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We report on sytematic measurements of the low frequency conductivity in aequous supensions of highly charged colloidal spheres. System preparation in a closed tubing system results in precisely controlled number densities between 1E16/m3…

Soft Condensed Matter · Physics 2009-10-31 Dirk Hessinger , Martin Evers , Thomas Palberg

Charge disproportionation (CD) and spin differentiation in Na$_{1/2}$CoO$_2$ are studied using the correlated band theory approach. The simultaneous CD and gap opening seen previously is followed through a first order charge…

Strongly Correlated Electrons · Physics 2007-05-23 K. -W. Lee , J. Kunes , P. Novak , W. E. Pickett

We investigate electronic excitations in La2-x(Br,Sr)xCuO4 using resonant inelastic x-ray scattering (RIXS) at the oxygen K edge. RIXS spectra of the hole-doped cuprates show clear momentum dependence below 1 eV. The spectral weight…

Strongly Correlated Electrons · Physics 2017-09-26 K. Ishii , T. Tohyama , S. Asano , K. Sato , M. Fujita , S. Wakimoto , K. Tustsui , S. Sota , J. Miyawaki , H. Niwa , Y. Harada , J. Pelliciari , Y. Huang , T. Schmitt , Y. Yamamoto , J. Mizuki

We have developed and applied a mobility edge model that takes into account drift and diffusion currents to characterize the space charge limited current in organic semiconductors. The numerical solution of the drift-diffusion equation…

Materials Science · Physics 2015-05-30 Javier Dacuña , Alberto Salleo

A one-dimensional many-body model is established to mimic the charge distribution and dynamics in nonfullerene organic solar cells. Two essential issues are taken into account in the model: The alternating donor and acceptor structure and…

Materials Science · Physics 2018-12-05 Yao Yao

Using a combination of X-ray absorption spectroscopy experiments with first principle calculations, we demonstrate that insulating KCuO_2 contains Cu in an unusually-high formal-3+ valence state, the ligand-to-metal (O to Cu) charge…

Strongly Correlated Electrons · Physics 2015-11-25 D. Choudhury , P. Rivero , D. Meyers , X. Liu , Y. Cao , S. Middey , M. J. Whitaker , S. Barraza-Lopez , J. W. Freeland , M. Greenblatt , J. Chakhalian

We investigated how different materials affect the orbital-charge conversion in heterostructures with the naturally oxidized cooper capping layer. When we added a thin layer of $CuOx(3nm)$ onto yttrium iron garnet $(YIG)/W$ stacks, we…

Mesoscale and Nanoscale Physics · Physics 2024-01-29 E. Santos , J. E. Abrão , A. S. Vieira , J. B. S. Mendes , R. L. Rodríguez-Suárez , A. Azevedo

It is shown that the properties of the superconductivity observed in Sr$_2$RuO$_4$ can be accounted for by properly taking into account the internal degrees of freedom of the system. The electrons are strongly correlated in the RuO$_2$…

Superconductivity · Physics 2007-05-23 Ralph Werner

We discuss density functional theory calculations of hybrid inorganic/organic systems (HIOS) that explicitly include the global effects of doping (i.e. position of the Fermi level) and the formation of a space-charge layer. For the example…

The electronic structure of CoO is studied by resonant inelastic soft X-ray scattering spectroscopy using photon energies across the Co 2p absorption edges. The different spectral contributions from the energy-loss structures are identified…

Materials Science · Physics 2012-01-04 M. Magnuson , S. M. Butorin , J. -H. Guo , J. Nordgren

Rubidium superoxide, RbO_2, is a rare example of a solid with partially-filled electronic p states, which allows to study the interplay of spin and orbital order and other effects of strong electronic correlations in a material that is…

Strongly Correlated Electrons · Physics 2013-05-30 Roman Kovacik , Philipp Werner , Krzysztof Dymkowski , Claude Ederer

We have analyzed the experimental evidence of charge and orbital ordering in La0.5Sr1.5MnO4 using first principles band structure calculations. Our results suggest the presence of two types of Mn sites in the system. One of the Mn sites…

Strongly Correlated Electrons · Physics 2009-11-07 Priya Mahadevan , K. Terakura , D. D. Sarma

Quasi-particle spectra of the layer perovskite Sr$_2$RuO$_4$ are calculated within Dynamical Mean Field Theory for increasing values of the on-site Coulomb energy $U$. At small $U$ the planar geometry splits the $t_{2g}$ bands near $E_F$…

Strongly Correlated Electrons · Physics 2015-06-24 A. Liebsch

In the multiband systems, Hund's coupling ($J$) plays a significant role in the spin and charge excitations. We study the dependence of electronic anisotropy on $J$ in terms of Drude-weight along different directions as well as the orbital…

Strongly Correlated Electrons · Physics 2022-08-17 Garima Goyal , Dheeraj Kumar Singh

Metamagnetism in layered ruthenates has been interpreted as a novel kind of quantum critical behavior. In an external magnetic field, Ca$_{2-x}$Sr$_x$RuO$_4$ undergoes a metamagnetic transition accompanied by a pronounced magnetostriction…

Strongly Correlated Electrons · Physics 2008-08-17 Rafael Roldan , Andreas Ruegg , Manfred Sigrist

In frames of a rather conventional cluster approach, which combines the crystal field and the ligand field models we have considered different charge transfer (CT) states and O 2p-Mn 3d CT transitions in MnO$_{6}^{9-}$ octahedra. The…

Strongly Correlated Electrons · Physics 2009-11-07 A. S. Moskvin

In this study, the structural, electronic and optical properties of Pb doped rutile SnO$_2$ were investigated using the range separated hybrid exchange-correlation functional method. In the calculations, LDA functional was used instead of…

Materials Science · Physics 2021-07-28 Veysel Çelik

We investigate the possible superconducting instabilities of strongly correlated electron materials using a generalization of linear response theory to external pairing fields depending on frequency. We compute a pairing susceptibility…

Superconductivity · Physics 2024-09-18 Olivier Gingras , Antoine Georges , Olivier Parcollet

Understanding the evolution of the physicochemical bulk properties during the Li deintercalation (charging) process is critical for optimizing battery cathode materials. In this study, we combine X-ray photoelectron spectroscopy (XPS),…

Motivated by recent experimental progress in transition metal oxides with the K$_2$NiF$_4$ structure, we investigate the magnetic and orbital ordering in $\alpha$-Sr$_2$CrO$_4$. Using first principles calculations, first we derive a…

Strongly Correlated Electrons · Physics 2021-01-20 Bradraj Pandey , Yang Zhang , Nitin Kaushal , Rahul Soni , Ling-Fang Lin , Wen-Jun Hu , Gonzalo Alvarez , Elbio Dagotto