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Context Mixed-metal clusters have long been studied because of their peculiar properties and how they change with cluster size, composition and charge state and their potential roles in catalysis. The characterization of these clusters is…

Chemical Physics · Physics 2024-04-30 Paulo H. Acioli

We report on the structure and adsorption properties of Pd$_n$ ($n=1-4$) clusters supported on the rutile TiO$_2$ (110) surfaces with the possible presence of a surface oxygen vacancy or a subsurface Ti-interstitial atom. As predicted by…

Materials Science · Physics 2012-04-12 Jin Zhang , Anastassia N. Alexandrova

The dynamical and thermodynamic phase stabilities of the stoichiometric compound CrN including different structural and magnetic configurations are comprehensively investigated using a first-principles density-functional-theory (DFT) plus U…

We consider theories in which a dark sector is described by a Conformal Field Theory (CFT) over a broad range of energy scales. A coupling of the dark sector to the Standard Model breaks conformal invariance. While weak at high energies,…

High Energy Physics - Phenomenology · Physics 2023-04-19 Sungwoo Hong , Gowri Kurup , Maxim Perelstein

Solid-state amorphization of crystalline copper nanolayers embedded in a Cu64Zr36 metallic glass is studied by molecular dynamics simulations for different orientations of the crystalline layer. We show that solid-state amorphization is…

Materials Science · Physics 2015-05-07 Tobias Brink , Daniel Şopu , Karsten Albe

Dispersion corrected density functional theory ($\omega$B97X-D DFT) method is used to study the molecular hydrogen adsorption in $Ni_nMg_m$ $(1\geq n\geq 3,1\geq m\geq9)$ clusters. All these clusters can effectively adsorb multiple $H_2$ in…

Materials Science · Physics 2022-02-28 Bishwajit Boruah , Bulumoni Kalita

Metal clusters are partway between molecular and bulk systems and thus exhibit special physical and chemical properties. Atoms can rearrange within a cluster to form different structural isomers. Internal degrees of freedom and the…

Materials Science · Physics 2019-07-31 Barbara A. J. Lechner , Fabian Knoller , Alexander Bourgund , Ueli Heiz , Friedrich Esch

As a typical immiscible binary system, copper (Cu) and lithium (Li) show no alloying and chemical intermixing under normal circumstances. A notable example that takes advantages of the immiscibility between Cu and Li is the widespread…

Materials Science · Physics 2018-05-22 Muhua Sun , Jiake Wei , Zhi Xu , Qianming Huang , Yu Zhao , Wenlong Wang , Xuedong Bai

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

The nanocrystalline-amorphous textures are commonly observed in the coatings synthesized by energetic deposition.This work reports a theoretical study towards binary Cu-C phase separation.By performing a MD simulation using the LAMMPS…

Materials Science · Physics 2023-07-18 Jiajian Guan , Qin Jiang , Yue He , Xu Zhang , Bin Liao , Wei Gao , Lizhao Qin

We investigate the properties of clusters formed from two connected $\mathrm{Ge_{m}}$ cage-like clusters, such as experimentally synthesized $\mathrm{Au_3Ge_{18}^{5-}}$, using first-principles DFT methods. We focus particularly on…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Danielle McDermott , Kathie E. Newman

Materials with correlated electrons often respond very strongly to external or internal influences, leading to instabilities and states of matter with broken symmetry. This behavior can be studied theoretically either by evaluating the…

Strongly Correlated Electrons · Physics 2017-08-15 J. Kunes , I. Leonov , P. Augustinsky , V. Krapek , M. Kollar , D. Vollhardt

Recent density functional theory (DFT) calculations by Foerst et al. have predicted that vacancies in both low and high carbon steels have a carbon dimer bound to them. This is likely to change the thinking of metallurgists in the kinetics…

Materials Science · Physics 2015-06-15 A. T. Paxton , C. Elsaesser

We use spin-density-functional theory (SDFT) ab initio calculations to theoretically explore the possibility of achieving useful gate control over exchange coupling between cobalt clusters placed on a graphene sheet. By applying an electric…

Materials Science · Physics 2013-04-11 Hua Chen , Qian Niu , Zhenyu Zhang , Allan H. MacDonald

We study the optical properties of small gold chains doped with different transition metal (TM) atoms (Ni,Rh,Fe) by using the time-dependent density-functional theory (TDDFT) approach. The optical absorption spectrum of such systems…

Mesoscale and Nanoscale Physics · Physics 2011-09-06 N. Nayyar , A. Kabir , V. Turkowski , Talat S. Rahman

In order to test the Vibration-Transit (V-T) theory of liquid dynamics, ab initio density functional theory (DFT) calculations of thermodynamic properties of Na and Cu are performed and compared with experimental data. The calculations are…

Multi-center transition metal complexes (MCTMs) with magnetically interacting ions have been proposed as components for information processing devices and storage units. For any practical application of MCTMs as magnetic units, it is…

Chemical Physics · Physics 2023-04-03 Henry C. Fitzhugh , James W. Furness , Mark R. Pederson , Juan E. Peralta , Jianwei Sun

The evolution of cluster structure with size and the critical size for the transition from cluster to nanocrystal have long been fundamental problems in nanoscience. Due to limitations of experimental technology and computational methods,…

Materials Science · Physics 2025-12-25 Hongsheng Liu , Luneng Zhao , Yaning Li , Yuan Chang , Shi Qiu , Xiao Wang , Junfeng Gao , Feng Ding

Density Functional Theory (DFT) calculations, within the virtual crystal alloy approximation, are performed, along with the development of a Landau-type model employing a symmetry-allowed analytical expression of the internal energy and…

The formalism of electronic density-functional-theory, with Hubbard-U corrections (DFT+U), is employed in a computational study of the energetics of U_{1-x} Ce_x O_2 mixtures. The computational approach makes use of a procedure which…

Materials Science · Physics 2012-03-08 B. E. Hanken , C. R. Stanek , N. Grønbech-Jensen , M. Asta
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