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Multidimensional spectroscopy has a long history originating from nuclear magnetic resonance, and has now found widespread application at infrared and optical frequencies as well. However, the energy scales of traditional multidimensional…

Materials Science · Physics 2025-02-12 Albert Liu

A method for estimating the relative content of crystalline phases of a multiphase sample, based on probabilistic analysis of the intensities of the diffraction pattern reflexes, has been developed. The method is based on the introduction…

Materials Science · Physics 2023-11-21 S. V. Gabielkov , I. V. Zhyganiuk , A. D. Skorbun

There is renewed interest in the structure of the essential amino acid Phenylalanine in the solid state. Three new polymorphs were found in the years 2012 to 2014. Here, we investigate the structure, stability, and energetical ordering of…

Chemical Physics · Physics 2024-12-18 Thomas A. Niehaus , Emilien Prost , Vincent Loriot , Franck Lépine , Luc Bergé , Stefan Skupin

Terahertz Time-Domain Spectroscopy is a powerful technique for extracting the low-frequency optical properties of materials. However, the optical constants are difficult to determine directly from the experimental transfer function, such…

Optics · Physics 2025-06-02 Kamyar Rashidi , Matthew Y. Sfeir

Terahertz technology is mature enough for large-volume sensing applications. However, Dook van Mechelen says there are a few hurdles preventing its industrial debut. THz spectroscopy has a number of advantages that point to abundant…

Optics · Physics 2015-11-10 Dook van Mechelen

We review well-known signatures of disorder in crystallographic and inelastic neutron scattering data. We show that these can arise from different types of disorder, corresponding to different values of the system entropy. Correlating the…

Materials Science · Physics 2023-08-15 Anthony E. Phillips , Helen C. Walker

The main purpose of this article is to alert spectroscopists, particularly those involved in surveys, to the fact that rapidly pulsating sources induce periodic structures in spectra. This would allow the detection of new classes of objects…

High Energy Astrophysical Phenomena · Physics 2010-03-18 Ermanno F. Borra

Model selection in clustering requires (i) to specify a suitable clustering principle and (ii) to control the model order complexity by choosing an appropriate number of clusters depending on the noise level in the data. We advocate an…

Information Theory · Computer Science 2010-06-03 Joachim M. Buhmann

Spintronic terahertz emitters (STEs) generate broadband terahertz (THz) radiation, which is essential for spectroscopy, imaging, and communication. The performances and the essential physical parameters of STE devices are linked to the…

The determination of chemical abundances from stellar spectra is considered a mature field of astrophysics. Digital spectra of stars are recorded and processed with standard techniques, much like samples in the biological sciences.…

Astrophysics · Physics 2007-05-23 C. Allende Prieto

The large amount of powder diffraction data for which the corresponding crystal structures have not yet been identified suggests the existence of numerous undiscovered, physically relevant crystal structure prototypes. In this paper, we…

Materials Science · Physics 2024-10-31 Abhijith S. Parackal , Rhys E. A. Goodall , Felix A. Faber , Rickard Armiento

A method is presented for modelling the optical properties of a photonic crystal structure mounted on a substrate which is thick enough that the light reflected from the back is incoherent with reflections from the front. Transmission and…

Optics · Physics 2010-12-17 D. M. Whittaker , G. A. Gehring

Coherent continuous wave (CW) terahertz spectroscopy is an extremely valuable technique that allows for the interrogation of systems that exhibit narrow resonances in the terahertz (THz) frequency range, such as high-quality (high-Q) THz…

Optics · Physics 2019-05-01 Dominik Walter Vogt , Miro Erkintalo , Rainer Leonhardt

We propose a high resolution spatial diagnostic method via inserting a millimeter-gap grating into the collimated terahertz beam to monitor the minute variation of the terahertz beam in strong-field terahertz sources, which is difficult to…

Increasing the average power of broadband, few-cycle terahertz (THz) sources is currently a topic of intense investigation, fueled by recent immense progress in high average power femtosecond laser driving sources at 1030 nm. However, many…

THz near field microscopy opens a new frontier in material science. High spatial resolution requires the detection crystal to have uniform and reproducible response. We present the THz near field spatial and temporal response of ZnTe and…

Materials Science · Physics 2015-07-24 Katherine A. Niessen , A. G. Markelz

The ability to understand the atomistic mechanisms that occur in the solid phase transition is of crucial importance in materials research. To investigate the displacive phase transition at the atomic scale, we have implemented a numerical…

Materials Science · Physics 2025-06-06 Qiang Zhu , Byungkyun Kang , Kevin Parrish

The diffraction technique is widely used in the determination of crystal structures and is one of the bases for the modern science and technology. All related structure determination methods are based on the assumption that perfect single…

Materials Science · Physics 2020-08-25 Yihan Shen , Yibin Jiang , Jianhua Lin , Cheng Wang , Junliang Sun

Topological defects (TDs) are crucial for understanding important physical properties of crystalline materials including mechanical failure, ion transport, and two-dimensional melting. This concept has not translated to disordered materials…

Materials Science · Physics 2026-04-09 Matteo Baggioli , Michael L. Falk , Walter Kob