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Optical molecular clocks promise unparalleled sensitivity to the temporal variation of the electron-to-proton mass ratio and insight into possible new physics beyond the Standard Model. We propose to realize a molecular clock with bosonic…

Atomic Physics · Physics 2018-02-26 Mateusz Borkowski

We develop a method of spectroscopy that uses a weak static magnetic field to enable direct optical excitation of forbidden electric-dipole transitions that are otherwise prohibitively weak. The power of this scheme is demonstrated using…

Atomic Physics · Physics 2009-11-11 A. V. Taichenachev , V. I. Yudin , C. W. Oates , C. W. Hoyt , Z. W. Barber , L. Hollberg

Motivated by the ideas of using cold alkaline earth atoms trapped in an optical lattice for realization of optical atomic clocks, we investigate theoretically the perturbative effects of atom-atom interactions on a clock transition…

Quantum Physics · Physics 2009-11-10 D. E. Chang , Jun Ye , M. D. Lukin

We investigate theoretically the interaction of polar molecules with optical lattices and microwave fields. We demonstrate the existence of frequency windows in the optical domain where the complex internal structure of the molecule does…

Quantum Physics · Physics 2009-11-13 S. Kotochigova , E. Tiesinga

Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…

We consider a narrow magneto-dipole transition in the $^{169}$Tm atom at the wavelength of $1.14\,\mu$m as a candidate for a 2D optical lattice clock. Calculating dynamic polarizabilities of the two clock levels $[\text{Xe}]4f^{13}6s^2…

A novel form of quantum control is proposed by applying twisted-light also known as optical vortex beams to drive ultra-narrow atomic transitions in neutral Ca, Mg, Yb, Sr, Hg and Cd bosonic isotopes. This innovative all-optical…

Atomic Physics · Physics 2025-06-30 T. Zanon-Willette , F. Impens , E. Arimondo , D. Wilkowski , A. V. Taichenachev , V. I. Yudin

It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for…

Chemical Physics · Physics 2009-11-06 P. L. Chapovsky

We study the resonant control of two nonreactive polar molecules in an optical lattice site, focussing on the example of RbCs. Collisional control can be achieved by tuning bound states of the intermolecular dipolar potential, by varying…

Quantum Gases · Physics 2015-06-03 Thomas M. Hanna , Eite Tiesinga , William F. Mitchell , Paul S. Julienne

We present a consistent analysis of linear spectroscopy for arrays of nearest neighbor dipole-coupled two-level molecules that reveals distinct signatures of weak and strong coupling regimes separated for infinite size arrays by a quantum…

Quantum Physics · Physics 2015-06-16 A. A. Kocherzhenko , J. Dawlaty , B. P. Abolins , F. Herrera , D. B. Abraham , K. B. Whaley

Optical control of polyatomic molecules promises new opportunities in precision metrology, fundamental chemistry, quantum information, and many-body science. Contemporary experimental and theoretical efforts have mostly focused on cycling…

Atomic Physics · Physics 2022-12-26 Phelan Yu , Adrian Lopez , William A. Goddard , Nicholas R. Hutzler

Optical lattice clock systems with ultra-cold strontium-88 atoms have been used to demonstrate superradiant lasing and magnetic field-controlled optical transmission. We explain these phenomena theoretically with a rigorous model for…

Quantum Physics · Physics 2021-03-31 Yuan Zhang , Chong Xin Shan , Klaus Mølmer

Two-photon optical transitions combined with long-range dipole-dipole interactions can be used for the coherent manipulation of collective metastable states composed of different atoms. We show that it is possible to induce optical…

Quantum Physics · Physics 2007-05-23 M. D. Lukin , P. R. Hemmer

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

Atomic Physics · Physics 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

The impact of the optical field polarization on the spectrum of magnetically-induced transitions, a class of transitions forbidden at zero magnetic field, is studied with a weak-probe sub-Doppler technique. The high spectral resolution of…

Atomic Physics · Physics 2025-02-19 A. Sargsyan , E. Klinger , A. Amiryan , D. Sarkisyan

We describe a general technique that allows to induce and control strong interaction between spin states of neighboring atoms in an optical lattice. We show that the properties of spin exchange interactions, such as magnitude, sign, and…

Soft Condensed Matter · Physics 2009-11-07 L. -M. Duan , E. Demler , M. D. Lukin

Several extensions to the Standard Model of particle physics, including light dark matter candidates and unification theories, predict deviations from Newton's law of gravitation. For macroscopic distances, the inverse-square law of…

We present a proposal for controlling the conversion of ultracold atoms into molecules by fixing the phase difference between two oscillating magnetic fields. The scheme is based on the use of a magnetic Feshbach resonance with a field…

Quantum Gases · Physics 2015-11-05 J. Plata

Ultracold molecules provide opportunities for exploring quantum matter, chemical dynamics and information processing thanks to their rich interactions, which can be controlled by external fields. Magnetic fields tune interactions through…

The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…

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