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We studied ion concentration profiles and the charge density gradient caused by electrode reactions in weak electrolytes by using the Poisson--Nernst--Planck equations without assuming charge neutrality. In weak electrolytes, only a small…

Soft Condensed Matter · Physics 2018-02-08 Yohichi Suzuki , Kazuhiko Seki

Conserved-charge densities are very special observables in quantum many-body systems as, by construction, they encode information about the dynamics. Therefore, their evolution is expected to be of much simpler interpretation than that of…

Statistical Mechanics · Physics 2024-05-30 Bruno Bertini , Katja Klobas , Mario Collura , Pasquale Calabrese , Colin Rylands

The charge distribution at the interface between two electrolytes is studied for the case of non-vanishing ion fluxes. The analysis is an extension of the established Verwey-Niessen theory to non-equilibrium situations. Applying matched…

Soft Condensed Matter · Physics 2011-05-03 Steffen Hardt , Tobias Baier

The lattice fluid model of the system with short range and long range Coulomb interactions is suggested. In the framework of the collective variables method, the screening of the Coulomb interactions in the bulk is considered. It is shown…

Other Condensed Matter · Physics 2019-01-24 George Bokun , Dung di Caprio , Myroslav Holovko , Vyacheslav Vikhrenko

The equilibrium density profiles in a classical multicomponent plasma near a hard wall made with a dielectric material characterized by a relative dielectric constant $\ew$ are studied from the first Born-Green-Yvon equation combined with…

Statistical Mechanics · Physics 2007-05-23 Jean-Noel Aqua , Francoise Cornu

In spite of their enormous applications as alternative energy storage devices and lubricants, room temperature ionic liquids (ILs) still pose many challenges from a pure scientific view point. We develop an IL microscopic theory in terms of…

Soft Condensed Matter · Physics 2020-02-05 Yael Avni , Ram M. Adar , David Andelman

We have recently developed the QTPIE (charge transfer with polarization current equilibration) fluctuating-charge model, a new model with correct dissociation behavior for nonequilibrium geometries. The correct asymptotics originally came…

Chemical Physics · Physics 2010-10-13 Jiahao Chen , Todd J Martinez

Ion clustering has been proposed as a mechanism leading to the peculiar 'anomalous underscreening' phenomenon seen for electrostatic interactions between charge surfaces immersed in concentrated electrolytes. These interactions have been…

Soft Condensed Matter · Physics 2025-12-01 Clifford E. Woodward , David Ribar , Jan Forsman

A theoretical analysis of Coulomb systems on lattices in general dimensions is presented. The thermodynamics is developed using Debye-Huckel theory with ion-pairing and dipole-ion solvation, specific calculations being performed for 3D…

Statistical Mechanics · Physics 2009-11-07 Vladimir Kobelev , Anatoly B. Kolomeisky , Michael E. Fisher

We investigate the flow of an electrolyte through a rigid nanochannel decorated with a surface charge pattern. Employing lattice Boltzmann and dissipative particle dynamics methods, as well as analytical theory, we show that the…

Soft Condensed Matter · Physics 2024-01-12 Tine Curk , Sergi G. Leyva , Ignacio Pagonabarraga

We consider an ionic fluid made with two species of mobile particles carrying either a positive or a negative charge. We derive a sum rule for the fourth moment of equilibrium charge correlations. Our method relies on the study of the…

Statistical Mechanics · Physics 2016-11-30 Angel Alastuey , Riccardo Fantoni

A theoretical model of vapor-liquid phase transition in a system of charged hard cores of different diameters is suggested (with the parameters of the transition obtained in a number of studies using the Monte Carlo method). The model is…

Plasma Physics · Physics 2007-05-23 A. L. Khomkin , I. A. Mulenko

We calculate the conductance of atomic chains as a function of their length. Using the Density Matrix Renormalization Group algorithm for a many-body model which takes into account electron-electron interactions and the shape of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Rafael A. Molina , Dietmar Weinmann , Jean-Louis Pichard

We investigate a system of dense polyelectrolytes in solution. The Langevin dynamics of the system with linearized hydrodynamics is formulated in the functional integral formalism and a transformation made to collective coordinates. Within…

Soft Condensed Matter · Physics 2015-06-25 Kristian K. M"uller-Nedebock , Thomas A. Vilgis

Quantum--Mechanical methods that are both computationally fast and accurate are not yet available for electronic excitations having charge transfer character. In this work, we present a significant step forward towards this goal for those…

Chemical Physics · Physics 2015-06-12 Michele Pavanello , Troy Van Voorhis , Lucas Visscher , Johannes Neugebauer

We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

Soft Condensed Matter · Physics 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

We analytically calculate the correlation potential of a test ion near a \emph{strongly} charged plate inside a dilute $m:-n$ electrolyte. We do this by calculating the electrostatic Green's function in the presence of a nonlinear…

Soft Condensed Matter · Physics 2014-03-19 Bing-Sui Lu , Xiangjun Xing

The charge delocalization error, besides nondynamic correlation, has been a major challenge to density functional theory. Contemporary functionals undershoot the dissociation of symmetric charged dimers A2+, a simple but stringent test,…

Chemical Physics · Physics 2021-07-26 Emil Proynov , Jing Kong

We study the renormalization group behaviour of the topological charge density in full QCD on the lattice. We propose a way of extracting the necessary renormalization functions from Monte Carlo simulations.

High Energy Physics - Lattice · Physics 2009-10-28 B. Alles , A. Di Giacomo , H. Panagopoulos , E. Vicari

The collected charge of two pad diodes is measured along the diode width using a 5:2 GeV electron beam at the DESY II beam test facility. The electron beam enters parallel to the readout electrode plane and perpendicular to the edge of the…

Instrumentation and Detectors · Physics 2021-12-16 Mohammadtaghi Hajheidari , Erika Garutti , Joern Schwandt , Aliakbar Ebrahimi