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Two atoms in an ultracold gas are correlated at short inter-atomic distances due to threshold effects where the potential energy of their interaction dominates the kinetic energy. The correlations manifest themselves in a distinct nodal…

Atomic Physics · Physics 2011-04-15 Christiane P. Koch , Ronnie Kosloff

We suggest pump-probe spectroscopy to study pair correlations that determine the many-body dynamics in weakly interacting, dilute ultracold gases. A suitably chosen, short laser pulse depletes the pair density locally, creating a 'hole' in…

Quantum Physics · Physics 2009-12-22 Christiane P. Koch , Ronnie Kosloff

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond…

Quantum Physics · Physics 2015-06-22 Allan S. Johnson , Joel Yuen-Zhou , Alán Aspuru-Guzik , Jacob J. Krich

We examine electron-electron mediated relaxation following excitation of a correlated system by an ultrafast electric field pump pulse. The results reveal a dichotomy in the temporal evolution as one tunes through a Mott metal-to-insulator…

Strongly Correlated Electrons · Physics 2013-08-20 B. Moritz , A. F. Kemper , M. Sentef , T. P. Devereaux , J. K. Freericks

The development of high-intensity ultrashort laser pulses unlocks the potential of pump-probe spectroscopy in sub-femtosecond timescale. Notably, subcycle pump pulses can generate electronic states unreachable by conventional multicycle…

Strongly Correlated Electrons · Physics 2025-06-17 Kazuya Shinjo , Shigetoshi Sota , Seiji Yunoki , Takami Tohyama

An absorption of a weak pulse by two identical atoms moving in a trap is investigated. Based on atom-light interactions we present a microscopic model of a two-body wave function diagnosis. We study the influence of pulse properties on the…

Quantum Gases · Physics 2017-11-22 Rafał Ołdziejewski , Kazimierz Rzążewski

Ultrafast spectroscopies constitute a fundamental tool to investigate the dynamics of non-equilibrium many-body states in correlated materials. Two-pulses (pump-probe) experiments have shed new light on the interplay between high-energy…

Strongly Correlated Electrons · Physics 2016-09-01 Claudio Giannetti

We combine theoretical and experimental efforts to propose a method for studying energy fluctuations, in particular, to obtain the related bi-stochastic matrix of transition probabilities by means of simple measurements at the end of a…

Quantum Physics · Physics 2021-07-21 Marcela Herrera , John P. S. Peterson , Roberto M. Serra , Irene D'Amico

We investigate full quantum mechanical evolution of two electrons nonlinearly coupled to quantum phonons and simulate the dynamical response of the system subject to a short spatially uniform optical pulse that couples to dipole-active…

Statistical Mechanics · Physics 2025-03-06 K. Kovač , D. Golež , M. Mierzejewski , J. Bonča

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

The electron correlations in narrow energy bands are examined in framework of the Hubbard model. The single-particle Green function and energy spectrum are obtained in paramagnetic state at half-filling by means of new two-pole…

Strongly Correlated Electrons · Physics 2011-12-30 Leonid Didukh , Yuriy Skorenkyy

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Shaul Mukamel , Rafal Oszwaldowski , Lijun Yang

We investigate the effects of randomness in a strongly correlated electron model in one-dimension at half-filling. The ground state correlation functions are exactly written by products of 3$\times$3 transfer matrices and are evaluated…

Strongly Correlated Electrons · Physics 2009-10-28 Masanori Yamanaka , Mahito Kohmoto

This article gives an overview on recent theoretical progress in controlling the charge and spin dynamics in low-dimensional electronic systems by means of ultrashort and ultrabroadband electromagnetic pulses. A particular focus is put on…

Mesoscale and Nanoscale Physics · Physics 2017-02-15 Andrey S. Moskalenko , Zhen-Gang Zhu , Jamal Berakdar

A simple formula is obtained for coupling electrons in a complex system to the electromagnetic field. It includes the effect of intra-atomic excitations and nuclear motion, and can be applied in. e.g., first-principles-based simulations of…

Quantum Physics · Physics 2009-11-13 Roland E. Allen

Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron…

Strongly Correlated Electrons · Physics 2023-03-13 V. Valmispild , E. Gorelov , M. Eckstein , A. Lichtenstein , H. Aoki , M. Katsnelson , M. Ivanov , O. Smirnova

We present a model describing the use of ultra-short strong pulses to control the population of the excited level of a two-level quantum system. In particular, we study an off-resonance excitation with a few cycles pulse which presents a…

Quantum Physics · Physics 2015-06-15 Pankaj K. Jha , Hichem Eleuch , Fabio Grazioso

Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…

Chemical Physics · Physics 2024-04-11 Nikolay V. Golubev , Jiří Vaníček

We investigate the accuracy and efficiency of the semiclassical Frozen Gaussian method in describing electron dynamics in real time. Model systems of two soft-Coulomb-interacting electrons are used to study correlated dynamics under…

Chemical Physics · Physics 2015-05-30 Peter Elliott , Neepa T. Maitra
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