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We study the chemical nature of the bonding of an oxide layer to the parent metal. In order to disentangle chemical effects from strain/misfit, Ti(10$\bar{1}$0)/TiO$_{2}$(100) interface has been chosen. We use the density functional…

Materials Science · Physics 2012-12-10 Linggang Zhu , Graeme J. Ackland

We present a computational study of the adhesive and structural properties of the Al/Al2O3 interfaces as building blocks of the Metal-Insulator-Metal (MIM) tunnel devices, where electron transport is accomplished via tunnelling mechanism…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 M. Koberidze , M. J. Puska , R. M. Nieminen

A theory of combined interference and interaction effects on the diffusive transport properties of 3D topological insulator surface states is developed. We focus on a slab geometry (characteristic for most experiments) and show that…

Mesoscale and Nanoscale Physics · Physics 2013-08-06 E. J. König , P. M. Ostrovsky , I. V. Protopopov , I. V. Gornyi , I. S. Burmistrov , A. D. Mirlin

We derive a formula, useful for first-principles calculations, which relates the free energy of an oxide/metal interface to the free energies of surfaces and the work of separation of the interface. We distinguish the latter {\it…

Materials Science · Physics 2007-05-23 Iskander G. Batirev , Ali Alavi , Michael W. Finnis

Thermal Interface Materials (TIMs) are widely used in electronic packaging. Increasing power density and limited assembly space pose high demands on thermal management. Large cooling surfaces need to be covered efficiently. When joining the…

Machine Learning · Computer Science 2024-10-28 Simon Baeuerle , Marius Gebhardt , Jonas Barth , Andreas Steimer , Ralf Mikut

Appropriate candidates of the metallic sheet used for the electrodes of diamond semiconductor are investigated using computational approaches based on density functional theory (DFT). For twenty kinds of metallic elements $x$, we modeled a…

Materials Science · Physics 2017-09-12 Tom Ichibha , Kenta Hongo , Isaac Motochi , Nicholas W. Makau , George O. Amolo , Ryo Maezono

In this work, we perform a systematic computer simulation study of ice premelting, and explore the thickness and structure of quasi-liquid layers formed at the interface of ice with substrates of different hydrophilicity. Our study shows…

Soft Condensed Matter · Physics 2024-10-30 Łukasz Baran , Pablo Llombart , Luis G. MacDowell

We study the dynamics of the contact between a pair of surfaces (with properties designed to mimic ruthenium) via molecular dynamics simulations. In particular, we study the contact between a ruthenium surface with a single nanoasperity and…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Alan Barros de Oliveira , Andrea Fortini , Sergey V. Buldyrev , David Srolovitz

Dissipation and adhesion are important in many areas of materials science, including friction and lubrication, cold spray deposition, and micro-electromechanical systems (MEMS). Another interesting problem is the adhesion of mineral grains…

Materials Science · Physics 2022-05-06 Baochi Doan , Patrick K. Schelling

The adhesion between a polymer melt and substrate is studied in the presence of chemically attached chains on the substrate surface. Extensive molecular dynamics simulations have been carried out to study the effect of temperature, tethered…

Materials Science · Physics 2016-08-31 Scott W. Sides , Gary S. Grest , Mark J. Stevens

The adhesion of two-dimensional (2D) materials to other surfaces is so far believed to be a solid-solid mechanical contact. Here, we conduct both atomistic simulations and theoretical modeling to show that there exists a reversible…

Materials Science · Physics 2015-12-08 Zhengrong Guo , Tienchong Chang , Xingming Guo , Huajian Gao

To date, density functional theory (DFT) is one of the most accurate and yet practical theory to gain insight about materials properties. Although successful, the computational cost is the main hurdle even today. A way out is combining DFT…

Materials Science · Physics 2019-04-19 Shweta Mehta , Sheena Agarwal , Kavita Joshi

Ab initio-calculated ideal strength and toughness describe the upper limits for mechanical properties attainable in real systems and can, therefore, be used in selection criteria for materials design. We employ density-functional ab initio…

Materials Science · Physics 2020-04-01 D. G. Sangiovanni , F. Tasnadi , L. J. S. Johnson , M. Oden , I. A. Abrikosov

Engineering wear models are generally empirical and lack connections to the physical processes of debris generation at the nanoscale to microscale. Here, we thus analyze wear particle formation for sliding interfaces in dry contact with…

Materials Science · Physics 2019-05-15 Tobias Brink , Jean-François Molinari

Heterogeneous interfaces are central to many energy-related applications in the nanoscale. From the first-principles electronic structure perspective, one of the outstanding problems is accurately and efficiently calculating how the…

Materials Science · Physics 2023-08-29 Zhen-Fei Liu

The results of DFT supercell calculations of oxygen behavior upon the UN (001) and (110) surfaces as well as at the tilt grain boundary are presented. Oxygen adsorption, migration, incorporation into the surface N vacancies on (001) and…

Materials Science · Physics 2015-06-12 D. Bocharov , D. Gryaznov , Yu. F. Zhukovskii , E. A. Kotomin

Density functional theory (DFT) underpins modern atomistic simulations of transition-metal surfaces. It can predict key properties linked to catalytic performance, such as adsorption energies and barrier heights, enabling new paradigms in…

Materials Science · Physics 2026-03-23 Benjamin X. Shi , Timothy C. Berkelbach

Using density-functional theory we investigate several properties of Al(111), Al(100), Al(110), and stepped Al(111) surfaces. We report results of formation energies of surfaces, steps, adatoms, and vacancies. For the adsorption and…

mtrl-th · Physics 2008-02-03 Roland Stumpf , Matthias Scheffler

Electron-ion interactions play a central role for the energy relaxation processes and ultra-fast structure dynamics in laser-heated matter. The accurate prediction of the electron-ion energy exchange in a transient excited two-temperature…

Other Condensed Matter · Physics 2024-01-17 Jia Zhang , Rui Qin , Wenjun Zhu , Jan Vorberger

Diamond and diamond-like carbon (DLC) coatings are widely employed for their exceptional mechanical, thermal and chemical properties, but their industrial application is often limited by weak adhesion to metallic substrates. In this work,…

Materials Science · Physics 2026-01-21 Elisa Damiani , Margherita Marsili , Maria Clelia Righi