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Amorphous solids or glasses are known to exhibit stretched-exponential decay over broad time intervals in several of their macroscopic observables: intermediate scattering function, dielectric relaxation modulus, time-elastic modulus etc.…

Soft Condensed Matter · Physics 2017-01-19 B. Cui , R. Milkus , A. Zaccone

Glasses are out-of-equilibrium systems aging under the crystallization threat. During ordinary glass formation, the atomic diffusion slows down rendering its experimental investigation impractically long, to the extent that a timescale…

Disordered Systems and Neural Networks · Physics 2015-08-28 E. A. A. Pogna , C. Rodríguez-Tinoco , G. Cerullo , C. Ferrante , J. Rodríguez-Viejo , T. Scopigno

The complex shear modulus of solid $^4$He exhibits an anomaly in the same temperature region where torsion oscillators show a change in period. We propose that the observed stiffening of the shear modulus with decreasing temperature can be…

Statistical Mechanics · Physics 2012-12-06 Jung-Jung Su , Matthias J. Graf , Alexander V. Balatsky

We construct a linear response theory of applying shear deformations from boundary walls in the film geometry in Kubo's theoretical scheme. Our method is applicable to any solids and fluids. For glasses, we assume quasi-equilibrium around a…

Soft Condensed Matter · Physics 2018-12-27 Akira Onuki , Takeshi Kawasaki

Molecular dynamics simulations are performed to examine the dynamic response of amorphous solids to oscillatory shear at finite temperatures. The data were collected from a poorly annealed binary glass, which was deformed periodically in…

Soft Condensed Matter · Physics 2017-11-21 Nikolai V. Priezjev

We theoretically investigate glass transition behaviors of the glassy graphene in a wide range of temperature, where this amorphous graphene is described as a hard-sphere fluid. The dynamic arrest of a particle is assumingly caused by…

Soft Condensed Matter · Physics 2020-03-11 Tran Dinh Cuong , Anh D. Phan , Katsunori Wakabayashi , Pham Thanh Huy

We report surface shear rheological measurements on dense insoluble monolayers of micron sized colloidal spheres at the oil/water interface and of the protein $\beta$-lactoglobulin at the air/water surface. As expected, the elastic modulus…

Soft Condensed Matter · Physics 2009-11-10 Pietro Cicuta , Edward J. Stancik , Gerald G. Fuller

We compute the shear modulus of structural glasses from a first principle approach based on the cloned liquid theory. We find that the intra-state shear-modulus, which corresponds to the plateau modulus measured in linear visco-elastic…

Soft Condensed Matter · Physics 2015-05-18 Hajime Yoshino , Marc Mezard

The universal anomalous vibrational and thermal properties of amorphous solids are believed to be related to the local variations of the elasticity. Recently it has been shown that the vibrational properties are sensitive to the glass's…

Soft Condensed Matter · Physics 2019-09-30 Alireza Shakerpoor , Elijah Flenner , Grzegorz Szamel

We investigate by means of molecular dynamics simulation a coarse-grained polymer glass model focusing on (quasi-static and dynamical) shear-stress fluctuations as a function of temperature T and sampling time $\Delta t$. The linear…

Soft Condensed Matter · Physics 2018-01-17 I. Kriuchevskyi , J. P. Wittmer , H. Meyer , O. Benzerara , J. Baschnagel

We performed parallel measurements of heat effects and shear modulus relaxation for glassy Te$_{75}$Ge$_{15}$Ga$_{10}$ taken as a representative of practically important non-metallic glasses with covalent bonding. It is shown that the heat…

Disordered Systems and Neural Networks · Physics 2026-05-27 G. V. Afonin , R. A. Konchakov , D. A. Chareev , S. A. Badmaeva , R. S. Khmyrov , A. N. Vasiliev , N. P. Kobelev , V. A. Khonik

Randomly crosslinked macromolecules undergo a liquid-to-amorphous solid phase transition at a critical crosslink concentration. This transition has two main signatures: the random localization of a fraction of the monomers and the emergence…

Disordered Systems and Neural Networks · Physics 2009-10-31 Horacio E. Castillo , Paul M. Goldbart

The glass transition refers to the non-equilibrium process by which an equilibrium liquid is transformed to a non-equilibrium disordered solid, or vice versa. Associated response functions, such as heat capacities, are markedly different on…

Soft Condensed Matter · Physics 2013-03-26 Aaron S. Keys , Juan P. Garrahan , David Chandler

The yielding of foams, concentrated emulsions, pastes and other soft materials under applied strain is often characterized by measuring the complex shear modulus as a function of strain amplitude at low frequency. Results obtained for…

Soft Condensed Matter · Physics 2007-05-23 Reinhard Hohler , Sylvie Cohen-Addad , Vincent Labiausse

The elastic response of a two-dimensional amorphous solid to induced local shear transformations, which mimic the elementary plastic events occurring in deformed glasses, is investigated via Molecular Dynamics simulations. We show that for…

Soft Condensed Matter · Physics 2014-08-01 Francesco Puosi , Joerg Rottler , Jean-Louis Barrat

The structure, thermodynamics and slow activated dynamics of the equilibrated metastable regime of glass-forming fluids remains a poorly understood problem of high theoretical and experimental interest. We apply a highly accurate…

Soft Condensed Matter · Physics 2024-08-21 Subhashish Chaki , Baicheng Mei , Kenneth S. Schweizer

We propose a dynamical theory of low-temperature shear deformation in amorphous solids. Our analysis is based on molecular-dynamics simulations of a two-dimensional, two-component noncrystalline system. These numerical simulations reveal…

Statistical Mechanics · Physics 2009-10-30 M. L. Falk , J. S. Langer

Amorphous solids are viscoelastic. They dissipate energy when deformed at finite rate and finite temperature. We here use analytic theory and molecular simulations to demonstrate that linear viscoelastic dissipation can be directly related…

Soft Condensed Matter · Physics 2024-02-23 Jan Grießer , Lars Pastewka

We report measurements of the frequency-dependent shear moduli of aging colloidal systems that evolve from a purely low-viscosity liquid to a predominantly elastic glass or gel. Using microrheology, we measure the local complex shear…

Soft Condensed Matter · Physics 2009-11-13 S. Jabbari-Farouji , M. Atakhorram , D. Mizuno , E. Eiser , G. H. Wegdam , F. C. MacKintosh , Daniel Bonn , C. F. Schmidt

Using molecular dynamics simulation of a standard coarse-grained polymer glass model we investigate by means of the stress-fluctuation formalism the shear modulus $\mu$ as a function of temperature $T$ and sampling time $\Delta t$. While…

Soft Condensed Matter · Physics 2017-11-03 I. Kriuchevskyi , J. P. Wittmer , H. Meyer , J. Baschnagel