Related papers: Controlling ultrafast currents by the non-linear p…
We show that with the help of spin-orbit coupling, nonlinear light-matter interactions can efficiently couple with spin and valley degrees of freedom. This revealed spin photogalvanic effect can generate the long-time pursued intrinsic pure…
We theoretically study the interaction of an ultrafast intense linearly polarized optical pulse with monolayers of transition metal dichalcogenides (TMDCs). Such a strong pulse redistributes electrons between the bands and generates…
Owning to their high controllability, laser pulses have contributed greatly to our understanding of strongly correlated electron systems. However, typical multicycle pulses do not control the symmetry of systems that plays an important role…
The pronounced dependence of the nonlinear parameters of both dielectric and semiconductor materials on the wavelength, and the nonlinear interaction between the ultra-short laser pulse and the material requires precise control of the…
We study the photogalvanic effect caused by a simultaneous action of circular-polarized interband and linearly-polarized intraband illuminations. It is found that, in such conditions, the steady photocurrent appears. The effect originates…
Ultrafast nonlinear photonics enables a host of applications in advanced on-chip spectroscopy and information processing. These rely on a strong intensity dependent (nonlinear) refractive index capable of modulating optical pulses on…
We present ultrafast optical switching experiments on 3D photonic band gap crystals. Switching the Si inverse opal is achieved by optically exciting free carriers by a two-photon process. We probe reflectivity in the frequency range of…
Non-adiabatic photo-ionization is difficult to control as it relies on the derivatives of the envelope and not on phase-details of the short ionizing pulse. Here, we introduce a catalyzing state, whose presence render non-adiabatic…
All-optical switching in a ferromagnetic spin valve is studied here using atomistic spin drift-diffusion dynamics, which includes contributions from spin pumping and superdiffusive transport. We find the switching is governed principally by…
Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…
Photoinduced non-thermal phase transitions are new paradigms of exotic non-equilibrium physics of strongly correlated materials. An ultrashort optical pulse can drive the system to a new order through complex microscopic interactions that…
Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…
We develop a microscopic theory of an unconventional photogalvanic effect in two-dimensional materials with the Dirac energy spectrum of the carriers of charge under strong driving. As a test bed, we consider a layer of a transition metal…
The photogalvanic effect is the generation of a second-order direct current by illumination of a non-centrosymmetric material. In this work, we develop a first-principles real-time density matrix (FPDMD) formalism enabling the calculations…
Contemporary quantum plasmonics capture subtle corrections to the properties of plasmonic nano-objects in equilibrium. Here, we demonstrate nonequilibrium spill-out redistribution of the electronic density at the ultrafast time scale. As…
Time-dependent nonlinear media, such as rapidly generated plasmas produced via laser ionization of gases, can increase the energy of individual laser photons and generate tunable high-order harmonic pulses. This phenomenon, known as photon…
Two-dimensional (2D) ferroelectric materials like NbOI$_{2}$ have garnered significant interest, yet their temporal response and synergetic interaction with light remain underexplored. Previous studies on the polarization of oxide…
Superradiant lasers, which consist of incoherently driven atoms coupled to a lossy cavity, are a promising source of coherent light due to their stable frequency and superior narrow linewidth. We show that when a fraction of the atoms is…
We investigate the nonlinear Compton photon source for upcoming laser-particle experiments in the collision scenario of high-energy electron beams and relativistic laser pulses. The stronger laser field could not only improve the scattering…
We show that the sign of the circular photogalvanic effect can be changed by tuning the radiation frequency of circularly polarized light. Here resonant inversion of the photogalvanic effect has been observed for direct inter-subband…