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A quantum memory at microwave frequencies, able to store the state of multiple superconducting qubits for long times, is a key element for quantum information processing. Electronic and nuclear spins are natural candidates for the storage…
Diamonds with nitrogen-vacancy (NV) center ensembles are one of the most promising solid-state quantum platforms for various sensing applications. The combination of a long spin dephasing time ($T_2^*$) and a high NV center concentration is…
Sensitive nanoscale magnetic resonance imaging (MRI) of target spins using nitrogen-vacancy (NV) centers in diamond will require a quantitative understanding of dominant noise at the surface. We probe this noise by applying dynamical…
The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…
We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…
Solid-state spin systems including nitrogen-vacancy (NV) centers in diamond constitute an increasingly favored quantum sensing platform. However, present NV ensemble devices exhibit sensitivities orders of magnitude away from theoretical…
We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…
The nitrogen-vacancy (NV) center spin represents an appealing candidate for quantum information processing. Besides the widely used microwave control, its coherent manipulation may also be achieved using laser as mediated by the excited…
Spins of negatively charged nitrogen-vacancy (NV$^-$) defects in diamond are among the most promising candidates for solid-state qubits. The fabrication of quantum devices containing these spin-carrying defects requires position-controlled…
Coherent coupling between single quantum objects is at the heart of modern quantum physics. When coupling is strong enough to prevail over decoherence, it can be used for the engineering of correlated quantum states. Especially for…
Understanding and mitigating decoherence is a key challenge for quantum science and technology. The main source of decoherence for solid-state spin systems is the uncontrolled spin bath environment. Here, we demonstrate quantum control of a…
Monolithic integration, which refers to the incorporation of all device functionalities within a single material, shows significant potential for creating scalable solid-state quantum devices. This study demonstrated the coherent control of…
We present a theoretical investigation on the enhancement of the spin coherence with periodic, concatenated, or Uhrig dynamical decoupling $N$-pulse sequences in a $^{87}$Rb spin-1 Bose condensate, where the intrinsic dynamical instability…
Optically active solid-state spin defects have the potential to become a versatile resource for quantum information processing applications. Nitrogen-vacancy defect centers (NV) in diamond act as quantum memories and can be interfaced by…
Spin qubit coherence is a fundamental resource for the realization of quantum technologies. For solid-state platforms, spin decoherence is dominated by the magneto-active environment in the lattice, limiting their applicability. While…
In quantum information processing, it is vital to protect the coherence of qubits in noisy environments. Dynamical decoupling (DD), which applies a sequence of flips on qubits and averages the qubit-environment coupling to zero, is a…
We study the applicability of the time optimal bang-bang control designed for spin-1/2 [U. Boscain and P. Mason, J. Math. Phys. {\bf 47}, 062101 (2006)] to the rotation of the electron spin of a nitrogen-vacancy (NV) center in diamond. The…
In recent years, solid-state spin systems have emerged as promising candidates for quantum information processing (QIP). Prominent examples are the Nitrogen-Vacancy (NV) center in diamond, phosphorous dopants in silicon (Si:P), rare-earth…
Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics.…
Solid-state spin defects, especially nuclear spins with potentially achievable long coherence times, are compelling candidates for quantum memories and sensors. However, their current performances are still limited by the decoherence due to…