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Related papers: Transient reflectance of photoexcited Cd$_3$As$_2$

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Three dimensional (3D) Dirac semimetals which can be seen as 3D analogues of graphene have attracted enormous interests in research recently. In order to apply these ultrahigh-mobility materials in future electronic/optoelectronic devices,…

Mesoscale and Nanoscale Physics · Physics 2017-01-19 Wei Lu , Shaofeng Ge , Xuefeng Liu , Hong Lu , Caizhen Li , Jiawei Lai , Chuan Zhao , Zhimin Liao , Shuang Jia , Dong Sun

The relaxation dynamics of photoexcited quasiparticles of three-dimensional (3D) Dirac semimetals are vital towards their application in high performance electronic and optoelectronic devices. In this work, the relaxation dynamics of…

Optics · Physics 2018-10-03 Wei Lu , Jiwei Ling , Faxian Xiu , Dong Sun

The topological three-dimensional Dirac semimetal Cd3As2 has drawn great attention for the novel physics and promising applications in optoelectronic devices operating in the infrared and THz regimes. Among the extensive studies in the past…

Strongly Correlated Electrons · Physics 2022-06-17 Wenjie Zhang , Yunkun Yang , Peng Suo , Kaiwen Sun , Jun Peng , Xian Lin , Faxian Xiu , Guohong Ma

Topological properties of a three-dimensional Dirac semimetal Cd3As2, protected by crystal rotation and time-reversal symmetry, can be tuned with the application of pressure. Ultrafast spectroscopy is a unique tool to investigate the…

Materials Science · Physics 2025-03-03 Vikas Arora , D. V. S. Muthu , R Sankar , A K Sood

Femtosecond X-ray irradiation of solids excites energetic photoelectrons that thermalize on a timescale of a few hundred femtoseconds. The thermalized electrons exchange energy with the lattice and heat it up. Experiments with X-ray…

Materials Science · Physics 2017-07-07 Beata Ziaja , Nikita Medvedev , Victor Tkachenko , Theophilos Maltezopoulos , Wilfried Wurth

Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

Cadmium arsenide Cd$_3$As$_2$ hosts massless Dirac electrons in its ambient-conditions tetragonal phase. We report X-ray diffraction and electrical resistivity measurements of Cd$_3$As$_2$ upon cycling pressure beyond the critical pressure…

Using transient absorption (TA) microscopy as a hot electron thermometer we show disorder-assisted acoustic-phonon supercollisions (SCs) best describes the rate-limiting relaxation step in graphene over a wide range of lattice temperatures…

Materials Science · Physics 2013-10-25 Matt W. Graham , Su-Fei Shi , Zenghui Wang , Daniel C. Ralph , Jiwoong Park , Paul L. McEuen

Ultrafast time-resolved differential reflectivity of Bi2Se3 crystals is studied using optical pump-probe spectroscopy. Three distinct relaxation processes are found to contribute to the initial transient reflectivity changes. The deduced…

Materials Science · Physics 2010-11-09 J. Qi , X. Chen , W. Yu , P. Cadden-Zimansky , D. Smirnov , N. H. Tolk , I. Miotkowski , H. Cao , Y. P. Chen , Y. Wu , S. Qiao , Z. Jiang

We have used a combination of linear response time-domain THz spectroscopy (TDTS) and high-field non-linear THz spectroscopy to separately probe the electronic momentum and energy relaxation rates respectively of the Dirac semimetal…

Strongly Correlated Electrons · Physics 2024-08-19 Rishi Bhandia , David Barbalas , Run Xiao , Juan R. Chamorro , Tanya Berry , Tyrel M. McQueen , Nitin Samarth , N. P. Armitage

The thermoelectric effects of topological semimetals have attracted tremendous research interest because many topological semimetals are excellent thermoelectric materials and thermoelectricity serves as one of their most important…

Raman scattering in the three-dimensional Dirac semimetal Cd3As2 shows an intricate interplay of electronic and phonon degrees of freedom. We observe resonant phonon scattering due to interband transitions, an anomalous anharmonicity of…

Materials Science · Physics 2017-07-05 A. Sharafeev , V. Gnezdilov , R. Sankar , F. C. Chou , P. Lemmens

We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter…

Materials Science · Physics 2018-05-23 E. Uykur , R. Sankar , D. Schmitz , C. A. Kuntscher

We present femtosecond time-resolved pump-probe spectroscopic studies of a pseudogap (PG) along with the superconducting (SC) gap in an overdoped iron pnictide Ca(Fe0.927Co0.073)2As2. It is seen that the temperature evolution of the…

Superconductivity · Physics 2014-03-12 Sunil Kumar , L. Harnagea , S. Wurmehl , B. Buechner , A. K. Sood

In this paper we report a detailed analysis of the temperature-dependent optical properties of epitaxially grown cadmium arsenide (Cd$_3$As$_2$), a newly discovered three-dimensional Dirac semimetal. Dynamic Fermi level tuning -- instigated…

The efforts to pursue photo detection with extreme performance in terms of ultrafast response time, broad detection wavelength range, and high sensitivity have never been exhausted as driven by its wide range of optoelectronic and photonic…

Mesoscale and Nanoscale Physics · Physics 2017-01-20 Qinsheng Wang , Cai-Zhen Li , Shaofeng Ge , Jin-Guang Li , Wei Lu , Jiawei Lai , Xuefeng Liu , Junchao Ma , Da-Peng Yu , Zhi-Min Liao , Dong Sun

We investigate the ultrafast dynamics of photo-induced non-thermal lattice disorder in a polycrystalline aluminium thin film to elucidate transient short- and long-range lattice distortions, their thermalization and electron-phonon coupling…

Materials Science · Physics 2026-01-06 Fernando Rodriguez Diaz , Kasra Amini

Photoinduced effects in a single crystal of bilayered manganites, La2-2xSr1+2xMn2O7 (x=0.38), were investigated in a wide range of temperatures by pump-probe measurement at a photon energy of 1.6eV. In a ferromagnetic metallic state,…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Hirobe , Y. Kubo , K. Kouyama , H. Kunugita , K. Ema , H. Kuwahara

The temperature dependence of ultrafast photoinduced reflectivity transients is reported in Nd$_{0.5}$Sr$_{0.5}$MnO$_{3}$ thin film. The photoinduced reflectivity shows a complex response with very different temperature dependences on…

Condensed Matter · Physics 2009-11-10 T. Mertelj , D. Mihailovic , Z. Jagličič , A. A. Bosak , O. Yu. Gorbenko , A. R. Kaul

The evolution of charge carriers in photoexcited room temperature ZnO nanoparticles in solution is investigated using ultrafast ultraviolet photoluminescence spectroscopy, ultrafast Zn K-edge absorption spectroscopy and ab-initio molecular…

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