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We build up a consistent theory of quantum electrodynamics in the presence of macroscopic polarizable media. We use the Huttner-Barnett model of a dispersive and absorbing dielectric medium and formulate the theory in terms of interacting…

Quantum Physics · Physics 2012-08-17 Claudia Eberlein , Robert Zietal

A new theoretical approach for the calculation of optical properties of complex solutions is proposed. It is based on a dielectric matrix with included small metallic inclusions (less than 3 nm) of spherical shape. We take into account the…

Soft Condensed Matter · Physics 2015-05-13 Vitaliy N. Pustovit , Tigran V. Shahbazyan , Leonid G. Grechko

Time-dependent density functional theory (TDDFT) is rapidly emerging as a premier method for solving dynamical many-body problems in physics and chemistry. The mathematical foundations of TDDFT are established through the formal existence…

Quantum Physics · Physics 2014-08-22 J. D. Whitfield , M. -H. Yung , D. G. Tempel , S. Boixo , A. Aspuru-Guzik

Time-dependent density functional theory (TDDFT) is presently enjoying enormous popularity in quantum chemistry, as a useful tool for extracting electronic excited state energies. This article discusses how TDDFT is much broader in scope,…

Other Condensed Matter · Physics 2007-05-23 Kieron Burke , Jan Werschnik , E. K. U. Gross

Time-dependent density-functional theory (TDDFT) is deemed to be a formally rigorous way of dealing with the time-evolution of a many-electron system at the level of electron densities rather than the underlying wavefunctions, which in turn…

Chemical Physics · Physics 2024-11-26 Jochen Schirmer

In pursuit of a colloidal analogue to quantum density functional theory (DFT) predictions of atomic crystal structures, we report a new, classical DFT that predicts the relative thermodynamic stability of colloidal crystals of hard, convex…

Soft Condensed Matter · Physics 2026-01-15 Kristi Pepa , Isaac R. Spivack , Trevor F. G. Teague , Ryn Y. Oliphant , Domagoj Fijan , Sharon C. Glotzer

We investigate the collective plasmonic modes of metal nano-particles in periodic two-dimensional (2D) arrays within a point-dipole description. As an open system, the full-dynamic dispersion relations of the 2D arrays are obtained through…

Optics · Physics 2016-07-29 Yu-Rong Zhen , Kin Hung Fung , C. T. Chan

We consider electrodynamics on a noncommutative spacetime using the enveloping algebra approach and perform a non-relativistic expansion of the effective action. We obtain the Hamiltonian for quantum mechanics formulated on a canonical…

High Energy Physics - Theory · Physics 2009-11-11 Xavier Calmet , Michele Selvaggi

The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides…

Optics · Physics 2022-07-22 Ying Li , Christos Argyropoulos

The one dimensional (1D) driven quantum coupled pseudoforce system governing the dynamics of collective Langmuir electron oscillations is used in order to investigate the effects of variety of space charge distributions on plasmon…

Plasma Physics · Physics 2019-03-27 M. Akbari-Moghanjoughi

Quantum plasmonics explores how light interacts with collective charge oscillations at metal-dielectric interfaces, enabling strong confinement and enhanced quantum effects at the nanoscale. While traditional quantum optics focuses on…

Quantum Physics · Physics 2025-04-03 Mingyuan Hong

Two-dimensional mixtures of dipolar colloidal particles with different dipole moments exhibit extremely rich self-assembly behaviour and are relevant to a wide range of experimental systems, including charged and super-paramagnetic colloids…

Soft Condensed Matter · Physics 2019-04-16 W. R. C. Somerville , J. L. Stokes , A. M. Adawi , T. S. Horozov , A. J. Archer , D. M. A. Buzza

Properties and applications of a plasmonic cross-shaped nano-antenna is presented and compared to those of array of holes. A simple analytical model based on the superposition of waves are proposed and compared to the numerical results. A…

Optics · Physics 2021-02-02 Amir Djalalian-Assl

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

The adiabatic approximation in time-dependent density functional theory (TDDFT) is known to give an incorrect pole structure in the quadratic response function, leading to unphysical divergences in excited state-to-state transition…

Chemical Physics · Physics 2023-05-01 Davood Dar , Saswata Roy , Neepa T. Maitra

Using the Runge-Gross theorem that establishes the foundation of Time-dependent Density Functional Theory (TDDFT) we prove that for a given electronic Hamiltonian, choice of initial state, and choice of fragmentation, there is a unique…

Chemical Physics · Physics 2015-06-15 Martin A. Mosquera , Daniel Jensen , Adam Wasserman

We develop a microscopic quantum theory of surface plasmon polaritons valid for arbitrary metal-dielectric geometries. Our framework is based on the Power-Zienau-Woolley representation of quantum electrodynamics, which provides an optimal…

The quantization of plasmons has been analyzed mostly under the assumption of an infinite-sized bulk medium interacting with the electromagnetic field. We reformulate it for finite-size media, such as metallic or dielectric nano-structures,…

Quantum Physics · Physics 2019-10-23 V. Dorier , J. Lampart , S. Guérin , H. R. Jauslin

The Feynman quantum-classical isomorphism between classical statistical mechanics in 3+1 dimensions and quantum statistical mechanics in 3 dimensions is used to connect classical polymer self-consistent field theory with quantum…

Quantum Physics · Physics 2021-11-30 Russell B. Thompson

Electronic response properties of high-energy density (HED) systems influence planetary structure, drive evolution of fusion targets, and underpin diagnostics in laboratory astrophysics. Real-time time-dependent density functional theory…

Plasma Physics · Physics 2025-11-19 Alina Kononov , Minh Nguyen , Andrew D. Baczewski