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We study the dynamics of active Janus particles that self-propel in solution by light-activated catalytic decomposition of chemical "fuel." We develop an analytical model of a photo-active self-phoretic particle that accounts for…

Soft Condensed Matter · Physics 2019-05-23 W. E. Uspal

Surface bound catalytic chemical reactions self-propel chemically active Janus particles. In the vicinity of boundaries, these particles exhibit rich behavior, such as the occurrence of wall-bound steady states of "sliding". Most active…

The single-particle and collective dynamics of systems comprising Janus motors, solvent and reactive solute species maintained in nonequilibrium states are investigated. Reversible catalytic reactions with the solute species take place on…

Soft Condensed Matter · Physics 2019-05-01 Mu-Jie Huang , Jeremy Schofield , Pierre Gaspard , Raymond Kapral

We develop a new model, to our knowledge, for the many-body hydrodynamics of amphiphilic Janus particles suspended in a viscous background flow. The Janus particles interact through a hydrophobic attraction potential that leads to…

Soft Condensed Matter · Physics 2021-10-05 Szu-Pei Fu , Bryan Quaife , Rolf Ryham , Yuan-Nan Young

We present a derivation from first principles of the coupled equations of motion of an active self-diffusiophoretic Janus motor and the hydrodynamic densities of its fluid environment that are nonlinearly displaced from equilibrium. The…

Soft Condensed Matter · Physics 2024-01-05 Bryan Robertson , Jeremy Schofield , Raymond Kapral

We deeply investigate a simple model representative of the recently synthesized Janus particles, i.e. colloidal spherical particles whose surface is divided into two areas of different chemical composition. When the two surfaces are…

Soft Condensed Matter · Physics 2009-12-21 Francesco Sciortino , Achille Giacometti , Giorgio Pastore

A multicomponent mixture of Janus colloids with distinct catalytic coats and phoretic mobilities is a promising theoretical system to explore the collective behavior arising from nonreciprocal interactions. An active colloid produces (or…

Soft Condensed Matter · Physics 2024-02-15 Gennaro Tucci , Ramin Golestanian , Suropriya Saha

Janus motors with chemically active and inactive hemispheres can operate only under nonequilibrium conditions where detailed balance is broken by fluxes of chemical species that establish a nonequilibrium state. A microscopic model for…

Soft Condensed Matter · Physics 2018-08-01 Mu-Jie Huang , Jeremy Schofield , Pierre Gaspard , Raymond Kapral

Active Brownian particles are capable of taking up energy from their environment and converting it into directed motion; examples range from chemotactic cells and bacteria to artificial micro-swimmers. We have recently demonstrated that…

Soft Condensed Matter · Physics 2012-06-29 Ivo Buttinoni , Giovanni Volpe , Felix Kümmel , Giorgio Volpe , Clemens Bechinger

The electromagnetic field scattered by nano-objects contains a broad range of wave vectors and can be efficiently coupled to waveguided modes. The dominant contribution to scattering from subwavelength dielectric and plasmonic nanoparticles…

We demonstrate differential dynamic microscopy and particle tracking for the characterization of the spatiotemporal behavior of active Janus colloids in terms of the intermediate scattering function (ISF). We provide an analytical solution…

We study the relaxation dynamics of a binary liquid mixture near a light-absorbing Janus particle after switching on and off illumination using experiments and theoretical models. The dynamics is controlled by the temperature gradient…

Soft Condensed Matter · Physics 2022-02-02 Takeaki Araki , Juan Ruben Gomez-Solano , Anna Maciołek

We numerically investigated the Brownian motion of active Janus particles in a linear array of planar counter-rotating convection rolls at high P\'eclet numbers. Similarly to passive particles, active microswimmers exhibit advection…

Statistical Mechanics · Physics 2025-08-14 Pulak Kumar Ghosh , Fabio Marchesoni , Yunyun Li , Franco Nori

We consider the demixing of a binary fluid mixture, under gravity, which is steadily driven into a two phase region by slowly ramping the temperature. We assume, as a first approximation, that the system remains spatially isothermal, and…

Soft Condensed Matter · Physics 2009-11-10 M. E. Cates , J. Vollmer , A. Wagner , D. Vollmer

Catalytically active Janus particles suspended in solution create gradients in the chemical composition of the solution along their surfaces, as well as along any nearby container walls. The former leads to self-phoresis, while the latter…

Soft Condensed Matter · Physics 2016-09-22 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

We numerically investigate normal diffusion in a two-dimensional athermal suspension of active particles undergoing motility-induced phase separation. The particles are modeled as achiral Janus disks with fixed self-propulsion speed and…

Soft Condensed Matter · Physics 2025-02-20 Shubhadip Nayak , Poulami Bag , Pulak K. Ghosh , Yuxin Zhou , Qingqing Yin , Fabio Marchesoni , Franco Nori

Capillary interactions can be used to direct assembly of particles adsorbed at fluid-fluid interfaces. Precisely controlling the magnitude and direction of capillary interactions to assemble particles into favoured structures for materials…

Soft Condensed Matter · Physics 2016-07-11 Qingguang Xie , Gary B. Davies , Jens Harting

In this work, we use Molecular Dynamics and Lattice-Boltzmann simulations to study the properties of charged Janus particles in an electric field. We show that for relatively small net charge and thick electrostatic diffuse layer mobilities…

Soft Condensed Matter · Physics 2017-09-12 Taras Y. Molotilin , Vladimir Lobaskin , Olga I. Vinogradova

We propose a highly efficient mechanism to rectify the motion of active particles by exploiting particle-wall alignment interactions. Through numerical simulations of active particles' dynamics in a narrow channel, we demonstrate that a…

Soft Condensed Matter · Physics 2025-11-07 Poulami Bag , Tanwi Debnath , Shubhadip Nayak , Pulak K. Ghosh

Shear-thinning viscosity is a non-Newtonian behaviour that active particles often encounter in biological fluids such as blood and mucus. The fundamental question of how this ubiquitous non-Newtonian rheology affects the propulsion of…

Fluid Dynamics · Physics 2025-04-30 Guangpu Zhu , Brandon van Gogh , Lailai Zhu , On Shun Pak , Yi Man