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Manipulating spin polarization of electrons in nonmagnetic semiconductors by means of electric fields or optical fields is an essential theme of the conceptual nonmagnetic semiconductor-based spintronics. Here we experimentally demonstrate…

Mesoscale and Nanoscale Physics · Physics 2016-03-31 Xie Lu , Xiaodong Cui

In the field of photocatalytic water splitting, no current studies have explicitly investigated the coexistence of multiple band-edge alignments in two-dimensional (2D) materials with intrinsic electric fields. In this Letter, we designed…

Materials Science · Physics 2024-09-17 Zhi-Qiang Wen , Qiu Yang , Shu-Hao Cao , Zhao-Yi Zeng , Hua-Yun Geng , Xiang-Rong Chen

Moir\'e superlattices created by stacking atomic layers of transition metal dichalcogenide semiconductors have emerged as a class of fascinating artificial photonic and electronic materials. An appealing attribute of these structures is the…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Yueh-Chun Wu , Matthew DeCapua , ZhongChen Xu , Takashi Taniguchi , Kenji Watanabe , YouGuo Shi , Jun Yan

A new degree of freedom, the valley pseudospin, emerges in atomically thin two-dimensional transition metal dichalcogenides (MX2) and has attracted great scientific interest. The capability to manipulate the valley pseudospin, in analogy to…

Mesoscale and Nanoscale Physics · Physics 2014-12-10 Jonghwan Kim , Xiaoping Hong , Chenhao Jin , Su-Fei Shi , Chih-Yuan S. Chang , Ming-Hui Chiu , Lain-Jong Li , Feng Wang

We reveal an instantaneous optical valley selection rule that illuminates the coupling between the instantaneous optical chirality of the driving laser field and the chirality of valley systems. Building on this principle, we propose and…

Optics · Physics 2025-08-26 Wanzhu He , Xiaosong Zhu , Liang Li , Di Wu , Xiaotong Zhu , Pengfei Lan , Peixiang Lu

As hosts for tightly-bound electron-hole pairs carrying quantized angular momentum, atomically-thin semiconductors of transition metal dichalcogenides provide an appealing platform for optically addressing the valley degree of freedom. In…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Shao-Yu Chen , Thomas Goldstein , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Controlling crystallographic orientation in quasi-van der Waals (vdW) epitaxy remains a fundamental challenge, especially for material systems located near the boundary between weakly and strongly coupled growth regimes. In such marginal…

The valley degree of freedom is one of the most intriguing properties of atomically thin transition metal dichalcogenides. Together with the possibility to address this degree of freedom by valley-contrasting optical selection rules, it has…

Several monolayer transition metal dichalcogenides (TMDs) are direct band gap semiconductors and potentially efficient emitters in light emitting devices. Photons are emitted when strongly bound excitons decay radiatively, and accurate…

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

Mesoscale and Nanoscale Physics · Physics 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

2D materials with broken inversion symmetry posses an extra degree of freedom, the valley pseudospin, that labels in which of the two energy-degenerate crystal momenta, K or K', the conducting carriers are located. It has been shown that…

Quantum Physics · Physics 2023-09-20 Rui E. F. Silva , Misha Ivanov , Álvaro Jiménez-Galán

Electronic and spintronic devices rely on the fact that free charge carriers in solids carry electric charge and spin, respectively. There are, however, other properties of charge carriers that might be exploited in new families of devices.…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Kin Fai Mak , Keliang He , Jie Shan , Tony F. Heinz

Coupling between exciton states across the Brillouin zone in monolayer transition metal dichalcogenides can lead to ultrafast valley depolarization. Using time- and angle-resolved photoemission, we present momentum- and energy-resolved…

Atomically thin materials such as graphene and monolayer transition metal dichalcogenides (TMDs) exhibit remarkable physical properties resulting from their reduced dimensionality and crystal symmetry. The family of semiconducting…

Over the past few decades, thin film optoelectronic devices based on transition metal dichalcogenides (TMDs) have made significant progress. However, the sensitivity of the exciton states to environmental change presents challenges for…

Optics · Physics 2024-03-13 Shuangping Han , Pengyu Zan , Yu Yan , Yaoxing Bian , Chengbing Qin , Liantuan Xiao

We discuss selection rules and intensities of photocurrent of a two-dimensional electron gas in a strong magnetic field via absorptions of orbital angular momentum carried by obliquely irradiated optical vortex beams. By angular deflection,…

Mesoscale and Nanoscale Physics · Physics 2021-11-19 Hirohisa T. Takahashi , Jun-ichiro Kishine

Twisted light carries a well-defined orbital angular momentum (OAM) per photon. The quantum number l of its OAM can be arbitrarily set, making it an excellent light source to realize high-dimensional quantum entanglement and ultra-wide…

We calculate the binding energy, transition energies, oscillator strength, and absorption coefficient of indirect excitons in transition metal dichalcogenide (TMDC) double layers separated by an integer number of hexagonal boron nitride…

Mesoscale and Nanoscale Physics · Physics 2018-09-19 Matthew N. Brunetti , Oleg L. Berman , Roman Ya. Kezerashvili

We propose a scheme to trap and filter electrons, valley dependently, on a scale beyond the diffraction limit, in a gapped Dirac system using a circularly polarized light beam and a microscale metallic resonator. The main mechanism allowing…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Kevin Dini , Ivan V. Iorsh , Andrey Bogdanov , Ivan A. Shelykh

Rich valleytronics and diverse defect-induced or interlayer pre-bandgap excitonics have been extensively studied in transition metal dichalcogenides (TMDCs), a system with fascinating optical physics. However, more intense high-energy…

Materials Science · Physics 2021-04-02 Jinhua Hong , Masanori Koshino , Ryosuke Senga , Thomas Pichler , Hua Xu , Kazu Suenaga