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Related papers: Interatomic Coulombic Decay in two coupled Quantum…

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A real-space, real-time time-dependent density functional theory (RT-TDDFT) with Ehrenfest dynamics is used to simulate intermolecular Coulombic decay (ICD) processes following the ionization of an inner-valence electron. The approach has…

Chemical Physics · Physics 2025-05-22 Kedong Wang , Cody L. Covington , Kalman Varga

Electronically excited atoms or molecules in an environment are often subject to interatomic/intermolecular Coulombic decay (ICD) and/or electron transfer mediated decay (ETMD) mechanisms. A few of the numerous variables that can impact…

Chemical Physics · Physics 2022-09-15 Ravi Kumar , Dr. Nayana Vaval

Ionization of matter by energetic radiation generally causes complex secondary reactions which are hard to decipher. Using large helium nanodroplets irradiated by XUV photons, we show that the full chain of processes ensuing primary…

Atomic and Molecular Clusters · Physics 2023-07-26 L. Ben Ltaief , K. Sishodia , S. Mandal , S. De , S. R. Krishnan , C. Medina , N. Pal , R. Richter , T. Fennel , M. Mudrich

The recent availability of intense and ultrashort extreme ultraviolet sources opens the possibility to investigate ultrafast electronic relaxation processes in matter in an unprecedented regime. In this work we report on the observation of…

We investigate the interplay dynamics of a cavity qed system, where the two-level atoms are trapped in a double-well potential, and the cavity mode, with a frequency largely detuned to the atomic level splitting, is driven by a probe laser.…

Quantum Physics · Physics 2009-11-13 Jiang-Ming Zhang , Wu-Ming Liu , Duan-Lu Zhou

Systems of quantum dots (QD) connected to leads exhibit periodic conductance peaks as a function of gate voltage arising from the Coulomb blockade effect \cite{review1,review2,review3}. Much effort goes into minimizing the size of QDs and…

Mesoscale and Nanoscale Physics · Physics 2009-07-29 L. Bitton , R. Berkovits , A. Frydman

Light-induced energy confinement in nanoclusters via plasmon excitations influences applications in nanophotonics, photocatalysis, and the design of controlled slow electron sources. The resonant decay of these excitations through the…

Atomic and Molecular Clusters · Physics 2023-06-21 Rasheed Shaik , Hari R. Varma , Mohamed El-Amine Madjet , Fulu Zheng , Thomas Frauenheim , Himadri S. Chakraborty

We calculate Coulomb scattering lifetimes of electrons in two-subband quantum wires and in double-layer quantum wells by obtaining the quasiparticle self-energy within the framework of the random-phase approximation for the dynamical…

Condensed Matter · Physics 2009-10-28 Lian Zheng , S. Das Sarma

Charge-density-wave (CDW) is a modulation of the conduction electron density in a conductor. Under low temperature, it can spontaneously happen in some compounds that consist of anisotropic one-dimensional crystal structures, via a strong…

Mesoscale and Nanoscale Physics · Physics 2012-06-06 Ting-Ting Kang

Irradiation of condensed matter with ionizing radiation generally causes direct photoionization as well as secondary processes that often dominate the ionization dynamics. Here, large helium (He) nanodroplets with radius >40 nm doped with…

Atomic and Molecular Clusters · Physics 2024-12-06 L. Ben Ltaief , K. Sishodia , J. D. Asmussen , A. R. Abid , S. R. Krishnan , H. B. Pedersen , N. Sisourat , M. Mudrich

We found analytical solution for the time evolution of localized electron density in a system of two coupled single-level quantum dots (QDs) connected with continuous spectrum states in the presence of Coulomb interaction. This solution…

Mesoscale and Nanoscale Physics · Physics 2013-12-30 P. I. Arseev , N. S. Maslova , V. N. Mantsevich

We identified interatomic Coulombic decay (ICD) channels in argon dimers after spectator-type resonant Auger decay $2p^{-1}~3d \to 3p^{-2}3d, 4d$ in one of the atoms, using momentum resolved electron-ion-ion coincidence. The results…

Chemical Physics · Physics 2015-06-15 M. Kimura , H. Fukuzawa , K. Sakai , S. Mondal , E. Kukk , Y. Kono , S. Nagaoka , Y. Tamenori , N. Saito , K. Ueda

What is meant by continuum lowering and ionization potential depression (IPD) in a Coulomb system depends upon precisely what question is being asked. It is shown that equilibrium (equation-of-state) phenomena and non-equilibrium dynamical…

Plasma Physics · Physics 2014-11-21 B. J. B. Crowley

Low-energy electrons (LEEs) are known to be effective in causing strand breaks in DNA. Recent experiments show that an important direct source of LEEs is the intermolecular Coulombic decay (ICD) process. Here we propose a new cascade…

Atomic and Molecular Clusters · Physics 2014-02-14 Kirill Gokhberg , Premysl Kolorenc , Alexander I. Kuleff , Lorenz S. Cederbaum

It is shown that the homogeneous state of the spatially separated electrons and holes in the coupled quantum wells (CQW) is instable if the layer charge density is smaller than the critical value specified by the parameters of the CQW. The…

Mesoscale and Nanoscale Physics · Physics 2014-12-22 V. S. Babichenko , I. Ya. Polishchuk , A. I. Pavlov , A. Guseynov , M. I. Gozman

We investigate the ionization of HeNe from below the He 1s3p excitation to the He ionization threshold. We observe HeNe$^+$ ions with an enhancement by more than a factor of 60 when the He side couples resonantly to the radiation field.…

There are several important solid-state systems, such as defects in solids, superconducting circuits and molecular qubits, for attractive candidates of quantum computations. Molecular qubits, which benefit from the power of chemistry for…

Quantum Physics · Physics 2017-06-29 Yingqiu Dai , Zhifu Shi , Yue Fu , Xi Qin , Shiwei Mu , Yang Wu , Ji-Hu Su , Lei Qin , Yuan-Qi Zhai , Yi-Fei Deng , Xing Rong , Jiangfeng Du

We simulate the time-dependent coherent dynamics of a spatially indirect exciton (an electron-hole pair with the two particles confined in different layers) in a GaAs coupled quantum well system. We use a unitary wave-packet propagation…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 Federico Grasselli , Andrea Bertoni , Guido Goldoni

Commercial InGaN/GaN light emitting diode heterostructures continue to suffer from efficiency droop at high current densities. Droop mitigation strategies target Auger recombination and typically require structural and/or compositional…