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Multiferroics, combining ferroelectric and magnetic orders, enable magnetoelectric (ME) coupling for advanced applications. This mini review explores single-phase and composite multiferroics, examining phenomenological, microscopic,…

Mesoscale and Nanoscale Physics · Physics 2025-07-18 Michał Wanic

We study in this paper bond distortion effect on electric polarization in spiral multiferroic magnets based on cluster and chain models. The bond distortion break inversion symmetry and modify the $d$-$p$ hybridization. Consequently, it…

Strongly Correlated Electrons · Physics 2015-06-04 Hong-Bo Chen , Yi Zhou , You-Quan Li

The ferroelectric polarization of triangular-lattice antiferromagnets induced by helical spin-spiral order is not explained by any existing model of magnetic-order-driven ferroelectricity. We resolve this problem by developing a general…

Strongly Correlated Electrons · Physics 2011-10-11 H. J. Xiang , E. J. Kan , Y. Zhang , M. -H. Whangbo , X. G. Gong

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

Materials Science · Physics 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

Materials Science · Physics 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

We present a first-principles scheme for the computation of the magnetoelectric response of magnetic insulators. The method focuses on the lattice-mediated part of the magnetic response to an electric field, which we argue can be expected…

Materials Science · Physics 2009-12-17 Jorge Iniguez

A common scenario of magnetoelectric coupling in multiferroics is the electric polarization induced by spatially modulated spin structures. It is shown in this paper that the same mechanism works in magnetic dielectrics with inhomogeneous…

Materials Science · Physics 2012-11-13 A. P. Pyatakov , G. A. Meshkov , A. K. Zvezdin

We use a group theoretical approach to enumerate the possible couplings between magnetism and ferroelectric polarisation in the parent $Pm\bar{3}m$ perovskite structure. We show that third order magnetoelectric coupling terms must always…

Materials Science · Physics 2018-05-18 Mark S. Senn , Nicholas C. Bristowe

First-principles calculations, in combination with the four-state energy mapping method, are performed to extract the magnetic interaction parameters of multiferroic BiFeO$_3$. Such parameters include the symmetric exchange (SE) couplings…

Materials Science · Physics 2019-03-20 Changsong Xu , Bin Xu , Bertrand Dupé , L. Bellaiche

Using an effective Hamiltonian of mutiferroic BiFeO$_3$ (BFO) as a toy model, we explore the effect of the coefficient, C, characterizing the strength of the spin-current interaction, on physical properties. We observe that for larger C…

Materials Science · Physics 2013-12-17 Satadeep Bhattacharjee , Dovran Rahmedov , Dawei Wang , Laurent Bellaiche

Multiferroic CuFe1-xAlxO2 (x=0.02) exhibits a ferroelectric ordering accompanied by a proper helical magnetic ordering below T=7K under zero magnetic field. By polarized neutron diffraction and pyroelectric measurements, we have revealed a…

Strongly Correlated Electrons · Physics 2008-03-31 T. Nakajima , S. Mitsuda , S. Kanetsuki , K. Tanaka , K. Fujii , N. Terada , M. Soda , M. Matsuura , K. Hirota

A method is developed which allows to determine the first-order and the second-order magnetoelastic coefficients of a magnetic bulk material from the ab-initio calculation of the magnetocrystalline anisotropy energy as function of a…

Materials Science · Physics 2007-05-23 Matej Komelj , Manfred Faehnle

Below its N\'eel temperature, the frustrated magnet CdCr$_2$O$_4$ exhibits an antiferromagnetic spin-spiral ground state. Such states can give rise to a sizable magnetoelectric coupling. In this report, we measure the electric polarization…

Materials Science · Physics 2020-07-15 L. Rossi , D. Brüning , H. Ueda , Y. Skourski , T. Lorenz , B. Bryant

Magnetoelectric properties of a coupled spin-electron model on a doubly decorated square lattice in an external electric field applied along the crystallographic axis [11] are rigorously examined with the help of generalized…

Strongly Correlated Electrons · Physics 2018-12-26 Hana Čenčariková , Jozef Strečka

Evidence for a strong spin-lattice coupling in multiferroic HoMnO_3 is derived from thermal expansion measurements along a- and c-axis. The magnetoelastic effect results in sizable anomalies of the thermal expansivities at the…

Strongly Correlated Electrons · Physics 2009-11-11 C. dela Cruz , F. Yen , B. Lorenz , Y. Q. Wang , Y. Y. Sun , M. M. Gospodinov , C. W. Chu

Multiferroism can originate from the breaking of inversion symmetry caused by magnetic-spiral order. The usual mechanism for stabilizing a magnetic spiral is competition between magnetic exchange interactions differing by their range and…

The electronic contribution to the magnetically induced polarization in orthorhombic TbMnO3 is studied from first principles. We compare the cases in which the spin cycloid, which induces the electric polarization via the spin-orbit…

Materials Science · Physics 2009-12-16 Andrei Malashevich , David Vanderbilt

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

Multiferroics are those materials with more than one ferroic order, and magnetoelectricity refers to the mutual coupling between magnetism and electricity. The discipline of multiferroicity has never been so highly active as that in the…

Materials Science · Physics 2016-01-19 Shuai Dong , Jun-Ming Liu , Sang-Wook Cheong , Zhifeng Ren

Magnetoelectric multiferroics promise direct cross-control between coexisting ferroelectric and ferromagnetic orders, which is of interest for applications in magnetism and spintronics. A particularly interesting type of cross-control is…