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Many-body theory is developed to calculate the $\gamma$-spectra for positron annihilation with valence and core electrons in the noble gas atoms. A proper inclusion of correlation effects and core annihilation provides for an accurate…

Atomic Physics · Physics 2023-03-23 D. G. Green , G. F. Gribakin

Doppler-broadened $\gamma$-ray spectra for positron annihilation on molecules are calculated using many-body theory. By employing Gaussian bases for the electron and positron wavefunctions, a computable expression that involves a…

Atomic Physics · Physics 2025-02-19 S. K. Gregg , J. P. Cassidy , A. R. Swann , J. Hofierka , B. Cunningham , D. G. Green

A many-body theory approach to the calculation of gamma spectra of positron annihilation on many-electron atoms is developed. We evaluate the first-order correlation correction to the annihilation vertex and perform numerical calculations…

Atomic Physics · Physics 2010-02-16 L. J. M. Dunlop , G. F. Gribakin

Diagrammatic many-body theory is used to calculate the scattering phase shifts, normalized annihilation rates $Z_{\rm eff}$ and annihilation gamma spectra for positron collisions with the hydrogen-like ions He$^+$, Li$^{2+}$, B$^{4+}$ and…

Atomic Physics · Physics 2014-04-22 D. G. Green , G. F. Gribakin

Positron scattering and annihilation on noble gas atoms below the positronium formation threshold is studied ab initio using many-body theory methods. The many-body theory provides a near-complete understanding of the…

Atomic Physics · Physics 2014-09-12 D. G. Green , J. A. Ludlow , G. F. Gribakin

Annihilation momentum densities and correlation enhancement factors for low-energy positron annihilation on valence and core electrons of noble-gas atoms are calculated using many-body theory. s, p and d-wave positrons of momenta up to the…

Atomic Physics · Physics 2017-03-22 D. G. Green , G. F. Gribakin

A many-body theory approach is developed for the problem of positron-atom scattering and annihilation. Strong electron-positron correlations are included non-perturbatively through the calculation of the electron-positron vertex function.…

Atomic Physics · Physics 2007-05-23 G. F. Gribakin , J. Ludlow

Calculations of gamma spectra for positron annihilation on a selection of molecules, including methane and its fluoro-substitutes, ethane, propane, butane and benzene are presented. The annihilation gamma spectra characterise the momentum…

Atomic Physics · Physics 2012-04-18 D. G. Green , S. Saha , F. Wang , G. F. Gribakin , C. M. Surko

In this study, a fully self-consistent method was developed to obtain the wave functions of the positron and electrons in molecules simultaneously. The wave function of a positron at room temperature , with a characteristic energy of…

Atomic and Molecular Clusters · Physics 2020-06-24 Lin Tang , Xiaoguang Ma , Jipeng Sui , Meishan Wang , Chuanlu Yang

In the article by Ma~\emph{et al.}~[Phys.~Rev.~A {\bf 94}, 052709 (2016)], $\gamma$-ray spectra for positron annihilation on molecules were calculated in the independent-particle approximation with the positron wavefunction set to unity.…

Atomic Physics · Physics 2017-03-22 D. G. Green , G. F. Gribakin

Understanding the dynamics of positron cooling in gases, including the fraction of positrons surviving to thermalisation, is critical for accurate interpretation of positron lifetime spectra, for the development of efficient positron…

Atomic Physics · Physics 2017-11-22 D. G. Green

The many-body-theory approach to positronium-atom interactions developed in [Phys. Rev. Lett. \textbf{120}, 183402 (2018)] is applied to the sequence of noble-gas atoms He-Xe. The Dyson equation is solved separately for an electron and…

Atomic Physics · Physics 2023-05-24 A. R. Swann , D. G. Green , G. F. Gribakin

The positron-electron annihilation gamma-ray spectra of linear alkanes CnH2n+2 (n=1-12) have been studied systematically. A profile quality (PQ) parameter, is introduced to assess the agreement between the obtained theoretical profiles and…

Chemical Physics · Physics 2014-01-22 X. G. Ma , F. Wang

$\gamma$ spectra for positron annihilation in noble-gas atoms are calculated using many-body theory for positron momenta up to the positronium-formation threshold. This data is used, together with time-evolving positron-momentum…

Atomic Physics · Physics 2017-11-22 D. G. Green

Positrons bind to molecules leading to vibrational excitation and spectacularly enhanced annihilation. Whilst positron binding energies have been measured via resonant annihilation spectra for $\sim$90 molecules in the past two decades, an…

Atomic Physics · Physics 2023-03-23 J. Hofierka , B. Cunningham , C. M. Rawlins , C. H. Patterson , D. G. Green

We present first-principles approaches based on density functional theory for calculating positron states and annihilation characteristics in condensed matter. The treatment of the electron-positron correlation effects (the enhancement of…

Materials Science · Physics 2007-05-23 B. Barbiellini , M. Hakala , R. M. Nieminen , M. J. Puska

Annihilation spectra are presented for aromatic and heterocyclic ring molecules resolved as a function of incident positron energy using a trap-based positron beam. Comparisons with the vibrational mode spectra yield positron-molecule…

This paper studies the gamma-ray spectra of positron annihilation processes in a series of molecules. The results show that the average valence electron energy of the molecules has a linear correlation with the full width at half maximum…

Atomic and Molecular Clusters · Physics 2020-12-02 Fang Yuan , Xiaoguang Ma , Yu Wu , Chuanlu Yang

Measuring the Doppler broadening of the positron annihilation radiation or the angular correlation between the two annihilation gamma quanta reflects the momentum distribution of electrons seen by positrons in the material.Vacancy-type…

Materials Science · Physics 2007-05-23 I. Makkonen , M. Hakala , M. J. Puska

The aim of this work is to identify the mechanisms responsible for very large rates and other peculiarities observed in low-energy positron annihilation on molecules. The two mechanisms considered are: (i) Direct annihilation of the…

Atomic Physics · Physics 2009-10-31 G. F. Gribakin
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