Related papers: Delocalization of nonlinear optical responses in p…
We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…
Plasmonics aims to interface photonics and electronics. Finding optical, near-field analogues of much used electro-technical components is crucial to the success of such a platform. Here we present the plasmonic analogue of a non-reciprocal…
We demonstrate third harmonic generation in plasmonic antennas made of highly doped germanium and designed to be resonant in the mid infrared. Owing to the near-field enhancement, the result is an ultrafast, sub-diffraction, coherent light…
In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…
Highly nonlinear optical processes, such as multiphoton photoemission, require high intensities, typically achieved with ultrashort laser pulses and, hence, were first observed with the advent of picosecond laser technology. An alternative…
We report that femtosecond surface plasmon polariton pulses can propagate along a metal-dielectric waveguide and that they can be modulated on the femtosecond timescale by direct ultrafast optical excitation of the metal, thereby offering…
Plasmonic nanoantennas have been recently proposed to boost nonlinear optical processes. In a metal dipole nanoantenna with a dielectric nanoparticle placed in the gap, the linear field enhancement can be exploited to enhance third harmonic…
The nonlinear magneto-plasmonics aims to utilize plasmonic excitations to control the mechanisms and taylor the efficiencies of the non-linear light frequency conversion at the nanoscale. We investigate the mechanisms of magnetic second…
We demonstrate that both linear and nonlinear Fano resonances can be realized on two dimensional magnetic metamaterials. The Fano resonance comes from the interference between localized magnetic plasmon resonance and propagating surface…
We demonstrate effective background-free continuous wave nonlinear optical excitation of molecules that are sandwiched between asymmetrically constructed plasmonic gold nanoparticle clusters. We observe that near infrared photons are…
We measure nonlinear optical scattering from individual Au nanorods excited by ultrafast laser pulses on resonance with their longitudinal plasmon mode. Isolating single rods removes inhomogeneous broadening and allows the measurement of a…
Nonlinear photoluminescence (N-PL) is a broadband photon emission arising from non-equilibrium electron distribution generated at the surface of metallic nanostructures by an ultrafast pulsed laser illumination. N-PL is sensitive to surface…
We employ nonlinear autocorrelation measurements to investigate plasmon-assisted hot carrier dynamics generated in optical gold antennas. We demonstrate that surface plasmons enable a nonlinear formation of hot carriers, providing thus a…
Plasmonic waveguides provide an integrated platform to develop efficient nanoscale ultrafast photonic devices. Theoretical models that describe nonlinear optical phenomena in plasmonic waveguides, usually, only incorporate bulk…
Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a…
Nonlinear electron emission processes induced by surface plasmon oscillations have been studied both experimentally and theoretically. The measured above-threshold electron spectra extend up to energies whose appearance cannot be explained…
The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…
The deployment of plasmonic nanostructures to enhance nonlinear signal generation requires effective far-to-near field coupling and phase matching for frequency conversion. While the latter can be easily achieved at plasmonic hotspots, the…
Optical field localization at plasmonic tip-sample nanojunctions has enabled high spatial resolution chemical analysis through tip-enhanced linear optical spectroscopies, including Raman scattering and photoluminescence. Here, we illustrate…
Nonlinear nanophotonics is a rapidly developing field with many useful applications for a design of nonlinear nanoantennas, light sources, nanolasers, sensors, and ultrafast miniature metadevices. A tight confinement of the local…