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The strong-field control of plasmonic nanosystems opens up new perspectives for nonlinear plasmonic spectroscopy and petahertz electronics. Questions, however, remain regarding the nature of nonlinear light-matter interactions at…

Controlling the flow of electricity in metallic circuits with light is a key goal for future optoelectronics. In this work, we demonstrate all-optical generation and directional control of non-thermal drift photocurrents in a plasmonic gold…

We report on the generation of bulk photocurrents in materials driven by non-resonant bi-chromatic fields that are circularly polarized and co-rotating. The nonlinear photocurrents have a fully controllable directionality and amplitude…

Materials Science · Physics 2021-09-22 Ofer Neufeld , Nicolas Tancogne-Dejean , Umberto De Giovannini , Hannes Hubener , Angel Rubio

The nonlinear shift current, also known as the bulk photovoltaic current generated by linearly polarized light, has long been known to be absent in crystals with inversion symmetry. Here we argue that a non-zero shift current in…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Li-kun Shi , Dong Zhang , Kai Chang , Justin C. W. Song

We develop a theory of circular photogalvanic effect in non-gyrotropic two-dimensional transition metal dichalcogenide monolayers under interband optical transitions. Oblique incidence of circularly-polarized electromagnetic field or normal…

Mesoscale and Nanoscale Physics · Physics 2021-08-18 M. V. Entin , V. M. Kovalev

Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…

Materials Science · Physics 2021-10-07 Alfred Zong , Anshul Kogar , Nuh Gedik

We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate…

Optics · Physics 2009-11-07 S. Abbas Hosseini , Debabrata Goswami

We propose theoretically a method for the control of the frequency of the nonlinear optical response of a model nonlinear medium driven by an electric field and suggest an experimental realization on the basis of isotropic LiF, or NaCl…

Optics · Physics 2013-09-18 L. Chotorlishvili , A. Sukhov , S. Wimberger , J. Berakdar

The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…

Light-field-driven photocurrents represent a powerful tool for generating photocurrents without external bias in light-matter systems that lack inversion symmetry. While these photocurrents are used in electronic applications, such as…

In this work we suggest a phenomenological theory of photogalvanic phenomena in superconducting materials and structures revealing the diode effect. Starting from a generalized London model including the quadratic nonlinearity in the…

Superconductivity · Physics 2024-06-17 S. V. Mironov , A. S. Mel'nikov , A. I. Buzdin

We present a detailed experimental and theoretical study on the relativistic non-dipole effects in strong-field atomic ionisation by near-infrared linearly-polarised few-cycle laser pulses in the intensity range 1014 -1015 W/cm2. We record…

The ability to manipulate ferroelectrics at ultrafast speeds has long been an elusive target for materials research. Coherently exciting the ferroelectric mode with ultrashort optical pulses holds the promise to switch the ferroelectric…

Materials Science · Physics 2017-05-17 Roman Mankowsky , Alexander von Hoegen , Michael Först , Andrea Cavalleri

This paper reviews the field of extreme nonlinear optics in optical fibers, highlighting key phenomena and advancements. It discusses multiple ionization effects caused by femtosecond laser pulses that generate plasma and induce permanent…

Ultrafast lasers are ideal tools to process transparent materials because they spatially confine the deposition of laser energy within the material's bulk via nonlinear photoionization processes. Nonlinear propagation and filamentation were…

Optics · Physics 2021-03-03 Francois Courvoisier

Optical techniques for spatiotemporal control can produce laser pulses with custom amplitude, phase, or polarization structure. In nonlinear optics and plasma physics, the use of structured pulses typically follows a forward design…

We demonstrate a new concept for reconfigurable nanophotonic devices exploiting ultrafast nonlinear control of shaped wavefronts in a multimode nanomaterial consisting of semiconductor nanowires. Femtosecond pulsed laser excitation of the…

Optics · Physics 2014-09-30 Tom Strudley , Roman Bruck , Ben Mills , Otto L. Muskens

Spatiotemporal control over the intensity of a laser pulse has the potential to enable or revolutionize a wide range of laser-based applications that currently suffer from the poor flexibility offered by conventional optics. Specifically,…

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

We report on the observation of terahertz radiation induced edge photogalvanic currents in graphene, which are nonlinear in intensity. The increase of the radiation intensities up to MW/cm$^2$ results in a complex nonlinear intensity…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 S. Candussio , L. E. Golub , S. Bernreuter , T. Jötten , T. Rockinger , K. Watanabe , T. Taniguchi , J. Eroms , D. Weiss , S. D. Ganichev