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Reduced density-matrix functional theory (RDMFT) is a promising alternative approach to the problem of electron correlation. Like standard density functional theory, it contains an unknown exchange-correlation functional, for which several…

Chemical Physics · Physics 2017-03-03 N. N. Lathiotakis , Miguel A. L. Marques

Based on our derivation of finite temperature reduced density matrix functional theory and the discussion of the performance of its first-order functional this work presents several different correlation-energy functionals and applies them…

Other Condensed Matter · Physics 2012-08-24 Tim Baldsiefen , E. K. U. Gross

Density matrix embedding theory (DMET) formally requires the matching of density matrix blocks obtained from high-level and low-level theories, but this is sometimes not achievable in practical calculations. In such a case, the global band…

Computational Physics · Physics 2022-01-14 Fabian M. Faulstich , Raehyun Kim , Zhi-Hao Cui , Zaiwen Wen , Garnet Kin-Lic Chan , Lin Lin

Typical density functional theory (DFT) and approximations thereto solve the many-electron ground state problem by working from a numerically efficient non-interacting Kohn-Sham reference system; and benefit from useful minimization…

Chemical Physics · Physics 2025-04-02 Tim Gould

Common density-matrix functionals, the M\"uller and the power functional, have been benchmarked for the half-filled Hubbard dimer, which allows to model the bond dissociation problem and the transition from the weakly to the strongly…

Strongly Correlated Electrons · Physics 2016-03-09 Ebad Kamil , Robert Schade , Thomas Pruschke , Peter E. Blöchl

The distribution of noncollinear magnetism in an electronic system provides information about the kinetic energy as well as some kinetic energy densities. Two different everywhere-positive kinetic densities related to the…

Chemical Physics · Physics 2018-03-14 Erik I. Tellgren

The reduced dynamics formalism has recently emerged as a powerful tool to study the dynamics of non-equilibrium quantum impurity models in strongly correlated regimes. Examples include the non-equilibrium Anderson impurity model near the…

Mesoscale and Nanoscale Physics · Physics 2013-07-10 Guy Cohen , Eli Y. Wilner , Eran Rabani

The de-facto standard approach of promoting sparsity by means of $\ell_1$-regularization becomes ineffective in the presence of simplex constraints, i.e.,~the target is known to have non-negative entries summing up to a given constant. The…

Methodology · Statistics 2016-05-04 Ping Li , Syama Sundar Rangapuram , Martin Slawski

We introduce a generalization (gLDA) of the traditional Local Density Approximation (LDA) within density functional theory. The gLDA uses both the one-electron Seitz radius $\rs$ and a two-electron hole curvature parameter $\eta$ at each…

Chemical Physics · Physics 2015-06-18 Pierre-François Loos , Caleb J. Ball , Peter M. W. Gill

We study Density Functional Theory models for systems which are translationally invariant in some directions, such as a homogeneous 2-d slab in the 3-d space. We show how the different terms of the energy are modified and we derive reduced…

Mathematical Physics · Physics 2021-12-24 David Gontier , Salma Lahbabi , Abdallah Maichine

The effects of short-range correlations derived from a realistic meson-exchange potential on the single-particle density matrix in finite nuclei are investigated by analyzing the one-body density in terms of the natural orbits. Basic…

Nuclear Theory · Physics 2016-09-08 A. Polls , H. Müther , W. H. Dickhoff

We develop an energy density matrix that parallels the one-body reduced density matrix (1RDM) for many-body quantum systems. Just as the density matrix gives access to the number density and occupation numbers, the energy density matrix…

Strongly Correlated Electrons · Physics 2015-06-22 Jaron T. Krogel , Jeongnim Kim , Fernando A. Reboredo

It is virtually impossible to directly solve the Schr\"odinger equation for a many-electron wave function due to the exponential growth in degrees of freedom with increasing particle number. The two-body reduced density matrix (2-RDM)…

Quantum Physics · Physics 2022-04-22 Nicholas Cox

Density functional theory (DFT) has greatly expanded our ability to affordably compute and understand electronic ground states, by replacing intractable {\em ab initio} calculations by models based on paradigmatic physics from high- and…

Chemical Physics · Physics 2023-03-29 Tim Gould , Derk P. Kooi , Paola Gori-Giorgi , Stefano Pittalis

We analyze the properties of entangled random pure states of a quantum system partitioned into two smaller subsystems of dimensions $N$ and $M$. Framing the problem in terms of random matrices with a fixed-trace constraint, we establish,…

Statistical Mechanics · Physics 2016-05-11 Pierpaolo Vivo , Mauricio P. Pato , Gleb Oshanin

In this work we investigate the computational complexity of the pure consistency of local density matrices (PureCLDM) and pure N-representability (Pure-N-Representability; analog of PureCLDM for bosonic or fermionic systems) problems. In…

Quantum Physics · Physics 2025-04-09 Jonas Kamminga , Dorian Rudolph

The second-order reduced density matrix method (the RDM method) has performed well in determining energies and properties of atomic and molecular systems, achieving coupled-cluster singles and doubles with perturbative triples (CC SD(T))…

Strongly Correlated Electrons · Physics 2012-07-23 James S. M. Anderson , Maho Nakata , Ryo Igarashi , Katsuki Fujisawa , Makoto Yamashita

$N$-body non efimovian bound or quasi-bound states for particles with short range interactions are considered in arbitrary dimensions. The different resonance regimes near the threshold are depicted by using a generalization of the…

Quantum Gases · Physics 2024-10-09 Ludovic Pricoupenko

In the fields of quantum mechanics and quantum information science, the traces of reduced density matrix powers play a crucial role in the study of quantum systems and have numerous important applications. In this paper, we propose a…

Quantum Physics · Physics 2025-07-24 Rui-Qi Zhang , Xiao-Qi Liu , Jing Wang , Ming Li , Shu-Qian Shen , Shao-Ming Fei

The Gaussian unitary random matrix ensembles satisfying some additional symmetry conditions are considered. The effect of these conditions on the limiting normalized counting measures and correlation functions is studied.

Mathematical Physics · Physics 2008-04-24 Vladimir Vasilchuk