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We report on the observation of terahertz radiation in a non-centrosymmetric insulating oxide, paratellurite ($\alpha$-TeO$_2$) by irradiation of a femtosecond laser pulse at room temperature. In the power spectrum of the terahertz…

Materials Science · Physics 2015-06-22 M. Sotome , N. Kida , R. Takeda , H. Okamoto

Following excitation by a strong ultra-short laser pulse, molecules develop coordinated rotational motion, exhibiting transient alignment along the direction of the laser electric field, followed by periodic full and fractional revivals…

Quantum Physics · Physics 2007-05-23 Sharly Fleischer , Ilya. Sh. Averbukh , Yehiam Prior

We present a combined analytical and numerical study for coherent terahertz control of a single molecular polariton, formed by strongly coupling two rotational states of a molecule with a single-mode cavity. Compared to the bare molecules…

Quantum Physics · Physics 2023-02-08 Li-Bao Fan , Chuan-Cun Shu , Daoyi Dong , Jun He , Niels E. Henriksen , Franco Nori

Spontaneous formation of spatial structures (patterns) occurs in various contexts, ranging from sand dunes and rogue wave formation, to traffic jams. These last decades, very practical reasons also led to studies of pattern formation in…

On the basis of the recently proposed {\it Thermal Wave Model (TWM) for particle beams}, we give a description of the longitudinal charge particle dynamics in circular accelerating machines by taking into account both radiation damping and…

acc-phys · Physics 2015-06-24 R. Fedele , G. Miele , L. Palumbo

For facile manipulation of polarization states of light for applications in communications, imaging, and information processing, an efficient mechanism is desired for rotating light polarization with a minimum interaction length. Here, we…

With ever increasing availability of terahertz fields, it is important to find suitable detection techniques without compromising the measured dynamic range. Electro-optic terahertz sampling techniques, which are commonly used to detect…

Optics · Physics 2020-08-26 Gregory Bell , Michael Hilke

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh

Ring polymer molecular dynamics (RPMD) has proven to be an accurate approach for calculating thermal rate coefficients of various chemical reactions. For wider application of this methodology, efficient ways to generate the underlying…

Chemical Physics · Physics 2020-01-08 Ivan S. Novikov , Alexander V. Shapeev , Yury V. Suleimanov

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

Terahertz spintronics offers the prospect of devices which are both faster and more energy-efficient. A promising route to achieve this goal is to exploit current-induced spin-orbit torques. However, the high-frequency properties of these…

Mesoscale and Nanoscale Physics · Physics 2020-12-21 Filipe S. M. Guimarães , Juba Bouaziz , Manuel dos Santos Dias , Samir Lounis

We consider the classical picture of three dimensional motion of charged particles in pulsar magnetosphere. We adopt a perturbative method to solve the equation of motion, and find the trajectory of particles as they move along the rotating…

Astrophysics · Physics 2009-11-13 R. M. C. Thomas , R. T. Gangadhara

Spintronic terahertz emitters (STEs) are powerful sources of ultra-broadband single-cycle terahertz (THz) field transients. They work with any pump wavelength, and their polarity and polarization direction are easily adjustable. However, at…

We demonstrate the application of the efficient semi-inverse asymptotic method to resonant interaction of the nonlinear normal modes belonging to different branches of the CNT vibration spectrum. Under condition of the 1:1 resonance of the…

Mesoscale and Nanoscale Physics · Physics 2017-04-04 V. V. Smirnov , L. I. Manevitch

We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…

Atomic Physics · Physics 2015-05-14 E. Gershnabel , I. Sh. Averbukh

We predict a complete TM-TE transformation of the polarization of terahertz electromagnetic waves reflected from a strongly anisotropic boundary of a layered superconductor. We consider the case when the wave is incident on the…

Superconductivity · Physics 2013-03-19 Yu. O. Averkov , V. M. Yakovenko , V. A. Yampol'skii , Franco Nori

We examine the impact of the combination of a static electric field and a non resonant linearly polarized laser field on an asymmetric top molecule. Within the rigid rotor approximation, we analyze the symmetries of the Hamiltonian for all…

Chemical Physics · Physics 2015-05-28 J. J. Omiste , R. González-Férez , P. Schmelcher

A pair of circularly polarized laser pulses of opposite helicities are shown to control the route of spin reorientation phase transition in rare-earth antiferromagnetic orthoferrite (Sm$_{0.55}$Tb$_{0.45}$)FeO$_3$. The route can be…

Strongly Correlated Electrons · Physics 2024-04-30 N. E. Khokhlov , A. E. Dolgikh , B. A. Ivanov , A. V. Kimel

A mixed quantum-classical approach is introduced which allows the dynamical response of molecules driven far from equilibrium to be modeled. This method is applied to the interaction of molecules with intense, short-duration laser pulses.…

Atomic Physics · Physics 2012-05-21 Daniel Dundas

We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…

Chemical Physics · Physics 2016-05-11 A. Korobenko , V. Milner