Related papers: Ultralong-Range Rydberg Molecules in a Divalent-At…
We investigate the impact of combined electric and magnetic fields on the structure of ultralong-range polar Rydberg molecules. Our focus is hereby on the parallel as well as the crossed field configuration taking into account both the…
An operator that generates an approximate symmetry of long-range Rydberg molecules (LRRMs) formed by two alkali atoms, one in a Rydberg state and the other in the ground state, is identified. This is first done by evaluating the natural…
Out-of-equilibrium, strong correlation in a many-body system triggers emergent properties that can act in important ways to constrain the natural dissipation of energy and matter. Networks of atoms, intricately engineered to arrange…
We present photodissociation of ultracold long-range Rydberg molecules as a tool to characterize their electronic properties. We photoassociate K2 37P molecules with highly entangled electronic and nuclear spins of the two bound atoms and…
Atoms with a highly excited electron, called Rydberg atoms, can form unusual types of molecular bonds. The bond differs from the well known ionic and covalent bonds not only by its binding mechanism, but also by its bond length ranging up…
We report the observation of cold Cs Rydberg atom molecules bound at internuclear separations of R~3-9 um. The bound states result from avoided crossings between Rydberg atom pair interaction potentials in an applied electric field. The…
An approach to fast entanglement generation based on Rydberg dephasing of collective excitations (spin-waves) in large, optically thick atomic ensembles is proposed. Long-range $1/r^3$ atomic interactions are induced by microwave mixing of…
We demonstrate experimentally that a single Rb atom excited to the $79d_{5/2}$ level blocks the subsequent excitation of a second atom located more than $10 \mu\rm m$ away. The observed probability of double excitation of $\sim 30%$ is…
We observe a series of conical intersections in the potential energy curves governing both the collision between a Rydberg atom and a ground-state atom and the structure of Rydberg molecules. By employing the electronic energy of the…
We explore the electronic structure and rovibrational properties of an ultralong-range triatomic Rydberg molecule formed by a Rydberg atom and a ground state heteronuclear diatomic molecule. We focus here on interaction of Rb($27s$) Rydberg…
We propose a mechanism of ground-state blockade between two $N$-type Rydberg atoms in virtue of Rydberg-antiblockade effect and Raman transition. Inspired by the quantum Zeno effect, the strong Rydberg antiblockade interaction plays a role…
We demonstrate the interaction-induced blockade effect in an ultracold $^{88}$Sr gas via studying the time dynamics of a two-photon excitation to the triplet Rydberg series $5\mathrm{s}n\mathrm{s}\, ^3\textrm{S}_1$ for five different…
Controlling molecular binding at the level of single atoms is one of the holy grails of quantum chemistry. Rydberg macrodimers -- bound states between highly excited Rydberg atoms -- provide a novel perspective in this direction. Resulting…
Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from…
We report on the observation of highly excited ($\nu \sim 100)$ vibrational states of a trilobite ultralong-range Rydberg molecule in $^{87}$Rb. These states manifest spectroscopically in a regularly spaced series of peaks red-detuned from…
We propose a new method to create two-photon states in a controllable way using interaction between the Rydberg atoms during the storage and retrieval of slow light. A distinctive feature of the suggested procedure is that the slow light is…
Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases consisting of either matter or anti-matter systems. We review both the…
Sulfur difluoride radicals in their ground state have been produced by a "laser-free" pulsed dc discharge of the SF$_{6}$/Ar gas mixtures in a supersonic molecular beam and detected by mass-selective resonance-enhanced multilphoton…
We show that the dipole-dipole interaction between two Rydberg atoms can give rise to long range molecules. The binding potential arises from two states that converge to different separated atom asymptotes. These states interact weakly at…
We propose an implementation of a universal quantum gate between pairs of spatially separated atoms in a microwave cavity at finite temperature. The gate results from reversible laser excitation of Rydberg states of atoms interacting with…