott metal-insulator transition (MIT) between a Fermi liquid metal and a quantum spin-liquid insulator at half-filling in three dimensions (3D). Using a slave rotor approach, and incorporating gauge field…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Arun Paramekanti , Yong Baek Kim , T. Senthil

We synthesize and study single crystals of a new double-perovskite Sr2YIrO6. Despite two strongly unfavorable conditions for magnetic order, namely, pentavalent Ir5+(5d4) ions which are anticipated to have Jeff=0 singlet ground states in…

Strongly Correlated Electrons · Physics 2014-02-18 G. Cao , T. F. Qi , L. Li , J. Terzic , S. J. Yuan , L. E. DeLong , G. Murthy , R. K. Kaul

We have investigated magneto-transport properties in a single crystal of pyrochore-type Nd2Ir2O7. The metallic conduction is observed on the antiferromagnetic domain walls of the all-in all-out type Ir-5d moment ordered insulating bulk…

Materials Science · Physics 2016-10-31 K. Ueda , J. Fujioka , B. -J. Yang , J. Shiogai , A. Tsukazaki , S. Nakamura , S. Awaji , N. Nagaosa , Y. Tokura

We report the observation of metal-like to insulator transition (MTI) in the 3dpyrochlore oxide Tb2Ti2O7 at 603 K due to the interaction of empty 3d orbitals of Ti4+ with O2- ions, evidenced by the transition in resistivity. Magnetisation,…

Materials Science · Physics 2020-07-28 B. Santhosh Kumar , C. Venkateswaran

{\it Ab initio} analyses of A$_2$IrO$_4$ (A=Sr, Ba) are presented. Effective Hubbard-type models for Ir 5$d$ $t_{2g}$ manifolds downfolded from the global band structure are solved based on the dynamical mean-field theory. The results for…

Strongly Correlated Electrons · Physics 2012-03-02 R. Arita , J. Kuneš , A. V. Kozhevnikov , A. G. Eguiluz , M. Imada

A major challenge in condensed matter physics is integrating topological phenomena with correlated electron physics to leverage both types of states for next-generation quantum devices. Metal-insulator transitions (MITs) are central to…

A new mechanism of the Verway transition in magnetite (Fe3O4), which has been argued to be a charge ordering transition so far, is proposed. Based on the mean field calculations for the three band model of spinless fermions appropriate for…

Strongly Correlated Electrons · Physics 2007-05-23 Hitoshi Seo , Masao Ogata , Hidetoshi Fukuyama

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

We report the evolution of structural, magnetic and dielectric properties due to partial substitution of Ba by Sr in the high temperature multiferroic YBaCuFeO5. This compound exhibits ferroelectric and antiferromagnetic transitions around…

Materials Science · Physics 2017-05-31 Surender lal , Sanjay K. Upadhyay , K. Mukherjee , C. S. Yadav

4Hb-TaS2 has been proposed to possess unconventional superconductivity with broken time reveral symmetry due to distinctive layered structure, featuring a heterojunction between a 2D triangular Mott insulator and a charge density wave…

Strongly Correlated Electrons · Physics 2024-06-18 Junho Bang , Byeongin Lee , Hyungryul Yang , Sunghun Kim , Dirk Wulferding , Doohee Cho

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

An anapole state that breaks inversion and time reversal symmetries with preserving translation symmetry of underlying lattice has aroused great interest as a new quantum state, but only a few candidate materials have been reported.…

Strongly Correlated Electrons · Physics 2021-02-10 H. Murayama , K. Ishida , R. Kurihara , T. Ono , Y. Sato , Y. Kasahara , H. Watanabe , Y. Yanase , G. Cao , Y. Mizukami , T. Shibauchi , Y. Matsuda , S. Kasahara

TiPO$_4$ shows interesting structural and magnetic properties as temperature and pressure are varied, such as a spin-Peierls phase transition and the development of incommensurate modulations of the lattice. Recently, high pressure…

Strongly Correlated Electrons · Physics 2019-06-26 H. Johan M. Jönsson , Marcus Ekholm , Maxim Bykov , Leonid Dubrovinsky , Sander van Smaalen , Igor A. Abrikosov