Related papers: How quantum are classical spin ices?
We present an experimental determination of the isothermal magnetic susceptibility of the spin ice materials Dy2Ti2O7 and Ho2Ti2O7 in the temperature range 1.8-300 K. The use of spherical crystals has allowed the accurate correction for…
Recent experiments on the spin-ice material Dy2Ti2O7 suggest that the Pauling "ice entropy", characteristic of its classical Coulombic spin-liquid state, may be lost at low temperatures [D. Pomaranski et al., Nature Phys. 9, 353 (2013)].…
We report the low temperature magnetic properties of the pyrochlore Pr$_2$Hf$_2$O$_7$. Polycrystalline and single-crystal samples are investigated using time-of-flight neutron spectroscopy and macroscopic measurements, respectively. The…
We report the magnetic and thermal properties of Dy2Sn2-xSbxO7+x/2, x = 0, 0.25, and 0.5, and Dy2NbScO7. We find evidence for Ising-like single ion ground states in the Dy2Sn2-xSbxO7+x/2 materials. These materials possess nearly the same…
Magnetic pyrochlores with non-Kramers rare-earth ions provide a platform for exploring emergent gauge physics and quantum spin-ice behavior, yet the influence of structural disorder on their ground states remains insufficiently understood.…
The magnetically frustrated spin ice family of materials is host to numerous exotic phenomena such as magnetic monopole excitations and macroscopic residual entropy extending to low temperature. A finite-temperature ordering transition in…
We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…
We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…
We present a detailed theoretical overview of the thermodynamic properties of the dipolar spin ice model, which has been shown to be an excellent quantitative descriptor of the Ising pyrochlore materials Dy_2Ti_2O_7 and Ho_2Ti_2O_7. We show…
Insulating magnetic rare-earth pyrochlores related to spin ice host emergent bosonic monopolar spinons, which obey a magnetic analogue of quantum electrodynamics and may open a route to a magnetic analogue of electronics. However, the…
From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…
Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…
The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…
We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…
Recent experiments suggest that the Ising pyrochlore magnets ${\rm Ho_{2}Ti_{2}O_{7}}$ and ${\rm Dy_{2}Ti_{2}O_{7}}$ display qualitative properties of the ferromagnetic nearest neighbor spin ice model proposed by Harris {\it et al.}, Phys.…
Recent experiments on Ce$_2$Zr$_2$O$_7$ suggest that this material may host a novel form of quantum spin ice, a three-dimensional quantum spin liquid with an emergent photon. The Ce$^{3+}$ local moments on the pyrochlore lattice are…
In their recent communication (Phys. Rev. B 64, 060406(R) (2001)) Cornelius and Gardner have reported the results of magnetization and susceptibility studies on single crystals of the pyrochlore Ho2Ti2O7. The observed field dependence of…
Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…
Recently it has been suggested that long range magnetic dipolar interactions are responsible for spin ice behavior in the Ising pyrochlore magnets ${\rm Dy_{2}Ti_{2}O_{7}}$ and ${\rm Ho_{2}Ti_{2}O_{7}}$. We report here numerical results on…
Despite a well-ordered pyrochlore crystal structure and strong magnetic interactions between the Dy$^{3+}$ or Ho$^{3+}$ ions, no long range magnetic order has been detected in the pyrochlore titanates Ho$_2$Ti$_2$O$_7$ and…