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This study focuses on comparing the individual polymer chain dynamics in an entangled polymeric liquid under different shear and extension rates. Polymer chains under various shear rates and extension rates were simulated using a…

Chemical Physics · Physics 2021-01-15 Behrouz Behdani , Tong Mou , Cody Spratt , Slava Butcovich , Ryan Gettler , Joontaek Park

Physically confining polymers into nanoscale pores induces significant changes in their dynamics. Although different results on the effect of confinement on the dynamics of polymers have been reported, changes in the segmental mobility of…

Soft Condensed Matter · Physics 2022-05-27 R. Bharath Venkatesh , Daeyeon Lee

The influence of shape fluctuations on deformable thermosensitive microgels in aqueous solution is investigated by dynamic light scattering (DLS) and depolarized dynamic light scattering (DDLS). The systems under study consist of a solid…

Soft Condensed Matter · Physics 2009-02-20 S. Bolisetty , M. Hoffmann , S. Lekkala , Th. Hellweg , M. Ballauff , L. Harnau

The miscibility in several polymer blend mixtures (polymethylmethacrylate/polystyrene, (1,4-cis) polyisoprene/polystyrene, and polymethylmethacrylate/polyoxyethylene) has been investigated using Molecular Dynamics simulations for atomistic…

Chemical Physics · Physics 2009-05-29 Amirhossein Ahmadi , Juan J. Freire

The advances in new technologies have prompted the need for functional systems smaller than the gyration radius of polymer chains. Thus, understanding how nanoconfinement affects polymer properties has been the focus of a lot of research…

Soft Condensed Matter · Physics 2010-07-27 Fabrice Cousin , Jérémie Gummel , Daniel Clemens , Isabelle Grillo , François Boué

Droplet coalescence is ubiquitous in nature and the same time key to various technologies, such as inkjet printing. Here, we report on the coalescence of polymer droplets with different chain lengths coalescing on substrates of different…

Soft Condensed Matter · Physics 2023-09-21 Soheil Arbabi , Panagiotis E. Theodorakis

Active polymers possess numerous unique properties that are quite different from those observed in the system of small active molecule due to the intricate interplay between their activity and topological constraints. This study focuses on…

Soft Condensed Matter · Physics 2024-07-09 Jing Li , Bokai Zhang , Zhi-Yong Wang

In this paper, we have studied the effect of short branches on the thermal conductivity of a polyethylene (PE) chain. With a reverse non-equilibrium molecular dynamics method applied, thermal conductivities of the pristine PE chain and the…

Mesoscale and Nanoscale Physics · Physics 2017-03-31 Danchen Luo , Congliang Huang , Zun Huang

Molecular dynamics simulations are used to study structure formation in simple model polymer chains that are subject to excluded volume and torsional interactions. The changing conformations exhibited by chains of different lengths under…

Soft Condensed Matter · Physics 2009-11-07 D. C. Rapaport

Simulations are used to examine the microscopic origins of strain hardening in polymer glasses. While stress-strain curves for a wide range of temperature can be fit to the functional form predicted by entropic network models, many other…

Soft Condensed Matter · Physics 2009-11-13 Robert S. Hoy , Mark O. Robbins

Using molecular dynamics simulations we examine the dynamics of a family of model polymers with varying chain length and torsional potential barriers. We focus on features of the dynamics of polymers that are seen experimentally but absent…

Soft Condensed Matter · Physics 2019-06-11 Daniel Fragiadakis , C. Michael Roland

Molecular Dynamics simulations of a coarse-grained bead-spring model of flexible macromolecules tethered with one end to the surface of a cylindrical pore are presented. Chain length $N$ and grafting density $\sigma$ are varied over a wide…

Soft Condensed Matter · Physics 2007-05-23 Dimitar I. Dimitrov , Andrey Milchev , Kurt Binder , Dieter W. Heermann

Slow dynamics in a fluid are studied in one of the most basic systems possible: polydisperse hard spheres. Monodisperse hard spheres cannot be studied as the slow down in dynamics as the density is increased is preempted by crystallisation.…

Soft Condensed Matter · Physics 2009-10-31 Richard P. Sear

Ring polymers are an intriguing class of polymers with unique physical properties, and understanding their behavior is important for developing accurate theoretical models. In this study, we investigate the effect of chain stiffness and…

Soft Condensed Matter · Physics 2023-08-24 Shota Goto , Kang Kim , Nobuyuki Matubayasi

Soft glassy materials often consist of deformable objects. Here, we use a two-dimensional assembly of semi-flexible ring polymers as a model system to investigate how polydispersity in particle stiffness or size influences the onset of…

Soft Condensed Matter · Physics 2025-09-25 Rahul Nayak , Pinaki Chaudhuri , Satyavani Vemparala

Mechanical stretching behavior of poly(styrene-b-ethylene-co-butylene-b-styrene) (SEBS) triblock copolymer (87 wt% polyethylene-co-butylene (PEB) block, 13 wt% polystyrene (PS) block) was investigated by three different stretching and in…

At ultralow temperatures, polymers exhibit quantum behavior, which is calculated here for the second and fourth moments of the end-to-end distribution in the large-stiffness regime. The result should be measurable for polymers in wide…

Soft Condensed Matter · Physics 2009-10-20 H. Kleinert

We present thermophoretic measurements in aqueous suspensions of three different polystyrene (PS) particles of varying negative charge, size and surface coating. Our measurement technique is based on the observation of the colloidal…

Soft Condensed Matter · Physics 2017-10-11 Jerome Burelbach , Mykolas Zupkauskas , Robin Lamboll , Yang Lan , Erika Eiser

At ultralow temperatures, polymers exhibit quantum behavior, which is calculated here for the moments <R^2> and <R^4> of the end-to-end distribution in the large-stiffness regime. The result should be measurable for polymers in wide optical…

Soft Condensed Matter · Physics 2009-11-13 H. Kleinert

We present an extensive molecular dynamics (MD) simulation study of poly(ethylene oxide) (PEO) based densely cross-linked polymers, focussing on structural properties as well as the systems dynamics in the presence of lithium salt.…

Soft Condensed Matter · Physics 2022-11-15 Mirko Fischer , Andreas Heuer , Diddo Diddens