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The multiconfigurational time-dependent Hartree-Fock method (MCTDHF) is applied for simulations of the two-photon ionization of Helium. We present results for the single- and double ionization from the groundstate for photon energies in the…

Atomic Physics · Physics 2011-12-30 D. Hochstuhl , M. Bonitz

As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

Atomic Physics · Physics 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

The process of nonsequential two-photon double ionization of helium is studied by two complementary numerical approaches. First, the time-dependent Schr{\"o}dinger equation is solved and the final wave function is analyzed in terms of…

Quantum Physics · Physics 2010-09-13 Sølve Selstø , Tore Birkeland , Simen Kvaal , Raymond Nepstad , Morten Førre

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

Atomic Physics · Physics 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Double ionization (DI) is a fundamental process that despite its apparent simplicity provides rich opportunities for probing and controlling the electronic motion. Even for the simplest multielectron atom, helium, new DI mechanisms are…

Atomic Physics · Physics 2021-10-12 Henrik R. Larsson , David J. Tannor

The multiphoton ionization of hydrogen atoms in a strong elliptically polarized microwave field exhibits complex features that are not observed for ionization in circular and linear polarized fields. Experimental data reveal high…

Chaotic Dynamics · Physics 2007-05-23 Elena Shchekinova , Cristel Chandre , Turgay Uzer

Attosecond pump-probe ionization process can be used to prepare atomic ions in the coherent superposition of states with opposite parity. The multiphoton shake-up ionization of Helium, in particular, generates ions with same principal…

Atomic Physics · Physics 2019-12-12 Saad Mehmood , Eva Lindroth , Luca Argenti

We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…

Atomic Physics · Physics 2020-03-24 Fengzheng Zhu , Genliang Li , Aihua Liu

We present a fully {\it ab initio}, non-perturbative, time-dependent approach to describe single and double ionization of helium by proton and antiproton impact. A flexible and accurate finite-element discrete-variable-representation is…

Atomic Physics · Physics 2016-11-17 Xiaoxu Guan , Klaus Bartschat

We consider the classical dynamics of a two-electron system subjected to an intense bichromatic linearly polarized laser pulse. By varying the parameters of the field, such as the phase lag and the relative amplitude between the two colors…

Chaotic Dynamics · Physics 2011-04-04 Adam Kamor , Francois Mauger , Cristel Chandre , Turgay Uzer

We report on a kinematically complete experiment on strong field double ionization of helium using laser pulses with a wavelength of 394\,nm and intensities of $3.5-5.7\times10^{14}\,W/cm^2$. Our experiment reaches the most complete level…

By using the B-spline numerical method, we investigate a two-photon double-ionization (TPDI) process of helium in a high-frequency laser field with its frequency ranging from 1.6~a.u. to 3.0~a.u. and the pulse duration ranging from 75 to…

Atomic Physics · Physics 2020-01-08 Fei Li , Facheng Jin , Yujun Yang , Jing Chen , Zong-Chao Yan , Xiaojun Liu , Bingbing Wang

We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in…

Atomic Physics · Physics 2021-05-25 Luca Argenti , Eva Lindroth

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

Atomic Physics · Physics 2021-03-10 Yimeng Wang , Chris H. Greene

We report on the observation of phase space modulations in the correlated electron emission after strong field double ionization of helium using laser pulses with a wavelength of 394~nm and an intensity of $3\cdot10^{14}$W/cm$^2$. Those…

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

In a previous publication, procedures were proposed for unambiguously extracting amplitudes for single and double ionization from a time-dependent wavepacket by effectively propagating for an infinite time following a radiation pulse. Here…

Atomic Physics · Physics 2009-11-13 A. Palacios , T. N. Rescigno , C. W. McCurdy

We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of…

Quantum Physics · Physics 2016-08-17 Morten Førre , Sølve Selstø , Raymond Nepstad
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