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The analytical formula for the time-resolved dynamical Franz-Keldysh effect (Tr-DFKE) under an elliptically polarized laser in sub-femtosecond time-scale is reported. The Houston function is assumed as the time-dependent wave function of…

Optics · Physics 2016-11-23 T. Otobe

We introduce and analyze the properties of dynamical Franz-Keldysh effect, i.e. the change of density-of-states, or absorption spectra, of semiconductors under the influence of {\it time-dependent} electric fields. In the case of a harmonic…

Condensed Matter · Physics 2009-10-28 A. P. Jauho , K. Johnsen

The speed of ultra-fast optical switches is generally limited by the intrinsic electronic response time of the material. Here we show that the phase content of selected electromagnetic pulses can be used to measure the timescales…

An ultrafast anisotropic electro-optic effect of the zinc sulfide crystal is predicted employing a numerical pump-probe simulation. The numerical results indicate that the time-dependence of the anisotropic response of ZnS exhibits a phase…

Optics · Physics 2019-09-11 T. Otobe

We theoretically investigate a relation between the crystalline symmetry and the transient modulation of optical properties of crystalline dielectrics in pump-probe measurements using intense pump and attosecond probe fields. When the…

Materials Science · Physics 2020-04-29 Shunsuke Yamada , Kazuhiro Yabana

We report here the analytical formula for the time-resolved dynamical Franz-Keldysh effect (Tr-DFKE) under circularly polarized light. We assume the Houston function as the time-dependent wave function of the parabolic two-band system. Our…

Mesoscale and Nanoscale Physics · Physics 2016-05-31 T. Otobe

Starting from a quantum kinetic equation including the mean field and a conserving relaxation-time approximation we derive an analytic formula which describes the time dependence of the dielectric function in a plasma created by a short…

Strongly Correlated Electrons · Physics 2008-12-18 K. Morawetz , P. Lipavský , M. Schreiber

The deep ultraviolet, the bandgap region of dielectrics, is not readily accessible for established methods of ultrafast spectroscopy. Here, a miniature beamline, where a tailored deep ultraviolet field is used immediately after the…

Molecular absorption and photo-electron spectra can be efficiently predicted with real-time time-dependent density-functional theory (TDDFT). We show here how these techniques can be easily extended to study time-resolved pump-probe…

Atomic and Molecular Clusters · Physics 2013-01-10 Umberto De Giovannini , Gustavo Brunetto , Alberto Castro , Jessica Walkenhorst , Angel Rubio

The last decade has witnessed a rapid advancement in laser technology, enabling the direct monitoring and control of electronic motion on its natural attosecond to sub-femtosecond timescales. Ultrafast processes are conventionally studied…

Chemical Physics · Physics 2026-05-27 Torsha Moitra

We report a Keldysh-like model for the electron transition rate in dielectrics under an intense circularly polarized laser. We assume a parabolic two-band system and the Houston function as the time-dependent wave function of the valence…

Mesoscale and Nanoscale Physics · Physics 2016-12-21 T. Otobe , Y. Shinohara , S. A. Sato , K. Yabana

Energy transfer processes from a high-intensity ultrashort laser pulse to electrons in simple dielectrics, silicon, diamond, and $\alpha$-quartz are theoretically investigated by first-principles calculations based on time-dependent density…

Optics · Physics 2019-05-22 Atsushi Yamada , Kazuhiro Yabana

Recent advances in laser technology allow us to follow electronic motion at its natural time-scale with ultra-fast time resolution, leading the way towards attosecond physics experiments of extreme precision. In this work, we assess the use…

Other Condensed Matter · Physics 2016-06-22 Jessica Walkenhorst , Umberto De Giovannini , Alberto Castro , Angel Rubio

The redistribution of electrons in an ultrafast pump-probe experiment causes significant changes to the effective interaction between electrons and bosonic modes. We study the influence of these changes on pump-probe photoemission…

Mesoscale and Nanoscale Physics · Physics 2014-08-25 A. F. Kemper , M. A. Sentef , B. Moritz , J. K. Freericks , T. P. Devereaux

We present a theoretical description of femtosecond laser induced dynamics of the hydrogen molecule and of singly ionised sodium dimers, based on a real-space, real-time, implementation of time-dependent density functional theory (TDDFT).…

Condensed Matter · Physics 2007-05-23 Alberto Castro , M. A. L. Marques , Julio A. Alonso , George F. Bertsch , Angel Rubio

This study expands the spontaneous collapse assumptions into the relativistic quantum field theory framework for Dirac fields. By solving Lindblad's master equation using the Keldysh formalism, the effective action is derived, which…

High Energy Physics - Theory · Physics 2025-11-18 Y. M. P. Gomes

A theoretical frame for pump-probe photoemission is presented. The approach is based on a general formulation using the Keldysh formalism for the lesser Green's function to describe the real-time evolution of the electronic degrees of…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 J. Braun , R. Rausch , M. Potthoff , J. Minar , H. Ebert

The transient signals derived from femtosecond pump-probe experiments are analyzed in terms of the coherent evolution of the energy levels perturbed by the excitation pulse. The model system is treated as the sum of independent two-level…

Atomic Physics · Physics 2016-09-13 A. Peralta Conde , R. Montero , A. Longarte

We applied the time-resolved attosecond transient absorption spectroscopy to systematically investigate ultrafast optical responses of condensed matter systems. Under an intense pump pulse, absorption spectra indicate that the…

Strongly Correlated Electrons · Physics 2023-07-26 Youngjae Kim

Franz-Keldysh effect is expressed in the smearing of the absorption edge in semiconductors under high electric fields. While Franz and Keldysh considered a limited case of externally applied uniform electric field, the same effect may be…

Applied Physics · Physics 2018-08-30 Yury Turkulets , Ilan Shalish
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