English
Related papers

Related papers: Imaging an aligned polyatomic molecule with laser-…

200 papers

An emission tomography of laser-induced plasmas employed in the laser induced breakdown spectroscopy (LIBS) requires long signal integration times during which the plasma cannot be considered stationary. To reduce the integration time, it…

Plasma Physics · Physics 2010-08-04 Sergei V. Shabanov , Igor B. Gornushkin

In both light optics and electron optics, the amplitude of a wave scattered by an object is an observable that is usually recorded in the form of an intensity distribution in a real space image or a diffraction image. In contrast, retrieval…

Large polyatomic molecules typically exhibit low ionization potentials, Ip, leading to over-the-barrier ionization (OBI) already at relatively low intensities (~1013 W/cm2). We revisit laser-induced electron diffraction (LIED) in the…

Atomic Physics · Physics 2024-11-07 B. Belsa , K. M. Ziems , A. Sanchez , K. Chirvi , X. Liu , S. Grfe , J. Biegert

Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural phenomena such as light-induced phase transitions and chemical reactions. Whereas static electron densities in single molecules can be…

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

Refraction of an optical probe beam by a plasma can be measured with angular filter refractometry (AFR), which produces an image containing intensity contours that correspond to curves of constant refraction angle. Further analysis is…

We propose a scheme for ultrafast real-time imaging of laser-induced collective electron oscillations (Mie plasmons) in gas phase metal clusters by interferometrically stable scanning of two intense few-cycle optical laser pulses. The…

Atomic Physics · Physics 2017-09-13 Jörg Köhn , Thomas Fennel

This paper presents a new technique of optical beam-induced scattering of mid-IR-laser radiation, which is a special mode of the recently developed scanning mid-IR-laser microscopy. The technique in its present form is designed for…

Materials Science · Physics 2015-03-19 O. V. Astafiev , V. P. Kalinushkin , V. A. Yuryev

The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…

A barrier to realizing the potential of molecules for quantum information science applications is a lack of high-fidelity, single-molecule imaging techniques. Here, we present and theoretically analyze a general scheme for dispersive…

Measurements on the strong-field ionization of carbonyl sulfide molecules by short, intense, 2~\um wavelength laser pulses are presented from experiments where angle-resolved photoelectron distributions were recorded with a high-energy…

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in…

Atomic Physics · Physics 2008-11-18 Christian Buth , Robin Santra

It is proposed to use apertures with large acceptance angles to reduce the integration time when studying the emissivity of laser induced plasmas by means of the Abel inversion method. The spatial resolution lost due to contributions of…

Plasma Physics · Physics 2010-08-02 Sergei Shabanov , Igor Gornushkin

We show that the refractive index modification photoinduced in a biased nonlinear photorefractive crystal can be accurately measured and controlled by means of a background incoherent illumination and an external electric field. The…

We studied the photoelectron spectra generated by an intense few-cycle infrared laser pulse. By focusing on the angular distributions of the back rescattered high energy photoelectrons, we show that accurate differential elastic scattering…

Atomic Physics · Physics 2008-04-04 T Morishita , A. T. Le , Z. Chen , C. D. Lin

Based on the frequency-domain theory, we put forward a method of imaging the complex symmetrical polyatomic molecules by using IR+XUV two-color laser fields. Although the wave function of a polyatomic molecule, such as SF6, is quite complex…

Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…

Materials Science · Physics 2021-10-07 Alfred Zong , Anshul Kogar , Nuh Gedik

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

Photoelectron Angular Distributions (PADs) resulting from 800 nm and 1300 nm strong field ionization of impulsively aligned CF$_3$I molecules were analyzed using time-dependent density functional theory (TDDFT). The normalized difference…