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When water molecules are confined to nanoscale spacings, such as in the nanometer size pores of activated carbon fiber (ACF), their freezing point gets suppressed down to very low temperatures ($\sim$ 150 K), leading to a metastable liquid…

Soft Condensed Matter · Physics 2015-06-23 S. O. Diallo , L. Vlcek , E. Mamontov , J. K. Keum , Jihua Chen , J. S. Hayes , A. A. Chialvo

It is well known that water inside hydrophobic nano-channels diffuses faster than bulk water. Recent theoretical studies have shown that this enhancement depends on the size of the hydrophobic nanochannels. However, experimental evidence of…

We report a study of the effects of pressure on the diffusivity of water molecules confined in single- wall carbon nanotubes (SWNT) with average mean pore diameter of 16 Angstroms. The measurements were carried out using high-resolution…

Soft Condensed Matter · Physics 2015-06-16 S. O. Diallo , M. Jazdzewska , J. C. Palmer , E. Mamontov , K. E. Gubbins , M. Sliwinska-Bartkowiak

Context. The diffusion of volatile species on amorphous solid water ice affects the chemistry on dust grains in the interstellar medium as well as the trapping of gases enriching planetary atmospheres or present in cometary material. Aims.…

Instrumentation and Methods for Astrophysics · Physics 2021-03-01 Belén Maté , Stephanie Cazaux , Miguel Angel Satorre , Germán Molpeceres , Juan Ortigoso , Carlos Millán , Carmina Santonja

We report the diffusion of water molecules confined in the pores of folded silica materials (FSM-12 with average pore diameter of $\sim$ 16 \AA), measured by means of quasielastic neutron scattering using the cold neutron chopper…

Soft Condensed Matter · Physics 2015-06-16 S. O. Diallo , E. Mamontov , A. Podlesnyak , G. Ehlers , N. Wada , S. Inagaki , Y. Fukushima

We use $^2$H NMR to study the rotational motion of supercooled water in silica pores of various diameters, specifically, in the MCM-41 materials C10, C12, and C14. Combination of spin-lattice relaxation, line-shape, and stimulated-echo…

Soft Condensed Matter · Physics 2015-06-22 Matthias Sattig , Stefan Reutter , Franz Fujara , Mayke Werner , Gerd Buntkowsky , Michael Vogel

The evaporation coefficients of water in air and nitrogen were found as a function of temperature, by studying the evaporation of pure water droplet. The droplet was levitated in an electrodynamic trap placed in a climatic chamber…

Chemical Physics · Physics 2016-09-28 M. Zientara , D. Jakubczyk , K. Kolwas , M. Kolwas

We use molecular dynamics simulations to study the diffusion of water inside deformed carbon nanotubes, with different degrees of eccentricity at 300K. We found a water structural transition between tubular-like to single-file for the (7,7)…

In this article we investigate through molecular dynamics simulations the diffusion behavior of the TIP4P/2005 water when confined in pristine and deformed carbon nanotubes (armchair and zigzag). To analyze different diffusive mechanisms,…

Soft Condensed Matter · Physics 2021-02-03 Bruno H. S. Mendonça , Patricia Ternes , Evy Salcedo , Alan B. de Oliveira , Marcia C. Barbosa

We compared the diffusion of water confined in armchair and zigzag carbon nanotubes for rigid and flexible water models. Using one rigid model, TIP4P/2005, and two flexible models, SPC/Fw and SPC/FH, we found that the number of the number…

The diffusion of water molecules through mesoporous dust of amorphous carbon (a-C) is a key process in the evolution of prestellar, protostellar, and protoplanetary dust, as well as in that of comets. It also plays a role in the formation…

Instrumentation and Methods for Astrophysics · Physics 2024-03-05 Romain Basalgète , Gaël Rouillé , Cornelia Jäger

The influence of spatial confinement on the thermally excited stochastic cation dynamics of the room-temperature ionic liquid 1-N-butylpyridinium bis-((trifluoromethyl)sulfonyl)imide ([BuPy][Tf_2N]) inside porous carbide-derived carbons…

Chemical Physics · Physics 2020-06-02 Mark Busch , Tommy Hofmann , Bernhard Frick , Jan P. Embs , Boris Dyatkin , Patrick Huber

Molecular dynamics simulation is a prominent way of analyzing the dynamic properties of a system. The molecular dynamics simulation of diffusion, an important transport property, of dilute solution of cysteine in SPCE water at five…

Chemical Physics · Physics 2018-09-25 Hem Prasad Bhusal , Narayan Prasad Adhikari

The quest for efficient and economically accessible cleaner methods to develop sustainable carbon-free energy sources induced a keen interest in the production of hydrogen fuel. This can be achieved via the water-splitting process…

In the last decades a large effort has been devoted to the study of water confined in hydrophobic geometries at the nanoscale (tubes, slit pores), because of the multiple technological applications of such systems, ranging from drugs…

Soft Condensed Matter · Physics 2019-12-23 A Zaragoza , MA Gonzalez , L Joly , I Lopez-Montero , MA Canales , AL Benavides , C Valeriani

The diffusion of atoms and radicals on interstellar dust grains is a fundamental ingredient for predicting accurate molecular abundances in astronomical environments. Quantitative values of diffusivity and diffusion barriers usually rely…

Astrophysics of Galaxies · Physics 2021-12-22 Viktor Zaverkin , Germán Molpeceres , Johannes Kästner

Molecular dynamics simulations are carried out to explore the dynamical crossover phenomenon in strongly confined and mildly supercooled water in graphene oxide nanopores. In contrast to studies where confinement is used to study the…

Soft Condensed Matter · Physics 2020-03-09 Rajasekaran M , K. Ganapathy Ayappa

We have investigated the diffusion and structure of TIP4P/2005 water confined in carbon nanotubes subjected to external electric fields. A wide range of diameters has been used to show a highly size-dependent behavior of the water…

Water plays a key role in biological membrane transport. In ion channels and water-conducting pores (aquaporins), one dimensional confinement in conjunction with strong surface effects changes the physical behavior of water. In molecular…

Biological Physics · Physics 2019-07-02 Oliver Beckstein , Mark S. P. Sansom

Hydrated excess protons under hydrophobic confinement are a critical component of charge transport behavior and reactivity in nanoporous materials and biomolecular systems. Herein excess proton confinement effects are computationally…

Soft Condensed Matter · Physics 2020-06-04 Xinyou Ma , Chenghan Li , Alex B. F. Martinson , Gregory A. Voth
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