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Density matrix embedding theory (Phys. Rev. Lett. 109, 186404 (2012)) and density embedding theory ((Phys. Rev. B 89, 035140 (2014)) have recently been introduced for model lattice Hamiltonians and molecular systems. In the present work,…

Chemical Physics · Physics 2016-11-25 Ireneusz W. Bulik , Weibing Chen , Gustavo E. Scuseria

Density matrix embedding theory (DMET) is a relatively new technique for the calculation of strongly correlated systems. Recently, block product DMET (BPDMET) was introduced for the study of spin systems such as the antiferromagnetic $J_1 -…

Strongly Correlated Electrons · Physics 2017-05-30 Klaas Gunst , Sebastian Wouters , Stijn De Baerdemacker , Dimitri Van Neck

We describe a formulation of the density matrix embedding theory at finite temperature. We present a generalization of the ground-state bath orbital construction that embeds a mean-field finite-temperature density matrix up to a given order…

Strongly Correlated Electrons · Physics 2020-03-04 Chong Sun , Ushnish Ray , Zhi-Hao Cui , Miles Stoudenmire , Michel Ferrero , Garnet Kin-Lic Chan

We introduce DMET, a new quantum embedding theory for predicting ground-state properties of infinite systems. Like dynamical mean-field theory (DMFT), DMET maps the the bulk interacting system to a simpler impurity model and is exact in the…

Strongly Correlated Electrons · Physics 2015-03-20 Gerald Knizia , Garnet Kin-Lic Chan

We compute the ground-state phase diagram of the Hubbard and frustrated Hubbard models on the square lattice with density matrix embedding theory using clusters of up to 16 sites. We provide an error model to estimate the reliability of the…

Strongly Correlated Electrons · Physics 2016-01-27 Bo-Xiao Zheng , Garnet Kin-Lic Chan

The simulation of strongly correlated electron systems remains a formidable challenge. Certain experimentally relevant dynamical response functions are especially difficult to calculate, due to issues of finite-size effects and the ill…

Strongly Correlated Electrons · Physics 2026-03-25 Petar Brinić , Hugo U. R. Strand , Jakša Vučičević

Several variants of the recently proposed Density Matrix Embedding Theory (DMET) [G. Knizia and G. K-L. Chan, Phys. Rev. Lett. 109, 186404 (2012)] are formulated and tested. We show that spin symmetry breaking of the lattice mean-field…

Strongly Correlated Electrons · Physics 2015-06-17 Ireneusz W. Bulik , Gustavo E. Scuseria , Jorge Dukelsky

Quantum embedding based on the (one-electron reduced) density matrix is revisited by means of the unitary Householder transformation. While being exact and equivalent to (but formally simpler than) density matrix embedding theory (DMET) in…

Strongly Correlated Electrons · Physics 2021-07-12 Sajanthan Sekaran , Masahisa Tsuchiizu , Matthieu Saubanère , Emmanuel Fromager

Determining ground state energies of quantum systems by hybrid classical/quantum methods has emerged as a promising candidate application for near-term quantum computational resources. Short of large-scale fault-tolerant quantum computers,…

Quantum Physics · Physics 2016-10-25 Nicholas C. Rubin

We describe an efficient quantum embedding framework for realistic ab initio density matrix embedding (DMET) calculations in solids. We discuss in detail the choice of orbitals and mapping to a lattice, treatment of the virtual space and…

Strongly Correlated Electrons · Physics 2020-01-15 Zhi-Hao Cui , Tianyu Zhu , Garnet Kin-Lic Chan

The reduced density matrix of an interacting system can be used as the basis for a truncation scheme, or in an unbiased method to discover the strongest kind of correlation in the ground state. In this paper, we investigate the structure of…

Strongly Correlated Electrons · Physics 2009-11-11 Siew-Ann Cheong , Christopher L. Henley

Density matrix embedding theory (DMET) [Phys. Rev. Lett., 109, 186404 (2012)], introduced a new approach to quantum cluster embedding methods, whereby the mapping of strongly correlated bulk problems to an impurity with finite set of bath…

Strongly Correlated Electrons · Physics 2015-06-24 George H. Booth , Garnet Kin-Lic Chan

Density matrix embedding theory (DMET) describes finite fragments in the presence of a surrounding environment. In contrast to most embedding methods, DMET explicitly allows for quantum entanglement between both. In this chapter, we discuss…

Strongly Correlated Electrons · Physics 2018-02-19 Sebastian Wouters , Carlos A. Jiménez-Hoyos , Garnet K. -L. Chan

We illustrate how the systematic inclusion of multi-spin correlations of the quantum spin-lattice systems can be efficiently implemented within the framework of the coupled-cluster method by examining the ground-state properties of both the…

Statistical Mechanics · Physics 2017-08-24 Chen Zeng , D. J. J. Farnell , R. F. Bishop

Quantum embedding theories are promising approaches to investigate strongly-correlated electronic states of active regions of large-scale molecular or condensed systems. Notable examples are spin defects in semiconductors and insulators. We…

Materials Science · Physics 2021-12-14 He Ma , Nan Sheng , Marco Govoni , Giulia Galli

Entanglement in J_1-J_2, S=1/2 quantum spin chains with an impurity is studied using analytic methods as well as large scale numerical density matrix renormalization group methods. The entanglement is investigated in terms of the von…

Strongly Correlated Electrons · Physics 2011-11-09 Erik S. Sørensen , Ming-Shyang Chang , Nicolas Laflorencie , Ian Affleck

We extend density matrix embedding theory to periodic systems, resulting in an electronic band structure method for solid-state materials. The electron correlation can be captured by means of a local impurity model using various choices of…

Strongly Correlated Electrons · Physics 2019-09-27 Hung Q. Pham , Matthew R. Hermes , Laura Gagliardi

In this paper we discuss a family of models of particle and energy diffusion on a one-dimensional lattice, related to those studied previously in [Sasamoto-Wadati], [Barraquand-Corwin] and [Povolotsky] in the context of KPZ universality…

Mathematical Physics · Physics 2024-05-31 Rouven Frassek , Cristian Giardinà , Jorge Kurchan

Nanoscale physics and dynamical mean field theory have both generated increased interest in complex quantum impurity problems and so have focused attention on the need for flexible quantum impurity solvers. Here we demonstrate that the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jaebeom Yoo , Shailesh Chandrasekharan , Ribhu K. Kaul , Denis Ullmo , Harold U. Baranger

We investigate the cluster size convergence of the energy and observables using two forms of density matrix embedding theory (DMET): the original cluster form (CDMET) and a new formulation motivated by the dynamical cluster approximation…

Strongly Correlated Electrons · Physics 2017-01-11 Bo-Xiao Zheng , Joshua S. Kretchmer , Hao Shi , Shiwei Zhang , Garnet Kin-Lic Chan
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