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Related papers: The symmetry and light stuffing of Ho2Ti2O7, Er2Ti…

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We report synchrotron radiation diffraction and muon spin rotation (muSR) measurements on the frustrated pyrochlore magnet Tb2Ti2O7. The powder diffraction study of a crushed crystal fragment does not reveal any structural change down to 4…

Strongly Correlated Electrons · Physics 2014-12-22 P. Dalmas de Reotier , A. Yaouanc , A. Bertin , C. Marin , S. Vanishri , D. Sheptyakov , A. Cervellino , B. Roessli , C. Baines

We report a structural and thermodynamic study of the "stuffed spin ice" material Ho2TiO5 (i.e., Ho2(Ti1.33Ho0.67)O6.67), comparing samples synthesized through two different routes. Neutron powder diffraction and electron diffraction reveal…

Materials Science · Physics 2009-11-13 G. C. Lau , B. G. Ueland , M. L. Dahlberg , R. S. Freitas , Q. Huang , H. W. Zandbergen , P. Schiffer , R. J. Cava

The cubic symmetry of pyrochlore iridium oxides R2Ir2O7 (R = Nd, Eu, and Pr) has been investigated by high resolution X-ray diffraction experiments down to 4 K,in order to clarify the relationship between the metal-insulator transition…

Strongly Correlated Electrons · Physics 2014-12-12 Hiroshi Takatsu , Kunihiko Watanabe , Kazuki Goto , Hiroaki Kadowaki

The pyrochlore Ho2Ge2O7 is a new highly correlated spin ice material. Physical property measurements including x-ray diffraction, dc susceptibility and ac susceptibility, confirm that it shares the distinctive characteristics of other known…

The pyrochlore osmate Ho2Os2O7 is a candidate material for a fragile J=0 local singlet ground state, however little is known regarding the single-ion behavior of either the Os or Ho ions. To address this we present polarized neutron powder…

Strongly Correlated Electrons · Physics 2024-03-01 S. Calder , Z. Y. Zhao , M. H. Upton , J. -Q. Yan

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

By means of neutron scattering techniques we have investigated the frustrated pyrochlore magnet Ho_2Sn_2O_7, which was found to show a ferromagnetic spin-ice behavior below T \simeq 1.4 K by susceptibility measurements. High-resolution…

Disordered Systems and Neural Networks · Physics 2007-05-23 Hiroaki Kadowaki , Yoshinobu Ishii , Kazuyuki Matsuhira , Yukio Hinatsu

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

In this work we present a neutron Larmor diffraction study of the rare earth pyrochlores $R_2$Ti$_2$O$_7$, with $R$ = Tb, Dy, Ho. We measured the temperature dependence of the lattice parameter with precision $10^{-5}$, between 0.5 K and…

Strongly Correlated Electrons · Physics 2016-11-09 M Ruminy , F Groitl , T Keller , T Fennell

We have investigated the structural, electronic, and magnetic properties of the pyrochlore iridates Eu2Ir2O7 and Pr2Ir2O7 using a combination of resonant elastic x-ray scattering, x-ray powder diffraction, and resonant inelastic x-ray…

Tb2Ti2O7, a pyrochlore system, has garnered significant interest due to its intriguing structural and physical properties and their dependence on external physical parameters. In this study, utilizing high-brilliance synchrotron X-ray…

We present single-crystal neutron-diffuse-scattering measurements with polarization analysis on the spin ice Ho2-xYxTi2O7 (x = 0, 0.3, and 1). At 2 K, the spin flip scattering patterns are typical of a nearest-neighbor spin ice and the…

Strongly Correlated Electrons · Physics 2010-11-11 L. J. Chang , Y. Su , Y. -J. Kao , Y. Z. Chou , R. Mittal , H. Schneider , Th. Brueckel , G. Balakrishnan , M. R. Lees

Paramagnetic correlations in the magnetic material Yb2Ti2O7 have been investigated via neutron scattering, revealing a [111] rod of scattering intensity. Assuming interactions between the Yb^{3+} ions composed of all symmetry-allowed…

Strongly Correlated Electrons · Physics 2011-06-28 Jordan D. Thompson , Paul A. McClarty , Henrik M. Ronnow , Louis P. Regnault , Andreas Sorge , Michel J. P. Gingras

The superconducting pyrochlore oxide Cd2Re2O7 (Tc = 1 K), which is now considered as a candidate of the spin-orbit-coupled metal, shows an inversion-symmetry-breaking structural transition at Ts1 = 200 K. Ts1 decreases with increasing…

Strongly Correlated Electrons · Physics 2018-04-30 Yasuhito Matsubayashi , Takumi Hasegawa , Norio Ogita , Jun-ichi Yamaura , Zenji Hiroi

We report time-of-flight neutron scattering measurements of the magnetic spectrum of Tb3+ in Tb2Ti2O7. The data, which extend up to 120 meV and have calibrated intensity, enable us to consolidate and extend previous studies of the…

Strongly Correlated Electrons · Physics 2015-09-04 A. J. Princep , H. C. Walker , D. T. Adroja , D. Prabhakaran , A. T. Boothroyd

Large single crystals of the pyrochlore Pr2Hf2O7 have been successfully grown by the floating zone technique using an optical furnace equipped with high power Xenon arc lamps. Structural investigations have been carried out by both…

We provide experimental evidence for confinement of water molecules in the pores of hexagonal structure of YPO4 at elevated temperatures upto 600 K using powder neutron diffraction. In order to avoid the large incoherent scattering from the…

High resolution X-ray scattering measurements on single crystal Tb2Ti2O7 reveal finite structural correlations at low temperatures. This geometrically frustrated pyrochlore is known to exhibit a spin liquid, or cooperative paramagnetic…

Disordered Systems and Neural Networks · Physics 2009-11-13 J. P. C. Ruff , B. D. Gaulin , J. P. Castellan , K. C. Rule , J. P. Clancy , J. Rodriguez , H. A. Dabkowska

We report neutron scattering and muon spin relaxation measurements (muSR) on the pyrochlore antiferromagnet Yb2Ge2O7. Inelastic neutron scattering was used to probe the transitions between crystal electric field levels, allowing us to…

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi