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Harmonic calculations based on density-functional theory are generally the method of choice for the description of phonon spectra of metals and insulators. The inclusion of anharmonic effects is, however, delicate as it relies on…

Materials Science · Physics 2015-06-17 Ion Errea , Matteo Calandra , Francesco Mauri

The overall solid-to-solid phase transformation kinetics under non-isothermal conditions has been modeled by means of a differential equation method. The method requires provisions for expressions of the fraction of the transformed phase in…

Materials Science · Physics 2015-05-13 Ali R. Massih , Lars O. Jernkvist

Metals which can form intermetallic compounds by an exothermic reaction constitute a class of reactive materials with multiple applications. Ni-Al laminates of thin alternating layers are being considered as model nanometric metallic…

Materials Science · Physics 2015-06-17 Luis Sandoval , Geoffrey H. Campbell , Jaime Marian

We demonstrate an efficient and accurate, general-purpose first-principles blueprint for calculating anharmonic vibrational free energy and predicting structural phase transition temperatures of solids. Thermodynamic integration is…

Materials Science · Physics 2024-03-14 Junsoo Park , Zhigang Wu , John W. Lawson

We present a new technique which allows the fully {\em ab initio} calculation of the chemical potential of a substitutional impurity in a high-temperature crystal, including harmonic and anharmonic lattice vibrations. The technique uses the…

Materials Science · Physics 2015-06-24 D. Alfe` , G. D. Price , M. J. Gillan

While the vibrational thermodynamics of materials with small anharmonicity at low temperatures has been understood well based on the harmonic phonons approximation; at high temperatures, this understanding must accommodate how phonons…

Materials Science · Physics 2015-10-20 Tian Lan

A first-principles approach to the construction of concentration-temperature magnetic phase diagrams of metallic alloys is presented. The method employs self-consistent total energy calculations based on the coherent potential approximation…

Materials Science · Physics 2015-07-29 B. S. Pujari , P. Larson , V. P. Antropov , K. D. Belashchenko

The temperature dependence of the solid-liquid interfacial free energy, {\gamma}, is investigated for Al and Ni at the undercooled temperature regime based on a recently developed persistent-embryo method. The atomistic description of the…

Chemical Physics · Physics 2018-11-06 Yang Sun , Feng Zhang , Huajing Song , Mikhail I. Mendelev , Cai-Zhuang Wang , Kai-Ming Ho

Novel Ni-Co-Mn-Ti all-d-metal Heusler alloys are exciting due to large multicaloric effects combined with enhanced mechanical properties. An optimized heat treatment for a series of these compounds leads to very sharp phase transitions in…

Binary Ni$_{62}$Nb$_{38}$ alloy belongs to the unique class of binary off-eutectic systems, which are able to form a bulk glassy state [L. Xia et al., J. Appl. Phys. 99 (2006) 026103]. In the present work, the ($p$, $T$) phase diagram of…

Materials Science · Physics 2022-11-15 B. N. Galimzyanov , M. A. Doronina , A. V. Mokshin

The thermodynamic stability of germanium tin $\mathrm{Ge_{1-x}Sn_x}$ alloys is investigated across the composition range $0 \le x \le 1$ by applying density functional theory (DFT) together with the cluster expansion formalism (CE). It is…

Materials Science · Physics 2021-03-02 Alfonso Sanchez-Soares , Conor O'Donnell , James C. Greer

The thermoelectric power (TEP) measurements have been carried out to investigate the changes in the electronic structure associated with the intermartensitic and martensitic transitions in Ni$_{2+x}$Mn$_{1-x}$Ga (0 $\le$ x $\le$ 0.19). The…

Materials Science · Physics 2009-11-11 P. A. Bhobe , J. H. Monteiro , J. C. Cascalheira , S. K. Mendiratta , K. R. Priolkar , P. R. Sarode

When exploring new magnetic materials, the effect of alloying plays a crucial role for numerous properties. By altering the alloy composition, it is possible to tailor, e.g., the Curie temperature ($T_\text{C}$). In this work, $T_\text{C}$…

Materials Science · Physics 2024-12-19 Marian Arale Brännvall , Rickard Armiento , Björn Alling

We present a fast and accurate method to calculate vibrational properties for mechanically unstable high temperature phases that suffer from imaginary frequencies at zero temperature. The method is based on standard finite-difference…

Materials Science · Physics 2015-06-03 Nikolas Antolin , Oscar D. Restrepo , Wolfgang Windl

Amorphous metallic foams are prospective materials due to unique combination of their mechanical and energy-absorption properties. In the present work, atomistic dynamics simulations are performed under isobaric conditions with the pressure…

Materials Science · Physics 2020-05-22 Bulat N. Galimzyanov , Anatolii V. Mokshin

We study transient thermal processes in infinite harmonic crystals with complex (polyatomic) lattice. Initially particles have zero displacements and random velocities such that distribution of temperature is spatially uniform. Initial…

Statistical Mechanics · Physics 2019-06-24 Vitaly A. Kuzkin

In this work we study the thermal rectification efficiency, i.e., asymmetric heat flow, of a three-dimensional mass-graded anharmonic lattice of length $N$ and width $W$ by means of nonequilibrium molecular dynamics simulations. The…

Statistical Mechanics · Physics 2021-10-29 M. Romero-Bastida , M. Lindero-Hernández

The structural, electronic, mechanical and thermal properties of Ir$_{1-x}$Rh$_{x}$ alloys were studied systematically using ab initio density functional theory at different concentrations (x = 0.00, 0.25, 0.50, 0.75, 1.00). A Special…

Materials Science · Physics 2015-06-15 S. Ahmed , M. Zafar , M. Shakil , M. A. Choudhary

High-entropy alloys (HEAs) are a new class of materials constructed from multiple principal elements statistically arranged on simple crystallographic lattices. Due to the large amount of disorder present, they are excellent model systems…

Superconductivity · Physics 2018-03-28 Fabian O. von Rohr , Robert J. Cava

By means of molecular-dynamics simulations, temperature driven diffusionless structural phase transitions in equi- and nearly equiatomic ordered nickel-titanium alloys were investigated. For this purpose, a model potential from the…

Materials Science · Physics 2022-01-04 Daniel Mutter , Peter Nielaba