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Atomically thin transition metal dichalcogenides are highly promising for integrated optoelectronic and photonic systems due to their exciton-driven linear and nonlinear interaction with light. Integrating them into optical fibers yields…

The two-dimensional semiconductor MoS2 in its mono- and few-layer form is expected to have a significant exciton binding energy of several 100 meV, leading to the consensus that excitons are the primary photoexcited species. Nevertheless,…

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

Nanoplasmonic systems combined with optically-active two-dimensional materials provide intriguing opportunities to explore and control light-matter interactions at extreme sub-wavelength lengthscales approaching the exciton Bohr radius.…

We directly monitor exciton propagation in freestanding and SiO2-supported WS2 monolayers through spatially- and time-resolved micro-photoluminescence under ambient conditions. We find highly nonlinear behavior with characteristic,…

The multi-scale computational method of combining first-principles calculation and finite element electromagnetic simulations is used to study plasmon-enhanced interlayer charge transfer (ICT) exciton of 2D lateral and van der Waals…

Optics · Physics 2020-03-30 Xijiao Mu , Mengtao Sun

Strong spatial confinement and highly reduced dielectric screening provide monolayer transition metal dichalcogenides (TMDCs) with strong many-body effects, thereby possessing optically forbidden excitonic states (i.e., dark excitons) at…

We present a theoretical study of the optical response of a nonlinear oscillator formed by coupling a metal nanoparticle local surface plasmon resonance to excitonic degrees of freedom in a monolayer transition-metal dichalcogenide. We show…

Mesoscale and Nanoscale Physics · Physics 2019-06-13 Daniel B. S. Soh , Ryotatsu Yanagimoto , Eric Chatterjee , Hideo Mabuchi

By making use of circularly polarized light and electrostatic gating, monolayer molybdenum disulfide (ML-MoS$_2$) can form a platform supporting multiple types of charge carriers. They can be discriminated by their spin, valley index or…

Mesoscale and Nanoscale Physics · Physics 2017-08-17 Y. M. Xiao , W. Xu , F. M. Peeters , B. Van Duppen

Two-dimensional (2D) transition metal dichalcogenides (TMDCs), exemplified by molybdenum disulfide (MoS2), have shown exceptional potential for data-centred, energy-efficient electronic applications due to their unique electrical,…

Monolayer transition metal dichalcogenides are uniquely-qualified materials for photonics because they combine well defined tunable direct band gaps and selfpassivated surfaces without dangling bonds. However, the atomic thickness of these…

We propose a method that enables strong, coherent coupling between individual optical emitters and electromagnetic excitations in conducting nano-structures. The excitations are optical plasmons that can be localized to sub-wavelength…

Quantum Physics · Physics 2009-11-13 D. E. Chang , A. S. Sorensen , P. R. Hemmer , M. D. Lukin

Light emitters in vicinity of a hyperbolic metamaterial (HMM) show a range of quantum optical phenomena from spontaneous decay rate enhancement to strong coupling. In this study, we integrate monolayer Molybdenum disulfide (MoS$_2$) emitter…

Optics · Physics 2022-08-05 Harshavardhan R. Kalluru , Jaydeep K. Basu

When combined into van der Waals heterostructures, transition metal dichalcogenide monolayers enable the exploration of novel physics beyond their unique individual properties. However, for interesting phenomena such as interlayer charge…

By extracting the permittivity of monolayer MoS2 from experiments, the optical absorption of monolayer MoS2 prepared on top of one-dimensional photonic crystal (1DPC) or metal films is investigated theoretically. The 1DPC and metal films…

Optics · Physics 2016-02-01 Jiang-Tao Liu , Tong-Biao Wang , Xiao-Jing Li , Nian-Hua Liu

We report a photoluminescence (PL) and transient reflection spectroscopy study of exciton dynamics in monolayer transition transition-metal dichalcogenides (TMDs). PL saturation in monolayer MoSe2 occurs an excitation intensity more than…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Min Ju Shin , Dong Hak Kim , D. Lim

We study photoluminescence (PL) spectra and exciton dynamics of MoS$_2$ monolayer (ML) grown by the chemical vapor deposition technique. In addition to the usual direct A-exciton line we observe a low-energy line of bound excitons…

Mesoscale and Nanoscale Physics · Physics 2021-09-14 M. A. Akmaev , M. M. Glazov , M. V. Kochiev , P. V. Vinokurov , S. A. Smagulova , V. V. Belykh

Transition metal dichalcogenides layered nano-crystals are emerging as promising candidates for next-generation optoelectronic and quantum devices. In such systems, the interaction between excitonic states and atomic vibrations is crucial…

Mesoscale and Nanoscale Physics · Physics 2023-12-29 Jianbo Hu , Yang Xiang , Beatrice Matilde Ferrari , Emilio Scalise , Giovanni Maria Vanacore

The optical and electronic properties of multilayer transition metal dichalcogenides differ significantly from their monolayer counterparts due to interlayer interactions. The separation of individual layers can be tuned in a controlled way…

Excitons in two-dimensional transition metal dichalcogenides have a valley degree of freedom that can be optically accessed and manipulated for quantum information processing. Here, we integrate MoS2 with achiral silicon disk array…