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Highly accurate experimental structure factors of silicon are available in the literature, and these provide the ideal test for any \emph{ab initio} method for the construction of the all-electron charge density. In a recent paper [J. R.…

Materials Science · Physics 2015-05-14 J. R. Trail , D. M. Bird

We examine the challenge of performing accurate electronic structure calculations at high pressures by comparing the results of all-electron full potential linearized augmented-plane-wave calculations with those of the projector augmented…

Computational Physics · Physics 2018-01-11 Kanchan Sarkar , Mehmet Topsakal , N. A. W. Holzwarth , Renata M. Wentzcovitch

We formulate a Hartree-Fock-LAPW method for electronic band structure calculations. The method is based on the Hartree-Fock-Roothaan approach for solids with extended electron states and closed core shells where the basis functions of…

Materials Science · Physics 2016-08-31 A. V. Nikolaev , P. N. Dyachkov

Electron-phonon interactions are of great importance to a variety of physical phenomena, and their accurate description is an important goal for first-principles calculations. Isolated examples of materials and molecular systems have…

Materials Science · Physics 2024-03-14 Antonios M. Alvertis , David B. Williams-Young , Fabien Bruneval , Jeffrey B. Neaton

The combination of two-dimensional materials into heterostructures offers new opportunities for the design of optoelectronic devices with tunable properties. However, computing electronic and optical properties of such systems using…

Materials Science · Physics 2025-07-25 Maximilian Schebek , Ignacio Gonzalez Oliva , Claudia Draxl

Positron Annihilation Lifetime Spectroscopy (PALS) is a powerful technique for detecting microstructural defects in various material classes. In a commonly used 180{\deg} detector configuration equipped with plastic scintillators,…

Instrumentation and Detectors · Physics 2025-05-06 Dominik Boras , Danny Petschke , Torsten Staab

Positron Annihilation Lifetime Spectroscopy (PALS) is a non-destructive radiological technique widely used in material science studies. PALS typically relies on an analog coincidence measurement setup and allows the estimate of the positron…

Instrumentation and Detectors · Physics 2019-08-14 Ming Fang , Nathan Bartholomew , Angela Di Fulvio

In Kohn-Sham electronic structure computations, wave functions have singularities at nuclear positions. Because of these singularities, plane-wave expansions give a poor approximation of the eigenfunctions. In conjunction with the use of…

Numerical Analysis · Mathematics 2023-01-02 Xavier Blanc , Eric Cancès , Mi-Song Dupuy

We present a set of efficient techniques in first-principles electronic-structure calculations utilizing the real-space finite-difference method. These techniques greatly reduce the overhead for performing integrals that involve…

Materials Science · Physics 2009-11-10 Tomoya Ono , Kikuji Hirose

We used our previously implemented GW approximation (GWA) based on the all-electron full-potential projector augmented wave (PAW) method to study the optical properties of small, medium and large-band-gap semiconductors: Si, GaAs, AlAs,…

Materials Science · Physics 2016-08-31 B. Arnaud , M. Alouani

Positronium atoms (Ps) are widely used as a probe to characterize voids or vacancies in non-metallic materials, where Ps annihilation lifetime is strongly modified by pickoff, depending on the size of the trapping cavity and on the…

Strongly Correlated Electrons · Physics 2022-05-25 Giacomo Marlotti Tanzi , Giovanni Consolati , Fabrizio Castelli

The paper presents the application of the multi-layer perceptron regressor model for predicting the parameters of positron annihilation lifetime spectra using the example of alkanes in the solid phase. A good agreement of calculation…

Atomic Physics · Physics 2023-09-20 M. Pietrow , A. Miaskowski

Electron-positron interactions have been utilized in various fields of science. Here we develop time-dependent multi-component density functional theory to study the coupled electron-positron dynamics from first principles. We prove that…

Chemical Physics · Physics 2018-10-03 Yasumitsu Suzuki , Satoshi Hagiwara , Kazuyuki Watanabe

We analyze the electronic structure of group III-V semiconductors obtained within full potential linearized augmented plane wave (FP-LAPW) method and arrive at a realistic and minimal tight-binding model, parameterized to provide an…

Materials Science · Physics 2009-11-11 Ranjani Viswanatha , Sameer Sapra , Tanusri Saha-Dasgupta , D. D. Sarma

Ab initio electronic structure calculations of two-dimensional layered structures are typically performed using codes that were developed for three-dimensional structures, which are periodic in all three directions. The introduction of a…

Strongly Correlated Electrons · Physics 2016-06-22 Paolo E. Trevisanutto , Giovanni Vignale

The methods which are actively used for electronic structure calculations of low-lying states of heavy- and superheavy-element compounds are briefly described. The advantages and disadvantages of calculations with the Dirac-Coulomb-Breit…

Chemical Physics · Physics 2009-11-07 A. V. Titov , N. S. Mosyagin , T. A. Isaev , A. N. Petrov

The electronic structure and properties of PuO$_{2}$ and Pu$_{2}$O$_{3}$ have been studied from first principles by the all-electron projector-augmented-wave (PAW) method. The local density approximation (LDA)+$U$ and the generalized…

Materials Science · Physics 2007-12-24 Bo Sun , Ping Zhang , Xian-Geng Zhao

We present an approach to calculate the electronic structure for a range of materials using the quasiparticle self-consistent GW method with vertex corrections included in the screened Coulomb interaction W. This is achieved by solving the…

Materials Science · Physics 2023-10-10 Brian Cunningham , Myrta Gruening , Dimitar Pashov , Mark van Schilfgaarde

We discuss our new implementation of the Real-space Electronic Structure method for studying the atomic and electronic structure of infinite periodic as well as finite systems, based on density functional theory. This improved version which…

Materials Science · Physics 2009-10-31 U. V. Waghmare , Hanchul Kim , I. J. Park , Normand Modine , P. Maragakis , Efthimios Kaxiras