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Plasmons in ultranarrow metal gaps are highly sensitive to the electron density profile at the metal surfaces. Using a fully quantum mechanical approach, we study the effects of electron spill-out on gap plasmons and reflectance from…

Mesoscale and Nanoscale Physics · Physics 2018-10-12 Enok J. H Skjølstrup , Thomas Søndergaard , Thomas G. Pedersen

Herein, we investigate the optical properties of quantum plasmonic metasurfaces composed of metallic nano-objects with subnanometer gaps according to the time-dependent density functional theory, a fully quantum mechanical approach. When…

Optics · Physics 2019-06-17 Takashi Takeuchi , Masashi Noda , Kazuhiro Yabana

Surface adsorption, which is often coupled with surface dissolution, is generally unpredictable on alloys due to the complicated alloying and dissolution effects. Herein, we introduce the electronic gradient and cohesive properties of…

Materials Science · Physics 2021-08-26 Bo Li , Wang Gao , Qing Jiang

A quantum mechanical approach and local response theory are applied to study plasmons propagating in nanometer-thin gold slabs sandwiched between different dielectrics. The metal slab supports two different kinds of modes, classified as…

We develop a consistent quantum description of surface plasmons interacting with quantum emitters and external electromagnetic field. Within the framework of macroscopic electrodynamics in dispersive and absorptive medium, we derive, in the…

Mesoscale and Nanoscale Physics · Physics 2021-01-21 Tigran V. Shahbazyan

Metal-dielectric interfaces of various geometries are fundamental photonic material platforms for surface plasmons. Surface plasmon polaritons and localized surface plasmons are two surface plasmon modes that are excited on planar and…

We present a theoretical study of the dispersion relation of surface plasmon resonances of mesoscopic metal-dielectric-metal microspheres. By analyzing the solutions to Maxwell's equations, we obtain a simple geometric condition for which…

Optics · Physics 2009-11-11 Keisuke Hasegawa , Charles A. Rohde , Miriam Deutsch

We investigate theoretically the effects of interaction between an optical dipole (semiconductor quantum dot or molecule) and metal nanoparticles. The calculated absorption spectra of hybrid structures demonstrate strong effects of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Jie-Yun Yan , Wei Zhang , Suqing Duan , Xian-Geng Zhao , Alexander O. Govorov

Plasmon resonance, with strong coupling of light to electrons at a metal-dielectric interface, allows light confinement and control at subwavelength scale. It's fundamentally limited by the inherent mobility of the electrons, leading to the…

Optics · Physics 2019-02-20 Evgenii E. Narimanov

We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with conventional absorption peak at frequency close to intersubband…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Dai , M. E. Raikh , T. V. Shahbazyan

We investigate the scattering and absorption properties of anisotropic metal-dielectric core-shell nanoparticles. It is revealed that the radially anisotropic dielectric layer can accelerate the evanescent decay of the localized resonant…

Optics · Physics 2016-08-24 Wei Liu , Bing Lei , Andrey E. Miroshnichenko

Silver is considered to be the king among plasmonic materials because it features low inelastic absorption in the visible and infrared (vis-IR) spectral regions compared to other metals. In contrast, copper is commonly regarded as being too…

We study a highly controllable perfect plasmonic absorber -- a thin metamaterial layer which possess balanced electric and magnetic responses in some frequency range. We show that this regime is compatible with both metal-backed variant of…

Optics · Physics 2016-01-25 Mikhail Omelyanovich , Younes Ra'di , Constantin Simovski

Plasmons in nanostructured metals are widely utilized to trigger strong light--matter interactions with quantum light sources. While the nonclassical behavior of such quantum emitters (QEs) is well-understood in this context, the role of…

The possibility for controlling the probe-field optical gain and absorption switching and photon conversion by a surface-plasmon-polariton near field is explored for a quantum dot above the surface of a metal. In contrast to the linear…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

The effect of nonlocality on the optical response of metals lies at the forefront of research in nanoscale physics and, in particular, quantum plasmonics. In alkali metals, nonlocality manifests predominantly as electron density spill-out…

Mesoscale and Nanoscale Physics · Physics 2025-03-06 Ida Juliane Bundgaard , Christian Nicolaisen Hansen , P. Elli Stamatopoulou , Christos Tserkezis

Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

We explored a metal-insulator-metasurface structure exhibiting dual-band absorption in the visible and infrared regions with almost perfect absorbance. We demonstrated that the existence of the dual peak absorbance is due to the excitation…

The resonant scattering of surface plasmon-polariton waves by embedded semiconductor quantum dots above the dielectric/metal interface is explored in the strong-coupling regime. In contrast to non-resonant scattering by a localized…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

Nitrogen vacancy (NV) centers in diamond have emerged as a leading quantum sensor platform, combining exceptional sensitivity with nanoscale spatial resolution by optically detected magnetic resonance (ODMR). Because fluorescence-based ODMR…

Quantum Physics · Physics 2020-11-24 Laura Kim , Hyeongrak Choi , Matthew Trusheim , Dirk Englund
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