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Ultracold diatomic molecules find application in quantum studies ranging from controlled chemistry and precision measurement physics to quantum many-body simulation and potentially quantum computing. Accurate knowledge of molecular…

Atomic Physics · Physics 2024-05-14 Hela Ladjimi , Michał Tomza

We report calculations of Born-Oppenheimer potential energy curves of the chromium-rubidium heteronuclear molecule 52Cr-87Rb, and the long-range dispersion coefficient for the interaction between ground state Cr and Rb atoms. Our calculated…

Atomic Physics · Physics 2015-05-19 Z. Pavlovic , H. R. Sadeghpour , R. Cote , B. O. Roos

We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination…

Chemical Physics · Physics 2017-09-13 Maxence Lepers , Olivier Dulieu

The random-phase approximation with exchange (RPAE) is used with a $B$-spline basis to compute dynamic dipole polarizabilities of noble-gas atoms and several other closed-shell atoms (Be, Mg, Ca, Zn, Sr, Cd, and Ba). From these, values of…

Atomic Physics · Physics 2015-07-08 A. R. Swann , J. A. Ludlow , G. F. Gribakin

The efficiency of optical trapping of ultracold atoms depend on the atomic dynamic dipole polarizability governing the atom-field interaction. In this article, we have calculated the real and imaginary parts of the dynamic dipole…

Atomic Physics · Physics 2017-04-11 Hui Li , Jean-Francois Wyart , Olivier Dulieu , Sylvain Nascimbene , Maxence Lepers

Following the first principles the analytic Born-Oppenheimer (BO) potential curve for the ground state $X^1\Sigma^+$ of the molecule ClF is proposed for whole range of internuclear distances $R \in [0,\infty)$. It is based on matching the…

Chemical Physics · Physics 2023-09-06 Horacio Olivares Pilon , Alexander V Turbiner

We report a high-resolution spectroscopic investigation of the long-range states of the $^{23}$Na$^{87}$Rb molecule near its Na($3^2S_{1/2}$)+Rb($5^2P_{3/2}$) asymptote. This study was performed with weakly bound ultracold molecules…

The long-range interaction of excited neutral atoms has a number of interesting and surprising properties, such as the prevalence of long-range, oscillatory tails, and the emergence of numerically large can der Waals C_6 coefficients.…

Atomic Physics · Physics 2017-09-25 C. M. Adhikari , V. Debierre , U. D. Jentschura

We consider long-range interactions between two alkali-metal atoms in their respective ground states. We extend the previous relativistic many-body calculations of C_6 dispersion coefficients [Phys.Rev. Lett. {\bf 82}, 3589 (1999)] to…

Atomic Physics · Physics 2009-11-10 Sergey Porsev , Andrei Derevianko

By inferring the dynamic permittivity of different material media from the observations and calculating dynamic electric dipole polarizabilties of the Li through Cs alkali atoms, precise values of $C_3$ coefficients were estimated in Phys.…

Atomic Physics · Physics 2023-10-02 Harpreet Kaur , Vipul Badhan , Bindiya Arora , B. K. Sahoo

We study the van der Waals interaction between Rydberg alkali-metal atoms with fine structure ($n^2L_j$; $L\leq 2$) and heteronuclear alkali-metal dimers in the ground rovibrational state ($X^1\Sigma^+$; $v=0$, $J=0$). We compute the…

Atomic Physics · Physics 2020-04-01 Vanessa Olaya , Jesús Pérez-Ríos , Felipe Herrera

We consider the zero-temperature van der Waals interaction between two molecules, each of which has a zero or near-zero electronic gap between a groundstate and the first excited state, using a toy model molecule ( equilateral H3) as an…

Other Condensed Matter · Physics 2016-12-21 John F. Dobson , Andreas Savin , Janos G. Angyan , Ru-Fen Liu

The interaction of two excited hydrogen atoms in metastable states constitutes a theoretically interesting problem because of the quasi-degenerate 2P_{1/2} levels which are removed from the 2S states only by the Lamb shift. The total…

Atomic Physics · Physics 2017-02-15 U. D. Jentschura , V. Debierre , C. M. Adhikari , A. Matveev , N. Kolachevsky

Mutual Coulomb interactions between electrons lead to a plethora of interesting physical and chemical effects, especially if those interactions involve many fluctuating electrons over large spatial scales. Here, we identify and study in…

The isotropic and anisotropic coefficients $C^{l,m}_n$ of the long-range spherical expansion $\sim 1/R^n$ ($R$ -- the intermolecular distance) of the dispersion and inductions intermolecular energies are calculated using the first…

Chemical Physics · Physics 2023-04-04 Leonid Shirkov , Michał Tomza

General formulas for calculating the several leading long-range interactions among three identical atoms where two atoms are in identical $S$ states and the other atom is in a $P$ state are obtained using perturbation theory for the…

Atomic Physics · Physics 2016-08-16 Pei-Gen Yan , Li-Yan Tang , Zong-Chao Yan , James F. Babb

We consider the long-range states expected for complexes formed from an alkali-metal diatomic molecule in a singlet state and an alkali-metal atom. We explore the structure of the Hamiltonian for such systems, and the couplings between the…

Atomic Physics · Physics 2023-03-13 Matthew D. Frye , Jeremy M. Hutson

The mounting interest in conducting thorough analyses and studies of long-range interactions stems from their wide-ranging applications in cold atomic physics, making it a compelling area for research. In this work, we have evaluated long…

Atomic Physics · Physics 2025-04-23 Harpreet Kaur , Jyoti , Neelam Shukla , Bindiya Arora

Relativistic many-body calculations of van der Waals coefficients C_6 for dimers correlating to two ground state alkaline-earth atoms at large internuclear separations are reported. The following values and uncertainties were determined :…

Atomic Physics · Physics 2009-11-07 Sergey Porsev , Andrei Derevianko

Ultracold collisions between Cs atoms and Cs2 dimers in the electronic ground state are observed in an optically trapped gas of atoms and molecules. The Cs2 molecules are formed in the triplet ground state by cw-photoassociation through the…

Atomic Physics · Physics 2009-11-11 Peter Staanum , Stephan D. Kraft , Joerg Lange , Roland Wester , Matthias Weidemueller