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Two of the most striking experimental findings when investigating exciton spectra in cuprous oxide using high-resolution spectroscopy are the observability and the fine structure splitting of $F$ excitons reported by J. Thewes et al. [Phys.…

The observation of giant Rydberg excitons in cuprous oxide $\left(\mathrm{Cu_{2}O}\right)$ up to a principal quantum number of $n=25$ by T.~Kazimierczuk \emph{et al.} [Nature \textbf{514}, 343, (2014)] inevitably raises the question whether…

Materials Science · Physics 2017-12-07 Frank Schweiner , Jan Ertl , Jörg Main , Günter Wunner , Christoph Uihlein

Excitons, i.e. the bound states of an electron and a positively charged hole are the solid state analogue of the hydrogen atom. As such they exhibit a Rydberg series, which in cuprous oxide has been observed up to high principal quantum…

Mesoscale and Nanoscale Physics · Physics 2025-11-18 Jan Ertl , Patric Rommel , Jörg Main

Recent high-resolution absorption spectroscopy on excited excitons in cuprous oxide [Nature (London) 514, 343 (2014)] has revealed significant deviations of their spectrum from that of the ideal hydrogen-like series. Here we show that the…

Excitons, as bound states of electrons and holes, embody the solid state analogue of the hydrogen atom, whose quantum spectrum is explained within a classical framework by the Bohr-Sommerfeld atomic model. In a first hydrogenlike…

Mesoscale and Nanoscale Physics · Physics 2024-04-17 Jan Ertl , Michael Marquardt , Moritz Schumacher , Patric Rommel , Jörg Main , Manfred Bayer

The complex valence band structure of bulk cuprous oxide necessitates going beyond the parabolic approximation to precisely estimate exciton binding energies. The same is true for excitons in cuprous oxide quantum wells, for which many…

Mesoscale and Nanoscale Physics · Physics 2026-03-13 Niklas Scheuler , Jörg Main , Patric Rommel , Frieder Pfeiffer , Stefan Scheel , Pavel A. Belov

When an electron in a semiconductor gets excited to the conduction band the missing electron can be viewed as a positively charged particle, the hole. Due to the Coulomb interaction electrons and holes can form a hydrogen-like bound state…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Jan Ertl , Sebastian Rentschler , Jörg Main

Highly-excited states of excitons in cuprous oxide have recently been observed at a record quantum number of up to $n=25$. Here, we evaluate the long-range interactions between pairs of Rydberg excitons in Cu$_2$O, which are due to direct…

Quantum Gases · Physics 2018-10-17 Valentin Walther , Sjard Ole Krüger , Stefan Scheel , Thomas Pohl

The various decay mechanisms of excitons in cuprous oxide (Cu2O) are highly sensitive to defects which can relax selection rules. Here we report cryogenic hyperspectral imaging of exciton luminescence from cuprous oxide crystals grown via…

High-lying Rydberg states of Mott-Wannier excitons are receiving considerable interest due to the possibility of adding long-range interactions to the physics of exciton-polaritons. Here, we study Rydberg excitation in bulk synthetic…

Highly excited atoms with an electron moved into a level with large principal quantum number are fascinating hydrogen-like objects. The giant extension of these Rydberg atoms leads to huge interaction effects. Monitoring these interactions…

Mesoscale and Nanoscale Physics · Physics 2014-11-13 Tomasz Kazimierczuk , Dietmar Fröhlich , Stefan Scheel , Heinrich Stolz , Manfred Bayer

We study the absorption spectra of the yellow excitons in Cu$_2$O in high magnetic fields using polarization-resolved optical absorption measurements with a high frequency resolution. We show that the symmetry of the yellow exciton results…

The seminal work by T. Kazimierczuk et al. [Nature 514, 343 (2014)] has shown the existence of highly excited exciton states in a regime, where the correspondence principle is applicable and quantum mechanics turns into classical mechanics,…

Mesoscale and Nanoscale Physics · Physics 2022-08-05 Jan Ertl , Michael Marquardt , Moritz Schumacher , Patric Rommel , Jörg Main , Manfred Bayer

Experimental and theoretical investigations of excitons in cuprous oxide have revealed a significant fine-structure splitting of the excitonic Rydberg states caused by a strong impact of the valence band structure. We provide a…

Mesoscale and Nanoscale Physics · Physics 2020-06-23 Jan Ertl , Patric Rommel , Michel Mom , Jörg Main , Manfred Bayer

Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…

Mesoscale and Nanoscale Physics · Physics 2025-11-03 Julian Heckötter , David Janas , Marc Aßmann , Manfred Bayer

We have used high resolution transmission spectroscopy to study the exciton level spectrum in Cu$_2$O subject to a longitudinal external electric field, i.e., in the geometry where the transmitted light is propagating along the field…

Materials Science · Physics 2017-02-01 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , M. A. Semina , M. M. Glazov

The complete theoretical description of experimentally observed magnetoexcitons in cuprous oxide has been achieved by F. Schweiner et al [Phys. Rev. B 95, 035202 (2017)], using a complete basis set and taking into account the valence band…

Materials Science · Physics 2020-02-10 Patrik Zielinski , Patric Rommel , Frank Schweiner , Jörg Main

Hubbard excitons are bound states of doublons and holes that can be experimentally probed both in real materials, such as cuprates, and in cold atom quantum simulators. Here we compare properties of a Hubbard exciton to those of a pair of…

Strongly Correlated Electrons · Physics 2024-06-25 Annabelle Bohrdt , Eugene Demler , Fabian Grusdt

We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…

Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…

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