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In this report, a novel methodology based on the static coherent states approach is introduced with the capability of calculating various strong-field laser-induced nonlinearities in full dimensional single-electron molecular systems; an…

Quantum Physics · Physics 2019-10-10 Mohammadreza Eidi , Mohsen Vafaee , Hamed Koochaki Kelardeh , Alexandra Landsman

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

We theoretically investigate high-harmonic generation (HHG) in honeycomb-lattice graphene models when subjected to a DC electric field. By integrating the quantum master equation with the Boltzmann equation, we develop a numerical method to…

Mesoscale and Nanoscale Physics · Physics 2024-07-16 Minoru Kanega , Masahiro Sato

Strong laser light drives complex quantum electron dynamics in solids, which is captured by the high-harmonic generation (HHG) process. Here we report the observation of laser-dressed Floquet-Bloch states (FBSs) at the edge of the Brillouin…

The semiconductor Bloch equations (SBEs) are routinely used for simulations of strong-field laser-matter interactions in condensed matter. In systems without inversion or time-reversal symmetries, the Berry connections and transition dipole…

Atomic Physics · Physics 2020-05-13 Lun Yue , Mette B. Gaarde

We present a theoretical investigation of high-harmonic generation (HHG) from impurity-doped materials using the time-dependent Schr\"odinger equation (TDSE) approach. We demonstrate the factorization of HHG yields as a product of an…

Optics · Physics 2020-08-19 Van-Hung Hoang , Anh-Thu Le

We consider a quantum mechanical model for the high-order harmonic generation in bulk solids. The bandgap is assumed to be considerably larger than the exciting photon energy. Using dipole approximation, the dynamical equations for…

Quantum Physics · Physics 2017-11-09 Viktor Szaszkó-Bogár , Katalin Varjú , Péter Földi

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We propose a novel amplification mechanism for high harmonic generation (HHG) in solids by leveraging bandgap engineering with momentum k-gaps. By constructing a simple diatomic lattice featuring balanced, alternating gain and loss…

Optics · Physics 2025-03-28 Yiming Pan , Danni Chen , Xiaoxi Xu , Zhaopin Chen , Huaiqiang Wang

In frequently studied two-band models for solid-state high-harmonic generation, interband harmonics in principle can range from the minimum to the maximum bandgap. However, it is known that a laser-intensity dependent cutoff exists that may…

Optics · Physics 2024-03-13 Lina Bielke , Hannah Jürß , Vincent Burgtorf , Dieter Bauer

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous…

We propose a novel picture of high-harmonic generation (HHG) in solids based on the concept of temporally changing band structures. To demonstrate the utility of this picture, we focus on the high-order sideband generation (HSG) caused by…

Materials Science · Physics 2019-08-14 Tomohiro Tamaya , Takeo Kato

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

We propose an intuitive method, called time-dependent population imaging (TDPI), to map the dynamical processes of high harmonic generation (HHG) in solids by solving the time-dependent Schr\"{o}dinger equation (TDSE). It is shown that the…

Atomic Physics · Physics 2017-06-28 Xi Liu , Xiaosong Zhu , Pengfei Lan , Xiaofan Zhang , Dian Wang , Qingbin Zhang , Peixiang Lu

We theoretically investigate the spectral caustics of high-order harmonics in solids. We analyze the 1-dimension model of solids HHG and find that, apart from the caustics originated from the van Hove singularities in the energy-band…

Optics · Physics 2021-07-20 Jiaxiang Chen , Qinzhi Xia , Libin Fu

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas

Using real-space view of high harmonic generation (HHG) in solids, we develop a physically transparent and gauge-invariant approach for distinguishing intraband and interband HHG mechanisms. Our approach relies on resolving the harmonic…

Based on high-order harmonic generation (HHG) spectra obtained from solving the time-dependent Schrodinger equation for atoms, we established quantitatively that the HHG yield can be expressed as the product of a returning electron wave…

Atomic Physics · Physics 2008-08-14 Anh-Thu Le , Toru Morishita , C. D. Lin