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We consider two sequential models of deposition and aggregation for particles. The first model (No Diffusion) simulates surface diffusion through a deterministic capture area, while the second (Sequential Diffusion) allows the atoms to…

Materials Science · Physics 2007-05-23 Daniele Vilone , Claudio Castellano , Paolo Politi

In the electrochemical deposition of thin films the measurement of the current-time curve does not allow for a direct determination of the nucleus growth law, electrode surface coverage and mean film thickness. In this work we present a…

Soft Condensed Matter · Physics 2018-03-07 S. Politi , M. Tomellini

Growth of atomic indium chains - 1D islands - on the Si(100)-2x1 surface was observed by scanning tunneling microscopy (STM) at room temperature and simulated by means of a kinetic Monte Carlo method. Density of indium islands and island…

Materials Science · Physics 2015-05-13 Jakub Javorský , Martin Setvín , Ivan Ošt'ádal , Pavel Sobotík , Miroslav Kotrla

Point island models (PIMs) are presented for the formation of supported nanoclusters (or islands) during deposition on flat crystalline substrates at lower submonolayer coverages. These models treat islands as occupying a single adsorption…

Mesoscale and Nanoscale Physics · Physics 2016-07-07 Y. Han , E. Gaudry , T. J. Oliveira , J. W. Evans

Nucleation on top of two-dimensional islands with step edge barriers is investigated using scaling arguments. The nucleation rate is expressed in terms of three basic time scales: The time interval between deposition events, the residence…

Materials Science · Physics 2009-10-31 Joachim Krug

We investigate the influence of intermixing on heteroepitaxial growth dynamics, using a two-dimensional point island model, expected to be a good approximation in the early stages of epitaxy. In this model, which we explore both…

Statistical Mechanics · Physics 2015-06-22 K. I. Mazzitello , L. M. Delgado , J. L. Iguain

If a stochastic system during some periods of its evolution can be divided into non-interacting parts, the kinetics of each part can be simulated independently. We show that this can be used in the development of efficient Monte Carlo…

Materials Science · Physics 2009-11-13 V. I. Tokar , H. Dreyssé

We discuss effects of the different chemical bondings on the island morphology and on the island density scaling in two-component submonolayer growth. Different regimes depending on the strength of the mutual interactions and on the…

Materials Science · Physics 2007-05-23 Miroslav Kotrla , Joachim Krug

The effects of cluster diffusion on the submonolayer island density and island-size distribution are studied for the case of irreversible growth of compact islands on a 2D substrate. In our model, we assume instantaneous coalescence of…

Materials Science · Physics 2015-05-27 Yevgen A. Kryukov , Jacques G. Amar

The self-diffusion of two-dimensional small Ag islands (containing up to $10$ atoms) on Ag(111) surface has been studied using and self-learning kinetic Monte Carlo [J. Phys.: Condens. Matter 24, 354004 (2012)] simulations. A variety of…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Syed Islamuddin Shah , Giridhar Nandipati , Talat S. Rahman

The rate of second layer nucleation -- the formation of a stable nucleus on top of a two-dimensional island -- determines both the conditions for layer-by-layer growth, and the size of the top terrace of multilayer mounds in…

Materials Science · Physics 2007-05-23 J. Krug , P. Kuhn

This article reviews the basic computational techniques for carrying out multi-scale simulations using statistical methods, with the focus on simulations of epitaxial growth. First, the statistical-physics background behind Monte Carlo…

Materials Science · Physics 2009-04-17 Peter Kratzer

We generalize the level set approach to model epitaxial growth to include thermal detachment of atoms from island edges. This means that islands do not always grow and island dissociation can occur. We make no assumptions about a critical…

Materials Science · Physics 2009-11-07 M. Petersen , C. Ratsch , R. E. Caflisch , A. Zangwill

We investigate the kinetics of submonolayer epitaxial growth which is driven by a fixed flux of monomers onto a substrate. Adatoms diffuse on the surface, leading to irreversible aggregation of islands. We also account for the effective…

Statistical Mechanics · Physics 2009-10-31 P. L. Krapivsky , J. F. F. Mendes , S. Redner

Using kinetic Monte Carlo simulations and a bond-counting ansatz, thermal stability and diffusion of an adatom island on a crystal surface are studied. At low temperatures, the diffusion constant $D$ is found to decrease for a wide range of…

Condensed Matter · Physics 2009-10-31 T. Muller , W. Selke

A model that describes self diffusion, island nucleation and film growth on FCC(001) metal substrates is presented. The parameters of the model are optimized to describe Cu diffusion on Cu(001), by comparing activation energy barriers to a…

Materials Science · Physics 2008-02-03 O. Biham , I. Furman , M. Karimi , G. Vidali , R. Kennett , H. Zeng

We consider the influence of realistic island diffusion rates to homoepitaxial growth on metallic surfaces using a recently developed rate equation model which describes growth in the submonolayer regime with hyperthermal deposition. To…

Materials Science · Physics 2015-06-25 M. O. Jahma , M. Rusanen , A. Karim , I. T. Koponen , T. Ala-Nissila , T. S. Rahman

We develop a theory for nucleation on top of islands in epitaxial growth based on the derivation of lifetimes and rates governing individual microscopic processes. These processes are strongly affected by the additional step edge barrier…

Materials Science · Physics 2009-10-31 S. Heinrichs , J. Rottler , Ph. Maass

The capture numbers entering the rate equations (RE) for submonolayer film growth are determined from extensive kinetic Monte Carlo (KMC) simulations for simple representative growth models yielding point, compact, and fractal island…

Statistical Mechanics · Physics 2012-08-16 Martin Körner , Mario Einax , Philipp Maass

We use visibility graphs as a tool to analyse the results of kinetic Monte Carlo (kMC) simulations of submonolayer deposition in a one-dimensional point island model. We introduce an efficient algorithm for the computation of the visibility…

Mesoscale and Nanoscale Physics · Physics 2019-07-24 Damien Allen , Michael Grinfeld , Paul Mulheran